Cluster radioactivity of Og176118294

Matheson, Zachary; Giuliani, Samuel A.; Nazarewicz, Witold; Sadhukhan, Jhilam; Schunck, Nicolas

doi:10.1103/PhysRevC.99.041304

Title: Cluster radioactivity of ${}_{118}^{294}{Og}_{176}$

Abstract

According to theory, cluster radioactivity becomes an important decay mode in superheavy nuclei. We suggest that the strongly asymmetric fission, or cluster emission, is in fact the dominant fission channel for ${}_{118}^{294}{Og}_{176}$ , which is currently the heaviest synthetic isotope known. Our theoretical approach incorporates critical features of fission dynamics, including quantum tunneling and stochastic dynamics up to scission. We show that despite appreciable differences in static fission properties such as fission barriers and spontaneous fission lifetimes, the prediction of cluster radioactivity in ${}_{118}^{294}{Og}_{176}$ is robust with respect to the details of calculations, including the choice of energy density functional, collective inertia, and strength of the dissipation term.

Authors:

Matheson, Zachary ^[1]; Giuliani, Samuel A. ^[1]; Nazarewicz, Witold ^[1]; Sadhukhan, Jhilam ^[2]; Schunck, Nicolas ^[3]

Michigan State Univ., East Lansing, MI (United States)
Variable Energy Cyclotron Centre, Kolkata (India); Homi Bhabha National Inst., Mumbai (India)
Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)

Publication Date:: 2019-04-29

Research Org.:: Michigan State Univ., East Lansing, MI (United States); Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)

Sponsoring Org.:: USDOE National Nuclear Security Administration (NNSA); USDOE Office of Science (SC), Workforce Development for Teachers and Scientists (WDTS); USDOE Office of Science (SC), Nuclear Physics (NP)

OSTI Identifier:: 1513813

Alternate Identifier(s):: OSTI ID: 1509757; OSTI ID: 1557934; OSTI ID: 1615741

Report Number(s):: LLNL-JRNL-782120
Journal ID: ISSN 2469-9985; PRVCAN

Grant/Contract Number:: NA0003885; SC0013365; SC0014664; AC52-07NA27344; NA0002847; SC0018083; SC0008511

Resource Type:: Accepted Manuscript

Journal Name:: Physical Review C

Additional Journal Information:: Journal Volume: 99; Journal Issue: 4; Journal ID: ISSN 2469-9985

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 73 NUCLEAR PHYSICS AND RADIATION PHYSICS; Physics - Nuclear physics and radiation physics

Citation Formats


                    Matheson, Zachary, Giuliani, Samuel A., Nazarewicz, Witold, Sadhukhan, Jhilam, and Schunck, Nicolas. Cluster radioactivity of Og176118294.  United States: N. p., 2019. 
Web.  doi:10.1103/PhysRevC.99.041304.

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                    Matheson, Zachary, Giuliani, Samuel A., Nazarewicz, Witold, Sadhukhan, Jhilam, & Schunck, Nicolas. Cluster radioactivity of Og176118294.  United States.  https://doi.org/10.1103/PhysRevC.99.041304

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                    Matheson, Zachary, Giuliani, Samuel A., Nazarewicz, Witold, Sadhukhan, Jhilam, and Schunck, Nicolas. Mon .  
"Cluster radioactivity of Og176118294".  United States.  https://doi.org/10.1103/PhysRevC.99.041304.  https://www.osti.gov/servlets/purl/1513813.

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@article{osti_1513813,

  title        = {Cluster radioactivity of Og176118294},

  author       = {Matheson, Zachary and Giuliani, Samuel A. and Nazarewicz, Witold and Sadhukhan, Jhilam and Schunck, Nicolas},

  abstractNote = {According to theory, cluster radioactivity becomes an important decay mode in superheavy nuclei. We suggest that the strongly asymmetric fission, or cluster emission, is in fact the dominant fission channel for Og176118294, which is currently the heaviest synthetic isotope known. Our theoretical approach incorporates critical features of fission dynamics, including quantum tunneling and stochastic dynamics up to scission. We show that despite appreciable differences in static fission properties such as fission barriers and spontaneous fission lifetimes, the prediction of cluster radioactivity in Og176118294 is robust with respect to the details of calculations, including the choice of energy density functional, collective inertia, and strength of the dissipation term.},

  doi          = {10.1103/PhysRevC.99.041304},

  journal      = {Physical Review C},

  number       = 4,

  volume       = 99,

  place        = {United States},

  year         = {2019},

  month        = {4}

}

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Works referencing / citing this record:

