DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Fragility of Fermi arcs in Dirac semimetals

Abstract

We use tunable, vacuum ultraviolet laser based angle-resolved photoemission spectroscopy and density functional theory (DFT) calculations to study the electronic properties of Dirac semimetal candidate cubic PtBi2 . In addition to bulk electronic states we also find surface states in PtBi2, which is expected as PtBi2 was theoretically predicated to be a candidate Dirac semimetal. The surface states are also well reproduced from DFT band calculations. Impressively, the topological surface states form Fermi contours rather than double Fermi arcs that were observed in Na3Bi. The surface bands forming the Fermi contours merge with bulk bands in proximity to the Dirac point projections, as expected. Our data validate the existence of Dirac states in PtBi2 and reveal the fragility of the Fermi arcs in Dirac semimetals. Because the Fermi arcs are not topologically protected in general, they can be deformed into Fermi contours, as proposed by M. Kargarian et al. [Proc. Natl. Acad. Sci. USA 113, 8648 (2016)]. Our results demonstrate the validity of this theory in PtBi2 .

Authors:
 [1];  [1];  [2];  [1];  [1];  [1];  [1];  [1];  [1];  [1];  [1]
  1. Ames Lab., Ames, IA (United States); Iowa State Univ., Ames, IA (United States)
  2. Ames Lab., Ames, IA (United States)
Publication Date:
Research Org.:
Ames Laboratory (AMES), Ames, IA (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division; USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI Identifier:
1514886
Alternate Identifier(s):
OSTI ID: 1507457
Report Number(s):
IS-J-9936
Journal ID: ISSN 2469-9950; PRBMDO
Grant/Contract Number:  
AC02-07CH11358; GBMF4411; DMR-1420451
Resource Type:
Accepted Manuscript
Journal Name:
Physical Review B
Additional Journal Information:
Journal Volume: 99; Journal Issue: 16; Journal ID: ISSN 2469-9950
Publisher:
American Physical Society (APS)
Country of Publication:
United States
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY

Citation Formats

Wu, Yun, Jo, Na Hyun, Wang, Lin-Lin, Schmidt, Connor A., Neilson, Kathryn M., Schrunk, Benjamin, Swatek, Przemyslaw, Eaton, Andrew, Bud'ko, S. L., Canfield, P. C., and Kaminski, Adam. Fragility of Fermi arcs in Dirac semimetals. United States: N. p., 2019. Web. doi:10.1103/PhysRevB.99.161113.
Wu, Yun, Jo, Na Hyun, Wang, Lin-Lin, Schmidt, Connor A., Neilson, Kathryn M., Schrunk, Benjamin, Swatek, Przemyslaw, Eaton, Andrew, Bud'ko, S. L., Canfield, P. C., & Kaminski, Adam. Fragility of Fermi arcs in Dirac semimetals. United States. https://doi.org/10.1103/PhysRevB.99.161113
Wu, Yun, Jo, Na Hyun, Wang, Lin-Lin, Schmidt, Connor A., Neilson, Kathryn M., Schrunk, Benjamin, Swatek, Przemyslaw, Eaton, Andrew, Bud'ko, S. L., Canfield, P. C., and Kaminski, Adam. Wed . "Fragility of Fermi arcs in Dirac semimetals". United States. https://doi.org/10.1103/PhysRevB.99.161113. https://www.osti.gov/servlets/purl/1514886.
@article{osti_1514886,
title = {Fragility of Fermi arcs in Dirac semimetals},
author = {Wu, Yun and Jo, Na Hyun and Wang, Lin-Lin and Schmidt, Connor A. and Neilson, Kathryn M. and Schrunk, Benjamin and Swatek, Przemyslaw and Eaton, Andrew and Bud'ko, S. L. and Canfield, P. C. and Kaminski, Adam},
abstractNote = {We use tunable, vacuum ultraviolet laser based angle-resolved photoemission spectroscopy and density functional theory (DFT) calculations to study the electronic properties of Dirac semimetal candidate cubic PtBi2 . In addition to bulk electronic states we also find surface states in PtBi2, which is expected as PtBi2 was theoretically predicated to be a candidate Dirac semimetal. The surface states are also well reproduced from DFT band calculations. Impressively, the topological surface states form Fermi contours rather than double Fermi arcs that were observed in Na3Bi. The surface bands forming the Fermi contours merge with bulk bands in proximity to the Dirac point projections, as expected. Our data validate the existence of Dirac states in PtBi2 and reveal the fragility of the Fermi arcs in Dirac semimetals. Because the Fermi arcs are not topologically protected in general, they can be deformed into Fermi contours, as proposed by M. Kargarian et al. [Proc. Natl. Acad. Sci. USA 113, 8648 (2016)]. Our results demonstrate the validity of this theory in PtBi2 .},
doi = {10.1103/PhysRevB.99.161113},
journal = {Physical Review B},
number = 16,
volume = 99,
place = {United States},
year = {Wed Apr 17 00:00:00 EDT 2019},
month = {Wed Apr 17 00:00:00 EDT 2019}
}

