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Title: A single-column particle-resolved model for simulating the vertical distribution of aerosol mixing state: WRF-PartMC-MOSAIC-SCM v1.0

Abstract

The PartMC-MOSAIC particle-resolved aerosol model was previously developed to predict the aerosol mixing state as it evolves in the atmosphere. However, the modeling framework was limited to a zero-dimensional box model approach without resolving spatial gradients in aerosol concentrations. This paper presents the development of stochastic particle methods to simulate turbulent diffusion and dry deposition of aerosol particles in a vertical column within the planetary boundary layer. The new model, WRF-PartMC-MOSAIC-SCM, resolves the vertical distribution of aerosol mixing state. We verified the new algorithms with analytical solutions for idealized test cases and illustrate the capabilities with results from a 2-day urban scenario that shows the evolution of black carbon mixing state in a vertical column.

Authors:
 [1]; ORCiD logo [1]; ORCiD logo [1]
  1. Univ. of Illinois at Urbana-Champaign, Champaign, IL (United States)
Publication Date:
Research Org.:
Univ. of Illinois at Urbana-Champaign, Champaign, IL (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Biological and Environmental Research (BER) (SC-23)
OSTI Identifier:
1511023
Grant/Contract Number:  
[SC0003921; SC0011771]
Resource Type:
Accepted Manuscript
Journal Name:
Geoscientific Model Development (Online)
Additional Journal Information:
[Journal Name: Geoscientific Model Development (Online); Journal Volume: 10; Journal Issue: 11]; Journal ID: ISSN 1991-9603
Publisher:
European Geosciences Union
Country of Publication:
United States
Language:
English
Subject:
54 ENVIRONMENTAL SCIENCES

Citation Formats

Curtis, Jeffrey H., Riemer, Nicole, and West, Matthew. A single-column particle-resolved model for simulating the vertical distribution of aerosol mixing state: WRF-PartMC-MOSAIC-SCM v1.0. United States: N. p., 2017. Web. doi:10.5194/gmd-10-4057-2017.
Curtis, Jeffrey H., Riemer, Nicole, & West, Matthew. A single-column particle-resolved model for simulating the vertical distribution of aerosol mixing state: WRF-PartMC-MOSAIC-SCM v1.0. United States. doi:10.5194/gmd-10-4057-2017.
Curtis, Jeffrey H., Riemer, Nicole, and West, Matthew. Thu . "A single-column particle-resolved model for simulating the vertical distribution of aerosol mixing state: WRF-PartMC-MOSAIC-SCM v1.0". United States. doi:10.5194/gmd-10-4057-2017. https://www.osti.gov/servlets/purl/1511023.
@article{osti_1511023,
title = {A single-column particle-resolved model for simulating the vertical distribution of aerosol mixing state: WRF-PartMC-MOSAIC-SCM v1.0},
author = {Curtis, Jeffrey H. and Riemer, Nicole and West, Matthew},
abstractNote = {The PartMC-MOSAIC particle-resolved aerosol model was previously developed to predict the aerosol mixing state as it evolves in the atmosphere. However, the modeling framework was limited to a zero-dimensional box model approach without resolving spatial gradients in aerosol concentrations. This paper presents the development of stochastic particle methods to simulate turbulent diffusion and dry deposition of aerosol particles in a vertical column within the planetary boundary layer. The new model, WRF-PartMC-MOSAIC-SCM, resolves the vertical distribution of aerosol mixing state. We verified the new algorithms with analytical solutions for idealized test cases and illustrate the capabilities with results from a 2-day urban scenario that shows the evolution of black carbon mixing state in a vertical column.},
doi = {10.5194/gmd-10-4057-2017},
journal = {Geoscientific Model Development (Online)},
number = [11],
volume = [10],
place = {United States},
year = {2017},
month = {11}
}

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Cited by: 5 works
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Works referenced in this record:

Weighted Flow Algorithms (WFA) for stochastic particle coagulation
journal, September 2011

  • DeVille, R. E. L.; Riemer, N.; West, M.
  • Journal of Computational Physics, Vol. 230, Issue 23
  • DOI: 10.1016/j.jcp.2011.07.027

