Microstructures and properties of high-entropy alloy films and coatings: a review

Li, Wei; Liu, Ping; Liaw, Peter K.

doi:10.1080/21663831.2018.1434248

Title: Microstructures and properties of high-entropy alloy films and coatings: a review

Abstract

In the past 14 years, as a branch of high-entropy alloy (HEA) materials, HEA films and coatings have exhibited the attractive and unique properties, relative to the conventional film and coating materials. The recent research and development of HEA films and coatings are reviewed in this paper. At first, the basic concept of HEAs films and coatings are introduced. Then, their preparation technologies, microstructures and appealing properties are summarized. Moreover, the possible reasons and design criteria for achieving the excellent properties are discussed. Finally, the suggested future research work for the HEA films and coatings are outlined. Preparation technologies, microstructures, and properties of HEA films and coatings are reviewed in this paper. The design criteria and suggested research directions are further discussed and proposed.

Authors:

Li, Wei ^[1]; Liu, Ping ^[1]; Liaw, Peter K. ^[2]

Univ. of Shanghai for Science and Technology, Shanghai (China). School of Materials Science and Engineering
Univ. of Tennessee, Knoxville, TN (United States). Department of Materials Science and Engineering

Publication Date:: Tue Feb 20 00:00:00 EST 2018

Research Org.:: Univ. of Illinois at Urbana-Champaign, IL (United States); Univ. of Tennessee, Knoxville, TN (United States)

Sponsoring Org.:: USDOE Office of Fossil Energy (FE)

OSTI Identifier:: 1510475

Grant/Contract Number:: FE0011194; FE0024054

Resource Type:: Accepted Manuscript

Journal Name:: Materials Research Letters

Additional Journal Information:: Journal Volume: 6; Journal Issue: 4; Journal ID: ISSN 2166-3831

Publisher:: Taylor and Francis

Country of Publication:: United States

Language:: English

Subject:: 36 MATERIALS SCIENCE; High-entropy alloys; films and coatings; preparation technologies; microstructure; properties

Citation Formats


                    Li, Wei, Liu, Ping, and Liaw, Peter K. Microstructures and properties of high-entropy alloy films and coatings: a review.  United States: N. p., 2018. 
Web.  doi:10.1080/21663831.2018.1434248.

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                    Li, Wei, Liu, Ping, & Liaw, Peter K. Microstructures and properties of high-entropy alloy films and coatings: a review.  United States.  https://doi.org/10.1080/21663831.2018.1434248

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                    Li, Wei, Liu, Ping, and Liaw, Peter K. Tue .  
"Microstructures and properties of high-entropy alloy films and coatings: a review".  United States.  https://doi.org/10.1080/21663831.2018.1434248.  https://www.osti.gov/servlets/purl/1510475.

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@article{osti_1510475,

  title        = {Microstructures and properties of high-entropy alloy films and coatings: a review},

  author       = {Li, Wei and Liu, Ping and Liaw, Peter K.},

  abstractNote = {In the past 14 years, as a branch of high-entropy alloy (HEA) materials, HEA films and coatings have exhibited the attractive and unique properties, relative to the conventional film and coating materials. The recent research and development of HEA films and coatings are reviewed in this paper. At first, the basic concept of HEAs films and coatings are introduced. Then, their preparation technologies, microstructures and appealing properties are summarized. Moreover, the possible reasons and design criteria for achieving the excellent properties are discussed. Finally, the suggested future research work for the HEA films and coatings are outlined. Preparation technologies, microstructures, and properties of HEA films and coatings are reviewed in this paper. The design criteria and suggested research directions are further discussed and proposed.},

  doi          = {10.1080/21663831.2018.1434248},

  journal      = {Materials Research Letters},

  number       = 4,

  volume       = 6,

  place        = {United States},

  year         = {Tue Feb 20 00:00:00 EST 2018},

  month        = {Tue Feb 20 00:00:00 EST 2018}

}

Copy to clipboard

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Arabian Journal for Science and Engineering, Vol. 44, Issue 7
DOI: 10.1007/s13369-019-03875-x

Thin film metallic glasses: Properties, applications and future
journal, January 2020