Fission and quasifission toward the superheavy mass region
journal, August 2019

Vardaci, E.; Itkis, M. G.; Itkis, I. M.
Journal of Physics G: Nuclear and Particle Physics, Vol. 46, Issue 10
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Effect of shell structure on the fission of sub-lead nuclei
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Scamps, Guillaume; Simenel, Cédric
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Effect of the doubly magic shell closures in ${}^{132}{Sn}$ and ${}^{208}{Pb}$ on the mass distributions of fission fragments of superheavy nuclei
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Ishizuka, C.; Zhang, X.; Usang, M. D.
Physical Review C, Vol. 101, Issue 1
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Role of dynamic pairing correlations in fission dynamics
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Bernard, R.; Giuliani, S. A.; Robledo, L. M.
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conference, December 2019

Vardaci, E.; Itkis, M. G.; Itkis, I. M.
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DOI: 10.1142/9789811209451_0037

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Title: Cluster radioactivity of Og 176 118 294

Abstract

Citation Formats

Analysis of the total kinetic energy of fission fragments with the Langevin equation journal, December 2017

Four-dimensional Langevin approach to low-energy nuclear fission of U 236 journal, December 2017

Calculated half-lives and kinetic energies for spontaneous emission of heavy ions from nuclei journal, May 1986

Some dynamical aspects of the fission process journal, May 1978

Heavy-Particle Radioactivity of Superheavy Nuclei journal, August 2011

Systematic studies of α and heavy-cluster emissions from superheavy nuclei journal, June 2018

Langevin model of low-energy fission journal, September 2017

Fission dynamics at low excitation energy journal, November 2014

Synthesis of the isotopes of elements 118 and 116 in the Cf 249 and Cm 245 + Ca 48 fusion reactions journal, October 2006

Systematic study of cluster radioactivity of superheavy nuclei journal, January 2018

Error analysis in nuclear density functional theory journal, February 2015

Fission properties of superheavy nuclei for r -process calculations journal, March 2018

Fission fragment charge and mass distributions in Pu 239 ( n , f ) in the adiabatic nuclear energy density functional theory journal, May 2016

Solution of the Skyrme-Hartree–Fock–Bogolyubovequations in the Cartesian deformed harmonic-oscillator basis. (VIII) hfodd (v2.73y): A new version of the program journal, July 2017

Search for the heaviest atomic nuclei among the products from reactions of mixed-Cf with a Ca 48 beam journal, August 2018

Spontaneous fission lifetimes from the minimization of self-consistent collective action journal, December 2013

Pairing-induced speedup of nuclear spontaneous fission journal, December 2014

Formation and distribution of fragments in the spontaneous fission of 240 Pu journal, December 2017

Fission barriers and probabilities of spontaneous fission for elements with Z≥ 100 journal, December 2015

Spontaneous fission properties of superheavy elements journal, April 2017

Towards a better parametrisation of Skyrme-like effective forces: A critical study of the SkM force journal, September 1982

Constrained hartree-fock and beyond journal, October 1989

Cluster decay of superheavy nuclei journal, March 2012

Heavy-particle radioactivity journal, April 2013

Status and perspectives of the Dubna superheavy element factory journal, January 2016

Electron and Nucleon Localization Functions of Oganesson: Approaching the Thomas-Fermi Limit journal, January 2018

Microscopic description of the fission path with the Gogny interaction journal, August 2018

Synthesis and study of properties of superheavy atoms. Factory of Superheavy Elements journal, September 2016

Production and Decay of the Heaviest Nuclei 1 293 , 294 17 and 1 294 18 journal, October 2012

Multidimensionally-constrained relativistic mean-field study of spontaneous fission: Coupling between shape and pairing degrees of freedom journal, April 2016