Modeling the evolution of aerosol particles in a ship plume using PartMC-MOSAIC
journal, January 2014


Suppression of Rain and Snow by Urban and Industrial Air Pollution
journal, March 2000


Development of a source oriented version of the WRF/Chem model and its application to the California regional PM 10 / PM 2.5 air quality study
journal, January 2014

  • Zhang, H.; DeNero, S. P.; Joe, D. K.
  • Atmospheric Chemistry and Physics, Vol. 14, Issue 1
  • DOI: 10.5194/acp-14-485-2014

Multi-spectral calculations of the direct radiative forcing of tropospheric sulphate and soot aerosols using a column model
journal, October 1997

  • Haywood, J. M.; Shine, K. P.
  • Quarterly Journal of the Royal Meteorological Society, Vol. 123, Issue 543
  • DOI: 10.1002/qj.49712354307

The effect of physical and chemical aerosol properties on warm cloud droplet activation
journal, January 2006

  • McFiggans, G.; Artaxo, P.; Baltensperger, U.
  • Atmospheric Chemistry and Physics, Vol. 6, Issue 9
  • DOI: 10.5194/acp-6-2593-2006

A size-composition resolved aerosol model for simulating the dynamics of externally mixed particles: SCRAM (v 1.0)
journal, January 2015

  • Zhu, S.; Sartelet, K. N.; Seigneur, C.
  • Geoscientific Model Development, Vol. 8, Issue 6
  • DOI: 10.5194/gmd-8-1595-2015

The effects of aging processes on critical supersaturation ratios of ultrafine carbon aerosols
journal, August 1999


Fully coupled “online” chemistry within the WRF model
journal, December 2005


Beyond single particle mass spectrometry: multidimensional characterisation of individual aerosol particles
journal, April 2009


Quantifying aerosol mixing state with entropy and diversity measures
journal, January 2013


Climate Modification by Atmospheric Aerosols
journal, June 1967


Climate: The Influence of Aerosols
journal, December 1969


Vertical dependence of black carbon, sulphate and biomass burning aerosol radiative forcing: VERTICAL DEPENDENCE OF AEROSOL FORCING
journal, December 2011

  • Samset, Bjørn H.; Myhre, Gunnar
  • Geophysical Research Letters, Vol. 38, Issue 24
  • DOI: 10.1029/2011GL049697

Aerosols, Cloud Microphysics, and Fractional Cloudiness
journal, September 1989


Simulating the evolution of soot mixing state with a particle‐resolved aerosol model
journal, January 2009

  • Riemer, N.; West, M.; Zaveri, R. A.
  • Journal of Geophysical Research, Vol. 114, Issue D9
  • DOI: 10.1029/2008JD011073

Simulation of particle diversity and mixing state over Greater Paris: a model–measurement inter-comparison
journal, January 2016

  • Zhu, Shupeng; Sartelet, Karine N.; Healy, Robert M.
  • Faraday Discussions, Vol. 189
  • DOI: 10.1039/C5FD00175G

In-situ measurements of the mixing state and optical properties of soot with implications for radiative forcing estimates
journal, July 2009

  • Moffet, R. C.; Prather, K. A.
  • Proceedings of the National Academy of Sciences, Vol. 106, Issue 29
  • DOI: 10.1073/pnas.0900040106

Modeling aerosols on the mesoscale-γ: Treatment of soot aerosol and its radiative effects
journal, January 2003


A Combined Local and Nonlocal Closure Model for the Atmospheric Boundary Layer. Part I: Model Description and Testing
journal, September 2007

  • Pleim, Jonathan E.
  • Journal of Applied Meteorology and Climatology, Vol. 46, Issue 9
  • DOI: 10.1175/JAM2539.1

Binning for Efficient Stochastic Multiscale Particle Simulations
journal, January 2013

  • Michelotti, M. D.; Heath, M. T.; West, M.
  • Multiscale Modeling & Simulation, Vol. 11, Issue 4
  • DOI: 10.1137/130908038

Radiative forcing by aerosols as derived from the AeroCom present-day and pre-industrial simulations
journal, January 2006

