Momentum-Resolved Surface Enhanced Raman Scattering from a Nanowire-Nanoparticle Junction Cavity
Abstract
Herein experimental evidence of directional surface enhanced Raman scattering from molecules situated inside a single nanowire–nanoparticle junction cavity is reported. The emission is confined to a narrow range of wavevectors perpendicular to the axis of the cavity. In addition to this, the molecules excite multiple guided modes of the nanowire which are imaged using leakage radiation Fourier microscopy. The emission wavevectors are further characterized as a function of output polarization. The excited guided modes of the wire show interesting polarization signatures. All the results are corroborated using finite element method based numerical simulations. Essentially, an important connection between gap-cavity enhanced Raman scattering and its directionality of emission is provided. The results may be relevant in understanding the cavity electrodynamics at the nanoscale and molecular coupling to extremely small gaps between a 1D and a 0D plasmonic nanostructure.
- Authors:
-
[1];
[1];
[2];
[3]
- Indian Inst. of Science Education and Research, Pune, IN (United States). Dept. of Physics
- Argonne National Lab. (ANL), Argonne, IL (United States). Center for Nanoscale Materials
- Indian Inst. of Science Education and Research, Pune, IN (United States). Dept. of Physics; Indian Inst. of Science Education and Research, Pune, IN (United States). Center for Energy Science
- Publication Date:
- Research Org.:
- Argonne National Laboratory (ANL), Argonne, IL (United States)
- Sponsoring Org.:
- Air Force Research Laboratory (AFRL); USDOE Office of Science (SC), Basic Energy Sciences (BES). Scientific User Facilities Division
- OSTI Identifier:
- 1562277
- Alternate Identifier(s):
- OSTI ID: 1510841
- Grant/Contract Number:
- AC02-06CH11357; AC02‐06CH11357
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Advanced Optical Materials
- Additional Journal Information:
- Journal Volume: 7; Journal Issue: 15; Journal ID: ISSN 2195-1071
- Publisher:
- Wiley
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; surface enhanced Raman scattering; Fourier plane imaging; directional emission; nanocavities
Citation Formats
Vasista, Adarsh B., Chaubey, Shailendra K., Gosztola, David J., Wiederrecht, Gary P., Gray, Stephen K., and Kumar, G. V. Pavan. Momentum-Resolved Surface Enhanced Raman Scattering from a Nanowire-Nanoparticle Junction Cavity. United States: N. p., 2019.
Web. doi:10.1002/adom.201900304.
Vasista, Adarsh B., Chaubey, Shailendra K., Gosztola, David J., Wiederrecht, Gary P., Gray, Stephen K., & Kumar, G. V. Pavan. Momentum-Resolved Surface Enhanced Raman Scattering from a Nanowire-Nanoparticle Junction Cavity. United States. https://doi.org/10.1002/adom.201900304
Vasista, Adarsh B., Chaubey, Shailendra K., Gosztola, David J., Wiederrecht, Gary P., Gray, Stephen K., and Kumar, G. V. Pavan. Mon .
"Momentum-Resolved Surface Enhanced Raman Scattering from a Nanowire-Nanoparticle Junction Cavity". United States. https://doi.org/10.1002/adom.201900304. https://www.osti.gov/servlets/purl/1562277.
@article{osti_1562277,
title = {Momentum-Resolved Surface Enhanced Raman Scattering from a Nanowire-Nanoparticle Junction Cavity},
author = {Vasista, Adarsh B. and Chaubey, Shailendra K. and Gosztola, David J. and Wiederrecht, Gary P. and Gray, Stephen K. and Kumar, G. V. Pavan},
abstractNote = {Herein experimental evidence of directional surface enhanced Raman scattering from molecules situated inside a single nanowire–nanoparticle junction cavity is reported. The emission is confined to a narrow range of wavevectors perpendicular to the axis of the cavity. In addition to this, the molecules excite multiple guided modes of the nanowire which are imaged using leakage radiation Fourier microscopy. The emission wavevectors are further characterized as a function of output polarization. The excited guided modes of the wire show interesting polarization signatures. All the results are corroborated using finite element method based numerical simulations. Essentially, an important connection between gap-cavity enhanced Raman scattering and its directionality of emission is provided. The results may be relevant in understanding the cavity electrodynamics at the nanoscale and molecular coupling to extremely small gaps between a 1D and a 0D plasmonic nanostructure.},
doi = {10.1002/adom.201900304},
journal = {Advanced Optical Materials},
number = 15,
volume = 7,
place = {United States},
year = {Mon May 06 00:00:00 EDT 2019},
month = {Mon May 06 00:00:00 EDT 2019}
}
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Works referenced in this record:
Nanowire-supported plasmonic waveguide for remote excitation of surface-enhanced Raman scattering
journal, August 2014
- Huang, Yingzhou; Fang, Yurui; Zhang, Zhenglong
- Light: Science & Applications, Vol. 3, Issue 8
Tailored Emission Spectrum of 2D Semiconductors Using Plasmonic Nanocavities
journal, November 2017
- Huang, Jiani; Akselrod, Gleb M.; Ming, Tian
- ACS Photonics, Vol. 5, Issue 2
SERS Orientational Imaging of Silver Nanoparticle Dimers
journal, October 2011
- Stranahan, Sarah M.; Titus, Eric J.; Willets, Katherine A.