Nucleon localization and fragment formation in nuclear fission journal, December 2016

A dynamic analysis of spontaneous-fission half-lives journal, May 1981

A new kind of natural radioactivity journal, January 1984

Excitation-energy dependence of fission in the mercury region journal, August 2014

Microscopic description of cluster radioactivity in actinide nuclei journal, October 2011

Least action description of spontaneous fission in fermium and nobelium nuclei based on the Gogny energy density functional journal, September 2018

Microscopic modeling of mass and charge distributions in the spontaneous fission of Pu 240 journal, January 2016

Colloquium : Superheavy elements: Oganesson and beyond journal, January 2019

α decay and cluster radioactivity of nuclei of interest to the synthesis of Z = 119 , 120 isotopes journal, April 2018

Quadrupole collective inertia in nuclear fission: Cranking approximation journal, November 2011

From asymmetric to symmetric fission in the fermium isotopes within the time-dependent generator-coordinate-method formalism journal, February 2019

Microscopic theory of nuclear fission: a review journal, October 2016

Fission properties for r -process nuclei journal, February 2012

Cluster radioactivity and very asymmetric fission through compact and creviced shapes journal, March 1998

Review of even element super-heavy nuclei and search for element 120 journal, June 2016

Fission properties of the Barcelona-Catania-Paris-Madrid energy density functional journal, November 2013

Fission-fragment mass distributions from strongly damped shape evolution journal, September 2011

Non-perturbative collective inertias for fission: A comparative study journal, December 2018

Discovery of element 117: Super-heavy elements and the “island of stability”* journal, March 2017

Dynamic versus static fission paths with realistic interactions journal, November 2014

The limits of nuclear mass and charge journal, June 2018

Spontaneous fission modes and lifetimes of superheavy elements in the nuclear density functional theory journal, February 2013

Island of Heavyweights journal, February 2018

Cluster radioactivity in superheavy nuclei journal, October 2018

Shapes and α- and β-decays of superheavy nuclei journal, December 2015

Fission and quasifission toward the superheavy mass region journal, August 2019

Deformed shell effects in Ca 48 + Bk 249 quasifission fragments journal, August 2019

Effect of shell structure on the fission of sub-lead nuclei journal, October 2019

Effect of the doubly magic shell closures in Sn 132 and Pb 208 on the mass distributions of fission fragments of superheavy nuclei journal, January 2020

Role of dynamic pairing correlations in fission dynamics journal, June 2019

Fission and Quasifission Toward the Superheavy Mass Region conference, December 2019

Title: Cluster radioactivity of ${}_{118}^{294}{Og}_{176}$

Analysis of the total kinetic energy of fission fragments with the Langevin equation
journal, December 2017

Four-dimensional Langevin approach to low-energy nuclear fission of ${}^{236}U$
journal, December 2017

Calculated half-lives and kinetic energies for spontaneous emission of heavy ions from nuclei
journal, May 1986

Some dynamical aspects of the fission process
journal, May 1978

Heavy-Particle Radioactivity of Superheavy Nuclei
journal, August 2011

Systematic studies of α and heavy-cluster emissions from superheavy nuclei
journal, June 2018

Langevin model of low-energy fission
journal, September 2017

Fission dynamics at low excitation energy
journal, November 2014

Synthesis of the isotopes of elements 118 and 116 in the ${}^{249}{Cf}$ and ${}^{245}{Cm} + {}^{48}{Ca}$ fusion reactions
journal, October 2006

Systematic study of cluster radioactivity of superheavy nuclei
journal, January 2018

Error analysis in nuclear density functional theory
journal, February 2015

Fission properties of superheavy nuclei for $r$ -process calculations
journal, March 2018

Fission fragment charge and mass distributions in ${}^{239}{Pu} (n, f)$ in the adiabatic nuclear energy density functional theory
journal, May 2016

Solution of the Skyrme-Hartree–Fock–Bogolyubovequations in the Cartesian deformed harmonic-oscillator basis. (VIII) hfodd (v2.73y): A new version of the program
journal, July 2017