  • Schulz, M.; Textor, C.; Kinne, S.
  • Atmospheric Chemistry and Physics, Vol. 6, Issue 12
  • DOI: 10.5194/acp-6-5225-2006

Development of an aerosol microphysical module: Aerosol Two-dimensional bin module for foRmation and Aging Simulation (ATRAS)
journal, January 2014


Direct simulation Monte Carlo for simultaneous nucleation, coagulation, and surface growth in dispersed systems
journal, June 2004

  • Maisels, Arkadi; Einar Kruis, F.; Fissan, Heinz
  • Chemical Engineering Science, Vol. 59, Issue 11
  • DOI: 10.1016/j.ces.2004.02.015

Development of an Improved Turbulence Closure Model for the Atmospheric Boundary Layer
journal, January 2009

  • Nakanishi, Mikio; Niino, Hiroshi
  • Journal of the Meteorological Society of Japan, Vol. 87, Issue 5
  • DOI: 10.2151/jmsj.87.895

The parameterization of the vertical dispersion of a scalar in the atmospheric boundary layer
journal, September 1993


Aircraft measurements of vertical profiles of aerosol mixing states
journal, January 2010

  • Pratt, Kerri A.; Prather, Kimberly A.
  • Journal of Geophysical Research, Vol. 115, Issue D11
  • DOI: 10.1029/2009JD013150

Modeling the formation of secondary organic aerosol within a comprehensive air quality model system
journal, November 2001

  • Schell, Benedikt; Ackermann, Ingmar J.; Hass, Heinz
  • Journal of Geophysical Research: Atmospheres, Vol. 106, Issue D22
  • DOI: 10.1029/2001JD000384

Development and validation of a black carbon mixing state resolved three-dimensional model: Aging processes and radiative impact: BC MIXING STATE RESOLVED WRF-CHEM
journal, March 2013

  • Matsui, H.; Koike, M.; Kondo, Y.
  • Journal of Geophysical Research: Atmospheres, Vol. 118, Issue 5
  • DOI: 10.1029/2012JD018446

The MESSy aerosol submodel MADE3 (v2.0b): description and a box model test
journal, January 2014

  • Kaiser, J. C.; Hendricks, J.; Righi, M.
  • Geoscientific Model Development, Vol. 7, Issue 3
  • DOI: 10.5194/gmd-7-1137-2014

Black carbon aerosol mixing state, organic aerosols and aerosol optical properties over the United Kingdom
journal, January 2011

  • McMeeking, G. R.; Morgan, W. T.; Flynn, M.
  • Atmospheric Chemistry and Physics, Vol. 11, Issue 17
  • DOI: 10.5194/acp-11-9037-2011

How much can the vertical distribution of black carbon affect its global direct radiative forcing?: HOW MUCH DO BC PROFILES AFFECT FORCING?
journal, October 2010

  • Zarzycki, Colin M.; Bond, Tami C.
  • Geophysical Research Letters, Vol. 37, Issue 20
  • DOI: 10.1029/2010GL044555

The Influence of Pollution on the Shortwave Albedo of Clouds
journal, July 1977


Aerosol dynamics using the quadrature method of moments: comparing several quadrature schemes with particle-resolved simulation
journal, July 2008


A new method for multicomponent activity coefficients of electrolytes in aqueous atmospheric aerosols
journal, January 2005


Climate Forcing by Anthropogenic Aerosols
journal, January 1992


Dependence of climate forcing and response on the altitude of black carbon aerosols
journal, April 2011


Soot and sulfate aerosol particles in the remote marine troposphere
journal, September 1999

  • Pósfai, Mihály; Anderson, James R.; Buseck, Peter R.
  • Journal of Geophysical Research: Atmospheres, Vol. 104, Issue D17
  • DOI: 10.1029/1999JD900208

A computationally efficient Multicomponent Equilibrium Solver for Aerosols (MESA)
journal, January 2005

  • Zaveri, Rahul A.; Easter, Richard C.; Peters, Leonard K.
  • Journal of Geophysical Research, Vol. 110, Issue D24
  • DOI: 10.1029/2004JD005618

