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Title: Phonon localization in heat conduction

Abstract

Nondiffusive phonon thermal transport, extensively observed in nanostructures, has largely been attributed to classical size effects, ignoring the wave nature of phonons. We report localization behavior in phonon heat conduction due to multiple scattering and interference events of broadband phonons, by measuring the thermal conductivities of GaAs/AlAs superlattices with ErAs nanodots randomly distributed at the interfaces. With an increasing number of superlattice periods, the measured thermal conductivities near room temperature increased and eventually saturated, indicating a transition from ballistic to diffusive transport. In contrast, at cryogenic temperatures the thermal conductivities first increased but then decreased, signaling phonon wave localization, as supported by atomistic Green's function simulations. The discovery of phonon localization suggests a new path forward for engineering phonon thermal transport.

Authors:
ORCiD logo [1];  [1];  [2]; ORCiD logo [1]; ORCiD logo [3]; ORCiD logo [1]; ORCiD logo [1];  [4];  [5];  [6]; ORCiD logo [6]; ORCiD logo [7]; ORCiD logo [7]; ORCiD logo [8]; ORCiD logo [6];  [9];  [2]; ORCiD logo [1]
  1. Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States). Dept. of Mechanical Engineering
  2. Univ. of California, Santa Barbara, CA (United States). Materials Dept.
  3. Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States). Dept. of Electrical Engineering and Computer Science
  4. Argonne National Lab. (ANL), Argonne, IL (United States). Advanced Photon Source; Univ. of Science and Technology of China, Hefei (China). National Synchrotron Radiation Lab.
  5. Argonne National Lab. (ANL), Argonne, IL (United States). Advanced Photon Source
  6. Brookhaven National Lab. (BNL), Upton, NY (United States). Condensed Matter Physics and Materials Science Dept.
  7. National Inst. of Standards and Technology (NIST), Gaithersburg, MD (United States). Center for Neutron Research
  8. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Center for Nanophase Materials Science
  9. Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States). Dept. of Electrical Engineering and Computer Science. Dept. of Physics
Publication Date:
Research Org.:
Brookhaven National Lab. (BNL), Upton, NY (United States); Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States); Univ. of California, Santa Barbara, CA (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Argonne National Lab. (ANL), Argonne, IL (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
OSTI Identifier:
1511938
Alternate Identifier(s):
OSTI ID: 1491683; OSTI ID: 1504458
Report Number(s):
BNL-210909-2019-JAAM
Journal ID: ISSN 2375-2548
Grant/Contract Number:  
SC0012704; SC0001299; SC0001009; AC02-06CH11357; AC05-00OR22725
Resource Type:
Accepted Manuscript
Journal Name:
Science Advances
Additional Journal Information:
Journal Volume: 4; Journal Issue: 12; Journal ID: ISSN 2375-2548
Publisher:
AAAS
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; 42 ENGINEERING

Citation Formats

Luckyanova, M. N., Mendoza, J., Lu, H., Song, B., Huang, S., Zhou, J., Li, M., Dong, Y., Zhou, H., Garlow, J., Wu, L., Kirby, B. J., Grutter, A. J., Puretzky, A. A., Zhu, Y., Dresselhaus, M. S., Gossard, A., and Chen, G.. Phonon localization in heat conduction. United States: N. p., 2018. Web. doi:10.1126/sciadv.aat9460.
Luckyanova, M. N., Mendoza, J., Lu, H., Song, B., Huang, S., Zhou, J., Li, M., Dong, Y., Zhou, H., Garlow, J., Wu, L., Kirby, B. J., Grutter, A. J., Puretzky, A. A., Zhu, Y., Dresselhaus, M. S., Gossard, A., & Chen, G.. Phonon localization in heat conduction. United States. doi:10.1126/sciadv.aat9460.
Luckyanova, M. N., Mendoza, J., Lu, H., Song, B., Huang, S., Zhou, J., Li, M., Dong, Y., Zhou, H., Garlow, J., Wu, L., Kirby, B. J., Grutter, A. J., Puretzky, A. A., Zhu, Y., Dresselhaus, M. S., Gossard, A., and Chen, G.. Fri . "Phonon localization in heat conduction". United States. doi:10.1126/sciadv.aat9460. https://www.osti.gov/servlets/purl/1511938.
@article{osti_1511938,
title = {Phonon localization in heat conduction},
author = {Luckyanova, M. N. and Mendoza, J. and Lu, H. and Song, B. and Huang, S. and Zhou, J. and Li, M. and Dong, Y. and Zhou, H. and Garlow, J. and Wu, L. and Kirby, B. J. and Grutter, A. J. and Puretzky, A. A. and Zhu, Y. and Dresselhaus, M. S. and Gossard, A. and Chen, G.},
abstractNote = {Nondiffusive phonon thermal transport, extensively observed in nanostructures, has largely been attributed to classical size effects, ignoring the wave nature of phonons. We report localization behavior in phonon heat conduction due to multiple scattering and interference events of broadband phonons, by measuring the thermal conductivities of GaAs/AlAs superlattices with ErAs nanodots randomly distributed at the interfaces. With an increasing number of superlattice periods, the measured thermal conductivities near room temperature increased and eventually saturated, indicating a transition from ballistic to diffusive transport. In contrast, at cryogenic temperatures the thermal conductivities first increased but then decreased, signaling phonon wave localization, as supported by atomistic Green's function simulations. The discovery of phonon localization suggests a new path forward for engineering phonon thermal transport.},
doi = {10.1126/sciadv.aat9460},
journal = {Science Advances},
number = 12,
volume = 4,
place = {United States},
year = {2018},
month = {12}
}

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Works referenced in this record:

Silicon nanowires as efficient thermoelectric materials
journal, January 2008

  • Boukai, Akram I.; Bunimovich, Yuri; Tahir-Kheli, Jamil
  • Nature, Vol. 451, Issue 7175, p. 168-171
  • DOI: 10.1038/nature06458

QUANTUM ESPRESSO: a modular and open-source software project for quantum simulations of materials
journal, September 2009

  • Giannozzi, Paolo; Baroni, Stefano; Bonini, Nicola
  • Journal of Physics: Condensed Matter, Vol. 21, Issue 39, Article No. 395502
  • DOI: 10.1088/0953-8984/21/39/395502

Enhanced thermoelectric performance of rough silicon nanowires
journal, January 2008

  • Hochbaum, Allon I.; Chen, Renkun; Delgado, Raul Diaz
  • Nature, Vol. 451, Issue 7175, p. 163-167
  • DOI: 10.1038/nature06381

Thin-film thermoelectric devices with high room-temperature figures of merit
journal, October 2001

  • Venkatasubramanian, Rama; Siivola, Edward; Colpitts, Thomas
  • Nature, Vol. 413, Issue 6856, p. 597-602
  • DOI: 10.1038/35098012

Quantitative measurement of displacement and strain fields from HREM micrographs
journal, August 1998


High-Thermoelectric Performance of Nanostructured Bismuth Antimony Telluride Bulk Alloys
journal, May 2008