Search for the heaviest atomic nuclei among the products from reactions of mixed-Cf with a ${}^{48}{Ca}$ beam
journal, August 2018

Spontaneous fission lifetimes from the minimization of self-consistent collective action
journal, December 2013

Pairing-induced speedup of nuclear spontaneous fission
journal, December 2014

Formation and distribution of fragments in the spontaneous fission of $^{240} Pu$
journal, December 2017

Fission barriers and probabilities of spontaneous fission for elements with Z≥ 100
journal, December 2015

Spontaneous fission properties of superheavy elements
journal, April 2017

Towards a better parametrisation of Skyrme-like effective forces: A critical study of the SkM force
journal, September 1982

Constrained hartree-fock and beyond
journal, October 1989

Cluster decay of superheavy nuclei
journal, March 2012

Heavy-particle radioactivity
journal, April 2013

Status and perspectives of the Dubna superheavy element factory
journal, January 2016

Electron and Nucleon Localization Functions of Oganesson: Approaching the Thomas-Fermi Limit
journal, January 2018

Microscopic description of the fission path with the Gogny interaction
journal, August 2018

Synthesis and study of properties of superheavy atoms. Factory of Superheavy Elements
journal, September 2016

Production and Decay of the Heaviest Nuclei ${}^{293, 294}1 17$ and ${}^{294}1 18$
journal, October 2012

Multidimensionally-constrained relativistic mean-field study of spontaneous fission: Coupling between shape and pairing degrees of freedom
journal, April 2016

Nucleon localization and fragment formation in nuclear fission
journal, December 2016

A dynamic analysis of spontaneous-fission half-lives
journal, May 1981

A new kind of natural radioactivity
journal, January 1984

Excitation-energy dependence of fission in the mercury region
journal, August 2014

Microscopic description of cluster radioactivity in actinide nuclei
journal, October 2011

Least action description of spontaneous fission in fermium and nobelium nuclei based on the Gogny energy density functional
journal, September 2018

Microscopic modeling of mass and charge distributions in the spontaneous fission of ${}^{240}{Pu}$
journal, January 2016

Colloquium : Superheavy elements: Oganesson and beyond
journal, January 2019

$α$ decay and cluster radioactivity of nuclei of interest to the synthesis of $Z = 119$ , 120 isotopes
journal, April 2018

Quadrupole collective inertia in nuclear fission: Cranking approximation
journal, November 2011

From asymmetric to symmetric fission in the fermium isotopes within the time-dependent generator-coordinate-method formalism
journal, February 2019

Microscopic theory of nuclear fission: a review
journal, October 2016

Fission properties for $r$ -process nuclei
journal, February 2012

Cluster radioactivity and very asymmetric fission through compact and creviced shapes
journal, March 1998

Review of even element super-heavy nuclei and search for element 120
journal, June 2016

Fission properties of the Barcelona-Catania-Paris-Madrid energy density functional
journal, November 2013

Fission-fragment mass distributions from strongly damped shape evolution
journal, September 2011

Non-perturbative collective inertias for fission: A comparative study
journal, December 2018

Discovery of element 117: Super-heavy elements and the “island of stability”*
journal, March 2017

Dynamic versus static fission paths with realistic interactions
journal, November 2014

The limits of nuclear mass and charge
journal, June 2018

Spontaneous fission modes and lifetimes of superheavy elements in the nuclear density functional theory
journal, February 2013

Island of Heavyweights
journal, February 2018

Cluster radioactivity in superheavy nuclei
journal, October 2018

Shapes and α- and β-decays of superheavy nuclei
journal, December 2015

Fission and quasifission toward the superheavy mass region
journal, August 2019

Deformed shell effects in Ca 48 + Bk 249 quasifission fragments
journal, August 2019

Effect of shell structure on the fission of sub-lead nuclei
journal, October 2019

Effect of the doubly magic shell closures in ${}^{132}{Sn}$ and ${}^{208}{Pb}$ on the mass distributions of fission fragments of superheavy nuclei
journal, January 2020

Role of dynamic pairing correlations in fission dynamics
journal, June 2019

Fission and Quasifission Toward the Superheavy Mass Region
conference, December 2019