Model for Simulating Aerosol Interactions and Chemistry (MOSAIC)
journal, January 2008

  • Zaveri, Rahul A.; Easter, Richard C.; Fast, Jerome D.
  • Journal of Geophysical Research, Vol. 113, Issue D13
  • DOI: 10.1029/2007JD008782

A new lumped structure photochemical mechanism for large-scale applications
journal, December 1999

  • Zaveri, Rahul A.; Peters, Leonard K.
  • Journal of Geophysical Research: Atmospheres, Vol. 104, Issue D23
  • DOI: 10.1029/1999JD900876

Three-dimensional modeling of the mixing state of particles over Greater Paris: 3-D MIXING STATE MODELING
journal, May 2016

  • Zhu, Shupeng; Sartelet, Karine; Zhang, Yang
  • Journal of Geophysical Research: Atmospheres, Vol. 121, Issue 10
  • DOI: 10.1002/2015JD024241

Aging of black carbon in outflow from anthropogenic sources using a mixing state resolved model: Model development and evaluation
journal, January 2009

  • Oshima, N.; Koike, M.; Zhang, Y.
  • Journal of Geophysical Research, Vol. 114, Issue D6
  • DOI: 10.1029/2008JD010680

Particle-resolved simulation of aerosol size, composition, mixing state, and the associated optical and cloud condensation nuclei activation properties in an evolving urban plume
journal, January 2010

  • Zaveri, Rahul A.; Barnard, James C.; Easter, Richard C.
  • Journal of Geophysical Research, Vol. 115, Issue D17
  • DOI: 10.1029/2009JD013616

Parameterization of surface resistances to gaseous dry deposition in regional-scale numerical models
journal, January 1989


Hybrid Monte Carlo Method for Simulation of Two-Component Aerosol Coagulation and Phase Segregation
journal, May 2002

  • Efendiev, Y.; Zachariah, M. R.
  • Journal of Colloid and Interface Science, Vol. 249, Issue 1
  • DOI: 10.1006/jcis.2001.8114

Black carbon absorption at the global scale is affected by particle-scale diversity in composition
journal, September 2016

  • Fierce, Laura; Bond, Tami C.; Bauer, Susanne E.
  • Nature Communications, Vol. 7, Issue 1
  • DOI: 10.1038/ncomms12361

A size-segregated particle dry deposition scheme for an atmospheric aerosol module
journal, January 2001


An Improved Mellor–Yamada Level-3 Model: Its Numerical Stability and Application to a Regional Prediction of Advection Fog
journal, March 2006


An Exact Method for Numerically Simulating the Stochastic Coalescence Process in a Cloud
journal, October 1975


Formation of photochemical air pollution in central California 1. Development of a revised motor vehicle emission inventory: PHOTOCHEMICAL AIR POLLUTION FORMATION, 1
journal, March 2002

  • Marr, Linsey C.; Black, Douglas R.; Harley, Robert A.
  • Journal of Geophysical Research: Atmospheres, Vol. 107, Issue D6
  • DOI: 10.1029/2001JD000689

In Situ Characterization of Cloud Condensation Nuclei, Interstitial, and Background Particles Using the Single Particle Mass Spectrometer, SPLAT II
journal, October 2010

  • Zelenyuk, Alla; Imre, Dan; Earle, Michael
  • Analytical Chemistry, Vol. 82, Issue 19
  • DOI: 10.1021/ac1013892

A three-dimensional sectional representation of aerosol mixing state for simulating optical properties and cloud condensation nuclei: Aerosol Mixing State Representation
journal, May 2016

  • Ching, Joseph; Zaveri, Rahul A.; Easter, Richard C.
  • Journal of Geophysical Research: Atmospheres, Vol. 121, Issue 10
  • DOI: 10.1002/2015JD024323

Multi-spectral calculations of the direct radiative forcing of tropospheric sulphate and soot aerosols using a column model
journal, October 1997

  • Haywood, Jm; Shine, Kp
  • Quarterly Journal of the Royal Meteorological Society, Vol. 123, Issue 543
  • DOI: 10.1256/smsqj.54306

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    • DOI: 10.1038/s41612-019-0081-9