Yiu, Pakman; Diyatmika, Wahyu; Bönninghoff, Niklas
Journal of Applied Physics, Vol. 127, Issue 3
DOI: 10.1063/1.5122884

Microstructure characterization of AlCoCrFeNiTi high-entropy alloy coating produced by atmospheric plasma spraying
journal, September 2019

Tian, Lihui; Wang, Jinchen; Zhang, Qian
Materials Research Express, Vol. 6, Issue 11
DOI: 10.1088/2053-1591/ab44f5

Effects of Al Addition on Microstructures and Mechanical Properties of CoCrFeMnNiAlx High Entropy Alloy Films
journal, December 2019

Hsu, Ya-Chu; Li, Chia-Lin; Hsueh, Chun-Hway
Entropy, Vol. 22, Issue 1
DOI: 10.3390/e22010002

Additive Manufacturing of High-Entropy Alloys: A Review
journal, December 2018

Chen, Shuying; Tong, Yang; Liaw, Peter
Entropy, Vol. 20, Issue 12
DOI: 10.3390/e20120937

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The Ni–Mo–P amorphous films were successfully deposited on the CoCrFeNi high-entropy alloys by electroless plating. This work will focus on reviewing and discussing the ambient-temperature mechanical properties, plastic deformation, and cracking mode of the coating-substrate system. The yielding strength (σ_y) and ultimate tensile strength (UTS) of the specimen plating for 1 h were 260 and 760 MPa, respectively, with 44.4% (σ_y) and 14.2% (UTS) improvement contrast to the uncoated HEAs (σ_y and UTS are 180 MPa and 560 MPa, respectively). It is attributed to the back stress and repulsive image stress to suppress the nucleation and mobility of dislocations. Duemore »« less
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Title: Microstructures and properties of high-entropy alloy films and coatings: a review

Abstract

Citation Formats

Microstructure and Wear Behavior of CoCrFeMnNbNi High-Entropy Alloy Coating by TIG Cladding journal, January 2015

Effect of nitrogen content and substrate bias on mechanical and corrosion properties of high-entropy films (AlCrSiTiZr)100−xNx journal, May 2012

Preparation and characterization of AlCrTaTiZr multi-element nitride coatings journal, December 2006

Effect of substrate bias on the structure and properties of multi-element (AlCrTaTiZr)N coatings journal, October 2006

In Vitro Biocompatibility of Si Alloyed Multi-Principal Element Carbide Coatings journal, August 2016

Structure and optoelectronic properties of multi-element oxide thin film journal, May 2011

Nanomechanical Properties and Deformation Behaviors of Multi-Component (AlCrTaTiZr)NxSiy High-Entropy Coatings journal, December 2013

Laser assisted high entropy alloy coating on aluminum: Microstructural evolution journal, September 2014

Nanostructured multi-element (TiZrNbHfTa)N and (TiZrNbHfTa)C hard coatings journal, October 2012

Microstructural development in equiatomic multicomponent alloys journal, July 2004

Controllable electrochemical synthesis and magnetic behaviors of Mg–Mn–Fe–Co–Ni–Gd alloy films journal, June 2014

The influence of Ge and In addition on the phase formation of CoCrCuFeNi high-entropy alloy thin films journal, October 2016

Nucleation barrier for phase transformations in nanosized crystals journal, May 2002

Sluggish diffusion in Co–Cr–Fe–Mn–Ni high-entropy alloys journal, August 2013

Dry sliding wear behavior of laser clad TiVCrAlSi high entropy alloy coatings on Ti–6Al–4V substrate journal, October 2012

Corrosion of Al CoCrFeNi high-entropy alloys: Al-content and potential scan-rate dependent pitting behavior journal, May 2017

Evolution of enhanced crystallinity and mechanical property of nanocomposite Ti–Si–N thin films using magnetron reactive co-sputtering journal, October 2012

Improved Diffusion-Resistant Ability of Multicomponent Nitrides: From Unitary TiN to Senary High-Entropy (TiTaCrZrAlRu)N journal, July 2013

Effect of seawater level on corrosion behavior of different alloys journal, August 2008

Evolution of microstructure and mechanical properties of in situ synthesized TiC–TiB2/CoCrCuFeNi high entropy alloy coatings journal, November 2015