- The Journal of Physical Chemistry Letters, Vol. 2, Issue 21
Multiple-Particle Nanoantennas for Enormous Enhancement and Polarization Control of Light Emission
journal, February 2009
- Li, Zhipeng; Shegai, Timur; Haran, Gilad
- ACS Nano, Vol. 3, Issue 3
Identification and control of multiple leaky plasmon modes in silver nanowires: Identification and control of multiple leaky…
journal, December 2015
- Yang, Hangbo; Qiu, Min; Li, Qiang
- Laser & Photonics Reviews, Vol. 10, Issue 2
Metal-Substrate-Mediated Plasmon Hybridization in a Nanoparticle Dimer for Photoluminescence Line-Width Shrinking and Intensity Enhancement
journal, February 2017
- Li, Guang-Can; Zhang, Yong-Liang; Jiang, Jing
- ACS Nano, Vol. 11, Issue 3
Plasmonic Nanoparticle Dimers for Optical Sensing of DNA in Complex Media
journal, July 2010
- Chen, Jennifer I. L.; Chen, Yeechi; Ginger, David S.
- Journal of the American Chemical Society, Vol. 132, Issue 28
Remote-excitation surface-enhanced Raman scattering with counter-propagating plasmons: silver nanowire-nanoparticle system
journal, December 2013
- Dasgupta, Arindam; Singh, Danveer; Tandon, Shreyash
- Journal of Nanophotonics, Vol. 8, Issue 1
A capillary force-induced Au nanoparticle–Ag nanowire single hot spot platform for SERS analysis
journal, January 2017
- Li, Pan; Yan, Xiunan; Zhou, Fei
- Journal of Materials Chemistry C, Vol. 5, Issue 13
Polyol Synthesis of Uniform Silver Nanowires: A Plausible Growth Mechanism and the Supporting Evidence
journal, July 2003
- Sun, Yugang; Mayers, Brian; Herricks, Thurston
- Nano Letters, Vol. 3, Issue 7
Plasmofluidic single-molecule surface-enhanced Raman scattering from dynamic assembly of plasmonic nanoparticles
journal, July 2014
- Patra, Partha Pratim; Chikkaraddy, Rohit; Tripathi, Ravi P. N.
- Nature Communications, Vol. 5, Issue 1
Ideal Dimers of Gold Nanospheres for Precision Plasmonics: Synthesis and Characterization at the Single-Particle Level for Identification of Higher Order Modes
journal, November 2017
- Yoon, Jun Hee; Selbach, Florian; Langolf, Ludmilla
- Small, Vol. 14, Issue 4
Nanoparticle-Mediated Coupling of Light into a Nanowire
journal, August 2007
- Knight, Mark W.; Grady, Nathaniel K.; Bardhan, Rizia
- Nano Letters, Vol. 7, Issue 8
Near-to-Far Field Transformations for Radiative and Guided Waves
journal, February 2016
- Yang, Jianji; Hugonin, Jean-Paul; Lalanne, Philippe
- ACS Photonics, Vol. 3, Issue 3
Directional out-coupling of light from a plasmonic nanowire-nanoparticle junction
journal, January 2015
- Singh, Danveer; Dasgupta, Arindam; Aswathy, V. G.
- Optics Letters, Vol. 40, Issue 6
Imaging Symmetry-Selected Corner Plasmon Modes in Penta-Twinned Crystalline Ag Nanowires
journal, June 2011
- Song, Mingxia; Bouhelier, Alexandre; Bramant, Pierre
- ACS Nano, Vol. 5, Issue 7
Gap Plasmons and Near-Field Enhancement in Closely Packed Sub-10 nm Gap Resonators
journal, October 2013
- Siegfried, Thomas; Ekinci, Yasin; Martin, Olivier J. F.
- Nano Letters, Vol. 13, Issue 11
Atoms and molecules in cavities, from weak to strong coupling in quantum-electrodynamics (QED) chemistry
journal, March 2017
- Flick, Johannes; Ruggenthaler, Michael; Appel, Heiko
- Proceedings of the National Academy of Sciences, Vol. 114, Issue 12
Probing nanoscale interfaces with electrochemical surface-enhanced Raman scattering
journal, February 2019
- Willets, Katherine A.