Journal Article:

Citation Metrics:
Cited by: 17 works
Citation information provided by
Web of Science

Save / Share:

Works referenced in this record:

Generalized Gradient Approximation Made Simple
journal, October 1996

  • Perdew, John P.; Burke, Kieron; Ernzerhof, Matthias
  • Physical Review Letters, Vol. 77, Issue 18, p. 3865-3868
  • DOI: 10.1103/PhysRevLett.77.3865

Quick iterative scheme for the calculation of transfer matrices: application to Mo (100)
journal, May 1984

  • Sancho, M. P. Lopez; Sancho, J. M. Lopez; Rubio, J.
  • Journal of Physics F: Metal Physics, Vol. 14, Issue 5
  • DOI: 10.1088/0305-4608/14/5/016

Use of frit-disc crucibles for routine and exploratory solution growth of single crystalline samples
journal, December 2015


Spectroscopic evidence for a type II Weyl semimetallic state in MoTe2
journal, July 2016

  • Huang, Lunan; McCormick, Timothy M.; Ochi, Masayuki
  • Nature Materials, Vol. 15, Issue 11
  • DOI: 10.1038/nmat4685

Weyl and Dirac semimetals in three-dimensional solids
journal, January 2018


Projector augmented-wave method
journal, December 1994


Maximally localized Wannier functions: Theory and applications
journal, October 2012

  • Marzari, Nicola; Mostofi, Arash A.; Yates, Jonathan R.
  • Reviews of Modern Physics, Vol. 84, Issue 4
  • DOI: 10.1103/RevModPhys.84.1419

Are the surface Fermi arcs in Dirac semimetals topologically protected?
journal, July 2016

  • Kargarian, Mehdi; Randeria, Mohit; Lu, Yuan-Ming
  • Proceedings of the National Academy of Sciences, Vol. 113, Issue 31
  • DOI: 10.1073/pnas.1524787113

Efficiency of ab-initio total energy calculations for metals and semiconductors using a plane-wave basis set
journal, July 1996


Large, non-saturating magnetoresistance in WTe2
journal, September 2014

  • Ali, Mazhar N.; Xiong, Jun; Flynn, Steven
  • Nature, Vol. 514, Issue 7521
  • DOI: 10.1038/nature13763

Simple scheme for surface-band calculations. II. The Green's function
journal, May 1981


Three-dimensional Dirac semimetal and quantum transport in Cd 3 As 2
journal, September 2013


Observation of Fermi arc surface states in a topological metal
journal, December 2014


Dirac node arcs in PtSn4
journal, April 2016

  • Wu, Yun; Wang, Lin-Lin; Mun, Eundeok
  • Nature Physics, Vol. 12, Issue 7
  • DOI: 10.1038/nphys3712

Special points for Brillouin-zone integrations
journal, June 1976

  • Monkhorst, Hendrik J.; Pack, James D.
  • Physical Review B, Vol. 13, Issue 12, p. 5188-5192
  • DOI: 10.1103/PhysRevB.13.5188

Time-Reversal-Breaking Weyl Fermions in Magnetic Heusler Alloys
journal, November 2016


Bulk and surface electronic structure of hexagonal structured PtBi 2 studied by angle-resolved photoemission spectroscopy
journal, December 2016


Experimental Realization of a Three-Dimensional Topological Insulator, Bi2Te3
journal, June 2009


Observation of a three-dimensional topological Dirac semimetal phase in high-mobility Cd3As2
journal, May 2014

  • Neupane, Madhab; Xu, Su-Yang; Sankar, Raman
  • Nature Communications, Vol. 5, Issue 1
  • DOI: 10.1038/ncomms4786

Evidence of Topological Surface State in Three-Dimensional Dirac Semimetal Cd3As2
journal, August 2014

  • Yi, Hemian; Wang, Zhijun; Chen, Chaoyu
  • Scientific Reports, Vol. 4, Issue 1
  • DOI: 10.1038/srep06106

Efficient iterative schemes for ab initio total-energy calculations using a plane-wave basis set
journal, October 1996


Discovery of a Three-Dimensional Topological Dirac Semimetal, Na3Bi
journal, January 2014


Observation of a large-gap topological-insulator class with a single Dirac cone on the surface
journal, May 2009

  • Xia, Y.; Qian, D.; Hsieh, D.
  • Nature Physics, Vol. 5, Issue 6, p. 398-402
  • DOI: 10.1038/nphys1274

Magnetic field effects on transport properties of PtSn 4
journal, January 2012


Experimental observation of topological Fermi arcs in type-II Weyl semimetal MoTe2
journal, September 2016

  • Deng, Ke; Wan, Guoliang; Deng, Peng
  • Nature Physics, Vol. 12, Issue 12
  • DOI: 10.1038/nphys3871

Maximally localized generalized Wannier functions for composite energy bands
journal, November 1997