AlCoCrCuFeNi high entropy alloy cluster growth and annealing on silicon: A classical molecular dynamics simulation study journal, November 2013

Design of Light-Weight High-Entropy Alloys journal, September 2016

Ru incorporation on marked enhancement of diffusion resistance of multi-component alloy barrier layers journal, February 2011

Effect of Nb addition on the structure and mechanical behaviors of CoCrCuFeNi high-entropy alloy coatings journal, February 2014

Multi-Principal-Element Alloys with Improved Oxidation and Wear Resistance for Thermal Spray Coating journal, February 2004

Size and pressure effects on solid transition temperatures of ZrO2 journal, June 2006

The microstructure and strengthening mechanism of thermal spray coating NixCo0.6Fe0.2CrySizAlTi0.2 high-entropy alloys journal, April 2011

High-Entropy Alloys: A Critical Review journal, April 2014

Phase stability in high entropy alloys: Formation of solid-solution phase or amorphous phase journal, December 2011

A study of the corrosion behavior of gamma titanium aluminide in 3.5wt% NaCl solution and seawater journal, September 2007

Microstructure characterization of Al x CoCrCuFeNi high-entropy alloy system with multiprincipal elements journal, April 2005

Solid solution or amorphous phase formation in TiZr-based ternary to quinternary multi-principal-element films journal, August 2014

Thermal Stability of Superhard Nitride Coatings from High-Entropy Multicomponent Ti–V–Zr–Nb–Hf Alloy journal, January 2014

Electrical, magnetic, and Hall properties of AlxCoCrFeNi high-entropy alloys journal, February 2011

Phase stability of non-equiatomic CoCrFeMnNi high entropy alloys journal, October 2015

Mechanical performance of the Al x CoCrCuFeNi high-entropy alloy system with multiprincipal elements journal, May 2005

Characterization of multi-principal-element (TiZrNbHfTa)N and (TiZrNbHfTa)C coatings for biomedical applications journal, June 2012

Effects of Different Levels of Boron on Microstructure and Hardness of CoCrFeNiAlxCu0.7Si0.1By High-Entropy Alloy Coatings by Laser Cladding journal, January 2017

Microstructure and oxidation behavior of new refractory high entropy alloys journal, January 2014

Molecular dynamics simulation of Al–Co–Cr–Cu–Fe–Ni high entropy alloy thin film growth journal, January 2016

Facile preparation and magnetic study of amorphous Tm-Fe-Co-Ni-Mn multicomponent alloy nanofilm journal, February 2011

Effect of valence electron concentration on stability of fcc or bcc phase in high entropy alloys journal, May 2011

Effects of silicon content on the structure and properties of (AlCrMoTaTi)N coatings by reactive magnetron sputtering journal, December 2014

Phase transformations and phase stability in nanocrystalline materials journal, December 2005

Guidelines in predicting phase formation of high-entropy alloys journal, April 2014

Synthesis and characterization of refractory TiZrNbWMo high-entropy alloy coating by laser cladding journal, February 2017

Thermal stability and oxidation resistance of laser clad TiVCrAlSi high entropy alloy coatings on Ti–6Al–4V alloy journal, December 2011

Tailoring magnetic behavior of CoFeMnNiX (X = Al, Cr, Ga, and Sn) high entropy alloys by metal doping journal, May 2017

Kinetic equation of the effect of thickness on grain growth in nanocrystalline films journal, December 2009

Effect of Heat Treatment on Borides Precipitation and Mechanical Properties of CoCrFeNiAl1.8Cu0.7B0.3Si0.1 High-Entropy Alloy Prepared by Arc-Melting and Laser-Cladding journal, May 2017

Superior Oxidation Resistance of (Al 0.34 Cr 0.22 Nb 0.11 Si 0.11 Ti 0.22 ) 50 N 50 High-Entropy Nitride journal, January 2013

Microstructure Characterization of Laser Clad TiVCrAlSi High Entropy Alloy Coating on Ti-6Al-4V Substrate journal, October 2010

Towards hard yet self-lubricious CrAlSiN coatings journal, January 2015

Characteristics of TiVCrAlZr multi-element nitride films prepared by reactive sputtering journal, August 2010

Laser additive synthesis of high entropy alloy coating on aluminum: Corrosion behavior journal, March 2015