- Current Opinion in Electrochemistry, Vol. 13
Polarization Dependence of Surface-Enhanced Raman Scattering in Gold Nanoparticle−Nanowire Systems
journal, August 2008
- Wei, Hong; Hao, Feng; Huang, Yingzhou
- Nano Letters, Vol. 8, Issue 8
Direction-resolved radiation from polarization-controlled surface plasmon modes on silver nanowire antennas
journal, January 2016
- Jia, Zhili; Wei, Hong; Pan, Deng
- Nanoscale, Vol. 8, Issue 48
The Remote Light Emission Modulated by Local Surface Plasmon Resonance for the CdSe NW-Au NP Hybrid Structure
journal, November 2018
- He, Jingru; Li, Jing; Xia, Jing
- Advanced Materials Interfaces, Vol. 6, Issue 2
Gap-plasmon nanoantennas and bowtie resonators
journal, January 2012
- Gramotnev, Dmitri K.; Pors, Anders; Willatzen, Morten
- Physical Review B, Vol. 85, Issue 4
Nanoparticle-Enhanced Silver-Nanowire Plasmonic Electrodes for High-Performance Organic Optoelectronic Devices
journal, May 2018
- Kim, Taehyo; Kang, Saewon; Heo, Jungwoo
- Advanced Materials, Vol. 30, Issue 28
Squeezing Visible Light Waves into a 3-nm-Thick and 55-nm-Long Plasmon Cavity
journal, March 2006
- Miyazaki, Hideki T.; Kurokawa, Yoichi
- Physical Review Letters, Vol. 96, Issue 9
Super-resolution Optical Imaging of Single-Molecule SERS Hot Spots
journal, September 2010
- Stranahan, Sarah M.; Willets, Katherine A.
- Nano Letters, Vol. 10, Issue 9
Large spontaneous emission enhancement in plasmonic nanocavities
journal, May 2012
- Russell, Kasey J.; Liu, Tsung-Li; Cui, Shanying
- Nature Photonics, Vol. 6, Issue 7
Coupling a Single Trapped Atom to a Nanoscale Optical Cavity
journal, April 2013
- Thompson, J. D.; Tiecke, T. G.; de Leon, N. P.
- Science, Vol. 340, Issue 6137
Direct Observation of Beamed Raman Scattering
journal, February 2012
- Zhu, Wenqi; Wang, Dongxing; Crozier, Kenneth B.
- Nano Letters, Vol. 12, Issue 12
Single-molecule strong coupling at room temperature in plasmonic nanocavities
journal, June 2016
- Chikkaraddy, Rohit; de Nijs, Bart; Benz, Felix
- Nature, Vol. 535, Issue 7610
Chemical mapping of a single molecule by plasmon-enhanced Raman scattering
journal, June 2013
- Zhang, R.; Zhang, Y.; Dong, Z. C.
- Nature, Vol. 498, Issue 7452
Efficient Nanosecond Photoluminescence from Infrared PbS Quantum Dots Coupled to Plasmonic Nanoantennas
journal, September 2016
- Akselrod, Gleb M.; Weidman, Mark C.; Li, Ying
- ACS Photonics, Vol. 3, Issue 10
Remotely excited Raman optical activity using chiral plasmon propagation in Ag nanowires
journal, November 2013
- Sun, Mengtao; Zhang, Zhenglong; Wang, Peijie
- Light: Science & Applications, Vol. 2, Issue 11
Chiral nanophotonic waveguide interface based on spin-orbit interaction of light
journal, September 2014
- Petersen, Jan; Volz, Jürgen; Rauschenbeutel, Arno
- Science, Vol. 346, Issue 6205
Optical Constants of the Noble Metals
journal, December 1972
- Johnson, P. B.; Christy, R. W.
- Physical Review B, Vol. 6, Issue 12, p. 4370-4379
Differential Wavevector Distribution of Surface-Enhanced Raman Scattering and Fluorescence in a Film-Coupled Plasmonic Nanowire Cavity
journal, December 2017
- Vasista, Adarsh B.; Jog, Harshvardhan; Heilpern, Tal
- Nano Letters, Vol. 18, Issue 1
Surface-enhanced Raman scattering and fluorescence near metal nanoparticles
journal, July 2005
- Johansson, Peter; Xu, Hongxing; Käll, Mikael
- Physical Review B, Vol. 72, Issue 3
Raman Radiation Patterns of Graphene
journal, December 2015
- Budde, Harald; Coca-López, Nicolás; Shi, Xian
- ACS Nano, Vol. 10, Issue 2
Cavity optomechanics
journal, December 2014
- Aspelmeyer, Markus; Kippenberg, Tobias J.; Marquardt, Florian
- Reviews of Modern Physics, Vol. 86, Issue 4
Directional out-coupling of light from a plasmonic nanowire-nanoparticle junction
text, January 2015
- Singh, Danveer; Dasgupta, Arindam; G., Aswathy V.
- arXiv
Plasmofluidic Single-Molecule Surface Enhanced Raman Scattering from Dynamic Assembly of Plasmonic Nanoparticles
text, January 2018
- Patra, Partha Pratim; Chikkaraddy, Rohit; Tripathi, Ravi P. N.
- arXiv
Surface-enhanced Raman scattering and fluorescence near metal nanoparticles
text, January 2005
- Johansson, Peter; Xu, Hongxing; Käll, Mikael
- arXiv
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- Cao, Tun; Liu, Kuan; Lu, Li
- Advanced Optical Materials, Vol. 8, Issue 6