Neutron studies of gauge field and charge in Ih heavy-water ice

Morris, D. J.  P.; Siemensmeyer, K.; Hoffmann, J. -U.; Klemke, B.; Glavatskyi, I.; Seiffert, K.; Tennant, D. A.; Isakov, S. V.; Sondhi, S. L.; Moessner, R.

doi:10.1103/PhysRevB.99.174111

Title: Neutron studies of gauge field and charge in Ih heavy-water ice

Abstract

The distinctive character of water ice results from the partially disordered combination of covalent and hydrogen bonds in the network of hydrogen and oxygen atoms. The nontrivial hydrogen correlations we report in diffuse neutron scattering are analytically fit via a description of this state as a topological system exhibiting an emergent gauge field. This enables the density of correlation-terminating point defects to be decided as one defect per 500 oxygen sites at 30 K. Application of an analytical model of ice paves the way towards a detailed understanding of this ubiquitous solid.

Authors:

Morris, D. J. P. ^[1]; Siemensmeyer, K. ^[2]; Hoffmann, J. -U. ^[2]; Klemke, B. ^[2]; Glavatskyi, I. ^[3]; Seiffert, K. ^[4]; Tennant, D. A. ^[5]; Isakov, S. V. ^[6]; Sondhi, S. L. ^[7]; Moessner, R. ^[8]

Xavier Univ., Cincinnati, OH (United States)
Helmholtz-Zentrum Berlin, Berlin (Germany)
Scienion AG, Berlin (Germany)
Technische Universität Berlin, Berlin (Germany)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Google Inc., Zurich (Switzerland)
Princeton Univ., NJ (United States)
Max Planck Society, Dresden (Germany). Max Planck Inst. for the Physics of Complex Systems

Publication Date:: 2019-05-20

Research Org.:: Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

Sponsoring Org.:: USDOE

OSTI Identifier:: 1515645

Alternate Identifier(s):: OSTI ID: 1514736

Grant/Contract Number:: AC05-00OR22725; 9566

Resource Type:: Accepted Manuscript

Journal Name:: Physical Review B

Additional Journal Information:: Journal Volume: 99; Journal Issue: 17; Journal ID: ISSN 2469-9950

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY

Citation Formats


                    Morris, D. J.  P., Siemensmeyer, K., Hoffmann, J. -U., Klemke, B., Glavatskyi, I., Seiffert, K., Tennant, D. A., Isakov, S. V., Sondhi, S. L., and Moessner, R. Neutron studies of gauge field and charge in Ih heavy-water ice.  United States: N. p., 2019. 
Web.  doi:10.1103/PhysRevB.99.174111.

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                    Morris, D. J.  P., Siemensmeyer, K., Hoffmann, J. -U., Klemke, B., Glavatskyi, I., Seiffert, K., Tennant, D. A., Isakov, S. V., Sondhi, S. L., & Moessner, R. Neutron studies of gauge field and charge in Ih heavy-water ice.  United States.  https://doi.org/10.1103/PhysRevB.99.174111

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                    Morris, D. J.  P., Siemensmeyer, K., Hoffmann, J. -U., Klemke, B., Glavatskyi, I., Seiffert, K., Tennant, D. A., Isakov, S. V., Sondhi, S. L., and Moessner, R. Mon .  
"Neutron studies of gauge field and charge in Ih heavy-water ice".  United States.  https://doi.org/10.1103/PhysRevB.99.174111.  https://www.osti.gov/servlets/purl/1515645.

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@article{osti_1515645,

  title        = {Neutron studies of gauge field and charge in Ih heavy-water ice},

  author       = {Morris, D. J.  P. and Siemensmeyer, K. and Hoffmann, J. -U. and Klemke, B. and Glavatskyi, I. and Seiffert, K. and Tennant, D. A. and Isakov, S. V. and Sondhi, S. L. and Moessner, R.},

  abstractNote = {The distinctive character of water ice results from the partially disordered combination of covalent and hydrogen bonds in the network of hydrogen and oxygen atoms. The nontrivial hydrogen correlations we report in diffuse neutron scattering are analytically fit via a description of this state as a topological system exhibiting an emergent gauge field. This enables the density of correlation-terminating point defects to be decided as one defect per 500 oxygen sites at 30 K. Application of an analytical model of ice paves the way towards a detailed understanding of this ubiquitous solid.},

  doi          = {10.1103/PhysRevB.99.174111},

  journal      = {Physical Review B},

  number       = 17,

  volume       = 99,

  place        = {United States},

  year         = {2019},

  month        = {5}

}

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Similar Records

Title: Neutron studies of gauge field and charge in Ih heavy-water ice

Abstract

Citation Formats

Analytical theory for proton correlations in common-water ice I h journal, June 2015