Electrochemical deposition and microstructural characterization of AlCrFeMnNi and AlCrCuFeMnNi high entropy alloy thin films journal, December 2015

More than entropy in high-entropy alloys: Forming solid solutions or amorphous phase journal, October 2013

Molecular dynamics simulations of clusters and thin film growth in the context of plasma sputtering deposition journal, May 2014

Synthesis and characterization of multi-element oxynitride semiconductor film prepared by reactive sputtering deposition journal, December 2012

PVD hard coatings applied for the wear protection of drawing dies journal, October 2005

Characteristics of (TiAlCrNbY)C films deposited by reactive magnetron sputtering journal, March 2010

Investigation of the nanostructure and wear properties of physical vapor deposited CrCuN nanocomposite coatings journal, May 2005

(AlCrTaTiZr)N/(AlCrTaTiZr)N0.7 bilayer structure of high resistance to the interdiffusion of Cu and Si at 900°C journal, January 2011

Formation of core–shell structure in high entropy alloy coating by laser cladding journal, February 2016

Size Dependence of a First Order Solid-Solid Phase Transition: The Wurtzite to Rock Salt Transformation in CdSe Nanocrystals journal, July 1994

Nanostructured High-Entropy Alloys with Multiple Principal Elements: Novel Alloy Design Concepts and Outcomes journal, May 2004

Understanding phase stability of Al-Co-Cr-Fe-Ni high entropy alloys journal, November 2016

Solid-Solution CrCoCuFeNi High-Entropy Alloy Thin Films Synthesized by Sputter Deposition journal, June 2015

Effect of bias voltage on TiAlSiN nanocomposite coatings deposited by HiPIMS journal, January 2017

Surface Energies and Thermodynamic Phase Stability in Nanocrystalline Aluminas journal, August 1997

High-entropy alloys: a critical assessment of their founding principles and future prospects journal, April 2016

Solid-Solution Phase Formation Rules for Multi-component Alloys journal, June 2008

Effects of silicon content on the structure and mechanical properties of (AlCrTaTiZr)–Si x –N coatings by reactive RF magnetron sputtering journal, May 2011

On the significance of the H/E ratio in wear control: a nanocomposite coating approach to optimised tribological behaviour journal, November 2000

Dense and smooth amorphous films of multicomponent FeCoNiCuVZrAl high-entropy alloy deposited by direct current magnetron sputtering journal, April 2013

Structure and properties of two Al–Cr–Nb–Si–Ti high-entropy nitride coatings journal, April 2013

Prediction of A2 to B2 Phase Transition in the High-Entropy Alloy Mo-Nb-Ta-W journal, October 2013

Microstructure and Wear Behavior of CoCrFeMnNbNi High-Entropy Alloy Coating by TIG Cladding
journal, January 2015

Effect of nitrogen content and substrate bias on mechanical and corrosion properties of high-entropy films (AlCrSiTiZr)100−xNx
journal, May 2012

Preparation and characterization of AlCrTaTiZr multi-element nitride coatings
journal, December 2006

Effect of substrate bias on the structure and properties of multi-element (AlCrTaTiZr)N coatings
journal, October 2006

In Vitro Biocompatibility of Si Alloyed Multi-Principal Element Carbide Coatings
journal, August 2016

Structure and optoelectronic properties of multi-element oxide thin film
journal, May 2011

Nanomechanical Properties and Deformation Behaviors of Multi-Component (AlCrTaTiZr)NxSiy High-Entropy Coatings
journal, December 2013

Laser assisted high entropy alloy coating on aluminum: Microstructural evolution
journal, September 2014

Nanostructured multi-element (TiZrNbHfTa)N and (TiZrNbHfTa)C hard coatings
journal, October 2012

Microstructural development in equiatomic multicomponent alloys
journal, July 2004

Controllable electrochemical synthesis and magnetic behaviors of Mg–Mn–Fe–Co–Ni–Gd alloy films
journal, June 2014

The influence of Ge and In addition on the phase formation of CoCrCuFeNi high-entropy alloy thin films
journal, October 2016

Nucleation barrier for phase transformations in nanosized crystals
journal, May 2002