Topological insulators in Bi2Se3, Bi2Te3 and Sb2Te3 with a single Dirac cone on the surface
journal, May 2009

  • Zhang, Haijun; Liu, Chao-Xing; Qi, Xiao-Liang
  • Nature Physics, Vol. 5, Issue 6, p. 438-442
  • DOI: 10.1038/nphys1270

Discovery of a Weyl fermion semimetal and topological Fermi arcs
journal, July 2015


Inhomogeneous Electron Gas
journal, November 1964


Dirac semimetal and topological phase transitions in A 3 Bi ( A = Na , K, Rb)
journal, May 2012


Non-Abelian anyons and topological quantum computation
journal, September 2008


Possible origin of linear magnetoresistance: Observation of Dirac surface states in layered PtBi 2
journal, January 2018


Growth of single crystals from metallic fluxes
journal, June 1992


Simple scheme for surface-band calculations. I
journal, May 1981


WannierTools: An open-source software package for novel topological materials
journal, March 2018


The rise of graphene
journal, March 2007

  • Geim, A. K.; Novoselov, K. S.
  • Nature Materials, Vol. 6, Issue 3, p. 183-191
  • DOI: 10.1038/nmat1849

Synthesis, physical properties, and band structure of the layered bismuthide PtBi 2
journal, October 2016


Tunable vacuum ultraviolet laser based spectrometer for angle resolved photoemission spectroscopy
journal, March 2014

  • Jiang, Rui; Mou, Daixiang; Wu, Yun
  • Review of Scientific Instruments, Vol. 85, Issue 3, Article No. 033902
  • DOI: 10.1063/1.4867517

Giant linear magneto-resistance in nonmagnetic PtBi 2
journal, June 2016

  • Yang, Xiaojun; Bai, Hua; Wang, Zhen
  • Applied Physics Letters, Vol. 108, Issue 25
  • DOI: 10.1063/1.4954272

Fermi Arcs and Their Topological Character in the Candidate Type-II Weyl Semimetal MoTe 2
journal, August 2016


Three-dimensional Dirac semimetals: Design principles and predictions of new materials
journal, May 2015


Ultrahigh mobility and giant magnetoresistance in the Dirac semimetal Cd3As2
journal, November 2014

  • Liang, Tian; Gibson, Quinn; Ali, Mazhar N.
  • Nature Materials, Vol. 14, Issue 3
  • DOI: 10.1038/nmat4143

A stable three-dimensional topological Dirac semimetal Cd3As2
journal, May 2014

  • Liu, Z. K.; Jiang, J.; Zhou, B.
  • Nature Materials, Vol. 13, Issue 7
  • DOI: 10.1038/nmat3990

Extremely Large Magnetoresistance in a Topological Semimetal Candidate Pyrite PtBi 2
journal, June 2017


Maximally localized Wannier functions for entangled energy bands
journal, December 2001


Highly convergent schemes for the calculation of bulk and surface Green functions
journal, April 1985

  • Sancho, M. P. Lopez; Sancho, J. M. Lopez; Sancho, J. M. L.
  • Journal of Physics F: Metal Physics, Vol. 15, Issue 4
  • DOI: 10.1088/0305-4608/15/4/009

Self-Consistent Equations Including Exchange and Correlation Effects
journal, November 1965


The rise of graphene
book, August 2009

  • Rodgers, Peter; Geim, A. K.; Novoselov, K. S.
  • Nanoscience and Technology: A Collection of Reviews from Nature Journals, p. 11-19
  • DOI: 10.1142/9789814287005_0002

High-resolution X-ray luminescence extension imaging
journal, February 2021


Electronic structure of AlFeN films exhibiting crystallographic orientation change from c- to a-axis with Fe concentrations and annealing effect
journal, February 2020


WannierTools: An open-source software package for novel topological materials
text, January 2018


Non-Abelian Anyons and Topological Quantum Computation
text, January 2007


Maximally localized Wannier functions: Theory and applications
text, January 2011


Discovery of a Three-dimensional Topological Dirac Semimetal, Na3Bi
text, January 2013


Ultrahigh mobility and giant magnetoresistance in the Dirac semimetal Cd$_3$As$_2$
text, January 2014


Discovery of a Weyl Fermion Semimetal and Topological Fermi Arcs
text, January 2015


Use of frit-disc crucibles for routine and exploratory solution growth of single crystalline samples
text, January 2015


Spectroscopic evidence for type II Weyl semimetal state in MoTe2
text, January 2016


Giant Linear Magneto-resistance in Nonmagnetic PtBi2
text, January 2016


WannierTools: An open-source software package for novel topological materials
text, January 2017


Weyl and Dirac Semimetals in Three Dimensional Solids
text, January 2017


Maximally-localized Wannier functions for entangled energy bands
text, January 2001


Works referencing / citing this record:

Type-II Dirac states in full Heusler compounds X InPd 2 ( X = Ti, Zr, and Hf)
journal, December 2019