A Theory of Water and Ionic Solution, with Particular Reference to Hydrogen and Hydroxyl Ions journal, August 1933

The Structure and Entropy of Ice and of Other Crystals with Some Randomness of Atomic Arrangement journal, December 1935

Elastic diffuse neutron scattering due to D-D correlation functions seen in Ih ice journal, August 1980

Disorder in ice Ih journal, January 1995

Diffuse scattering in Ih ice journal, June 2014

The 3-dimensional eight vertex model and the proton-proton correlation functions in ice journal, May 1972

Theory of the dielectric constant of ice journal, November 1979

Correlations in ice-rule ferroelectrics journal, June 1980

Polarization fluctuations in ferroelectric models journal, January 1981

Frustration model of proton disorder in ice journal, October 1984

“Symmetrical” phase and collective excitations in the proton system of ice journal, June 1999

Ice: A strongly correlated proton system journal, July 2006

Classical and quantum theories of proton disorder in hexagonal water ice journal, March 2016

The “Coulomb Phase” in Frustrated Systems journal, August 2010

Spin Ice, Fractionalization, and Topological Order journal, March 2012

Neutron scattering lengths and cross sections journal, January 1992

A Technique for the Growth of high Quality Single Crystals of ice journal, March 1987

E2: The Flat-Cone Diffractometer at BER II journal, January 2018

Unit cells for the simulation of hexagonal ice journal, January 1997

Structure and Properties of Ice journal, April 1952

Properties and lattice imfections of ice crystals and the behaviour of H2O-HF solid solutions journal, December 1962

Mechanistic study of proton transfer and H∕D exchange in ice films at low temperatures (100–140K) journal, August 2007

Multiple-trapping model of dielectric relaxation of the ice I h journal, November 2017

Colloquium : Understanding ion motion in disordered solids from impedance spectroscopy scaling journal, July 2009

Dielectric Anisotropy in Ice Ih journal, June 1978

The crystallography of correlated disorder journal, May 2015

Neutron study of the topological flux model of hydrogen ions in water ice dataset, January 2018

Theory of the dielectric constant of ice journal, October 1981

Spin Ice, Fractionalization and Topological Order text, January 2011

Analytical theory for proton correlations in common water ice $I_h$ text, January 2015

Analytical theory for proton correlations in common-water ice $I_{h}$
journal, June 2015

A Theory of Water and Ionic Solution, with Particular Reference to Hydrogen and Hydroxyl Ions
journal, August 1933

The Structure and Entropy of Ice and of Other Crystals with Some Randomness of Atomic Arrangement
journal, December 1935

Elastic diffuse neutron scattering due to D-D correlation functions seen in Ih ice
journal, August 1980

Disorder in ice Ih
journal, January 1995

Diffuse scattering in Ih ice
journal, June 2014

The 3-dimensional eight vertex model and the proton-proton correlation functions in ice
journal, May 1972

Theory of the dielectric constant of ice
journal, November 1979

Correlations in ice-rule ferroelectrics
journal, June 1980

Polarization fluctuations in ferroelectric models
journal, January 1981

Frustration model of proton disorder in ice
journal, October 1984

“Symmetrical” phase and collective excitations in the proton system of ice
journal, June 1999

Ice: A strongly correlated proton system
journal, July 2006

Classical and quantum theories of proton disorder in hexagonal water ice
journal, March 2016

The “Coulomb Phase” in Frustrated Systems
journal, August 2010

Spin Ice, Fractionalization, and Topological Order
journal, March 2012

Neutron scattering lengths and cross sections
journal, January 1992

A Technique for the Growth of high Quality Single Crystals of ice
journal, March 1987

E2: The Flat-Cone Diffractometer at BER II
journal, January 2018

Unit cells for the simulation of hexagonal ice
journal, January 1997

Structure and Properties of Ice
journal, April 1952

Properties and lattice imfections of ice crystals and the behaviour of H2O-HF solid solutions
journal, December 1962

Mechanistic study of proton transfer and H∕D exchange in ice films at low temperatures (100–140K)
journal, August 2007

Multiple-trapping model of dielectric relaxation of the ice I _h
journal, November 2017

Colloquium : Understanding ion motion in disordered solids from impedance spectroscopy scaling
journal, July 2009

Dielectric Anisotropy in Ice Ih
journal, June 1978

The crystallography of correlated disorder
journal, May 2015

Neutron study of the topological flux model of hydrogen ions in water ice
dataset, January 2018

Theory of the dielectric constant of ice
journal, October 1981

Spin Ice, Fractionalization and Topological Order
text, January 2011

Analytical theory for proton correlations in common water ice $I_h$
text, January 2015