Sluggish diffusion in Co–Cr–Fe–Mn–Ni high-entropy alloys
journal, August 2013

Dry sliding wear behavior of laser clad TiVCrAlSi high entropy alloy coatings on Ti–6Al–4V substrate
journal, October 2012

Corrosion of Al CoCrFeNi high-entropy alloys: Al-content and potential scan-rate dependent pitting behavior
journal, May 2017

Evolution of enhanced crystallinity and mechanical property of nanocomposite Ti–Si–N thin films using magnetron reactive co-sputtering
journal, October 2012

Improved Diffusion-Resistant Ability of Multicomponent Nitrides: From Unitary TiN to Senary High-Entropy (TiTaCrZrAlRu)N
journal, July 2013

Effect of seawater level on corrosion behavior of different alloys
journal, August 2008

Evolution of microstructure and mechanical properties of in situ synthesized TiC–TiB2/CoCrCuFeNi high entropy alloy coatings
journal, November 2015

AlCoCrCuFeNi high entropy alloy cluster growth and annealing on silicon: A classical molecular dynamics simulation study
journal, November 2013

Design of Light-Weight High-Entropy Alloys
journal, September 2016

Ru incorporation on marked enhancement of diffusion resistance of multi-component alloy barrier layers
journal, February 2011

Effect of Nb addition on the structure and mechanical behaviors of CoCrCuFeNi high-entropy alloy coatings
journal, February 2014

Multi-Principal-Element Alloys with Improved Oxidation and Wear Resistance for Thermal Spray Coating
journal, February 2004

Size and pressure effects on solid transition temperatures of ZrO2
journal, June 2006

The microstructure and strengthening mechanism of thermal spray coating NixCo0.6Fe0.2CrySizAlTi0.2 high-entropy alloys
journal, April 2011

High-Entropy Alloys: A Critical Review
journal, April 2014

Phase stability in high entropy alloys: Formation of solid-solution phase or amorphous phase
journal, December 2011

A study of the corrosion behavior of gamma titanium aluminide in 3.5wt% NaCl solution and seawater
journal, September 2007

Microstructure characterization of Al x CoCrCuFeNi high-entropy alloy system with multiprincipal elements
journal, April 2005

Solid solution or amorphous phase formation in TiZr-based ternary to quinternary multi-principal-element films
journal, August 2014

Thermal Stability of Superhard Nitride Coatings from High-Entropy Multicomponent Ti–V–Zr–Nb–Hf Alloy
journal, January 2014

Electrical, magnetic, and Hall properties of AlxCoCrFeNi high-entropy alloys
journal, February 2011

Phase stability of non-equiatomic CoCrFeMnNi high entropy alloys
journal, October 2015

Mechanical performance of the Al x CoCrCuFeNi high-entropy alloy system with multiprincipal elements
journal, May 2005

Characterization of multi-principal-element (TiZrNbHfTa)N and (TiZrNbHfTa)C coatings for biomedical applications
journal, June 2012

Effects of Different Levels of Boron on Microstructure and Hardness of CoCrFeNiAlxCu0.7Si0.1By High-Entropy Alloy Coatings by Laser Cladding
journal, January 2017

Microstructure and oxidation behavior of new refractory high entropy alloys
journal, January 2014

Molecular dynamics simulation of Al–Co–Cr–Cu–Fe–Ni high entropy alloy thin film growth
journal, January 2016

Facile preparation and magnetic study of amorphous Tm-Fe-Co-Ni-Mn multicomponent alloy nanofilm
journal, February 2011

Effect of valence electron concentration on stability of fcc or bcc phase in high entropy alloys
journal, May 2011

Effects of silicon content on the structure and properties of (AlCrMoTaTi)N coatings by reactive magnetron sputtering
journal, December 2014

Phase transformations and phase stability in nanocrystalline materials
journal, December 2005

Guidelines in predicting phase formation of high-entropy alloys
journal, April 2014

Synthesis and characterization of refractory TiZrNbWMo high-entropy alloy coating by laser cladding
journal, February 2017

Thermal stability and oxidation resistance of laser clad TiVCrAlSi high entropy alloy coatings on Ti–6Al–4V alloy
journal, December 2011

Tailoring magnetic behavior of CoFeMnNiX (X = Al, Cr, Ga, and Sn) high entropy alloys by metal doping
journal, May 2017

Kinetic equation of the effect of thickness on grain growth in nanocrystalline films
journal, December 2009

Effect of Heat Treatment on Borides Precipitation and Mechanical Properties of CoCrFeNiAl1.8Cu0.7B0.3Si0.1 High-Entropy Alloy Prepared by Arc-Melting and Laser-Cladding
journal, May 2017

Superior Oxidation Resistance of (Al _0.34 Cr _0.22 Nb _0.11 Si _0.11 Ti _0.22 ) ₅₀ N ₅₀ High-Entropy Nitride
journal, January 2013

Microstructure Characterization of Laser Clad TiVCrAlSi High Entropy Alloy Coating on Ti-6Al-4V Substrate
journal, October 2010

Towards hard yet self-lubricious CrAlSiN coatings
journal, January 2015

Characteristics of TiVCrAlZr multi-element nitride films prepared by reactive sputtering
journal, August 2010

Laser additive synthesis of high entropy alloy coating on aluminum: Corrosion behavior
journal, March 2015

Electrochemical deposition and microstructural characterization of AlCrFeMnNi and AlCrCuFeMnNi high entropy alloy thin films
journal, December 2015

More than entropy in high-entropy alloys: Forming solid solutions or amorphous phase
journal, October 2013

Molecular dynamics simulations of clusters and thin film growth in the context of plasma sputtering deposition
journal, May 2014

Synthesis and characterization of multi-element oxynitride semiconductor film prepared by reactive sputtering deposition
journal, December 2012

PVD hard coatings applied for the wear protection of drawing dies
journal, October 2005

Characteristics of (TiAlCrNbY)C films deposited by reactive magnetron sputtering
journal, March 2010

Investigation of the nanostructure and wear properties of physical vapor deposited CrCuN nanocomposite coatings
journal, May 2005

(AlCrTaTiZr)N/(AlCrTaTiZr)N0.7 bilayer structure of high resistance to the interdiffusion of Cu and Si at 900°C
journal, January 2011

Formation of core–shell structure in high entropy alloy coating by laser cladding
journal, February 2016

Size Dependence of a First Order Solid-Solid Phase Transition: The Wurtzite to Rock Salt Transformation in CdSe Nanocrystals
journal, July 1994

Nanostructured High-Entropy Alloys with Multiple Principal Elements: Novel Alloy Design Concepts and Outcomes
journal, May 2004

Understanding phase stability of Al-Co-Cr-Fe-Ni high entropy alloys
journal, November 2016

Solid-Solution CrCoCuFeNi High-Entropy Alloy Thin Films Synthesized by Sputter Deposition
journal, June 2015

Effect of bias voltage on TiAlSiN nanocomposite coatings deposited by HiPIMS
journal, January 2017

Surface Energies and Thermodynamic Phase Stability in Nanocrystalline Aluminas
journal, August 1997

High-entropy alloys: a critical assessment of their founding principles and future prospects
journal, April 2016

Solid-Solution Phase Formation Rules for Multi-component Alloys
journal, June 2008

Effects of silicon content on the structure and mechanical properties of (AlCrTaTiZr)–Si _x –N coatings by reactive RF magnetron sputtering
journal, May 2011

On the significance of the H/E ratio in wear control: a nanocomposite coating approach to optimised tribological behaviour
journal, November 2000

Dense and smooth amorphous films of multicomponent FeCoNiCuVZrAl high-entropy alloy deposited by direct current magnetron sputtering
journal, April 2013

Structure and properties of two Al–Cr–Nb–Si–Ti high-entropy nitride coatings
journal, April 2013

Prediction of A2 to B2 Phase Transition in the High-Entropy Alloy Mo-Nb-Ta-W
journal, October 2013

Slurry Erosion Resistance of Laser Clad NiCoCrFeAl ₃ High-Entropy Alloy Coatings
journal, September 2015

Microstructure and thermal stability of a Ni-Cr-Co-Ti-V-Al high-entropy alloy coating by laser surface alloying
journal, September 2017

Soft Magnetic Properties of High-Entropy Fe-Co-Ni-Cr-Al-Si Thin Films
journal, August 2016