High-entropy functional materials
Abstract
While most papers on high-entropy alloys (HEAs) focus on the microstructure and mechanical properties for structural materials applications, there has been growing interest in developing high-entropy functional materials. The objective of this paper is to provide a brief, timely review on select functional properties of HEAs, including soft magnetic, magnetocaloric, physical, thermoelectric, superconducting, and hydrogen storage. Comparisons of functional properties between HEAs and conventional low- and medium-entropy materials are provided, and examples are illustrated using computational modeling and tuning the composition of existing functional materials through substitutional or interstitial mixing. Extending the concept of high configurational entropy to a wide range of materials such as intermetallics, ceramics, and semiconductors through the isostructural design approach is discussed. As a result, perspectives are offered in designing future high-performance functional materials utilizing the high-entropy concepts and high-throughput predictive computational modeling.
- Authors:
-
- National Energy Technology Lab. (NETL), Albany, OR (United States); AECOM, Albany, OR (United States)
- AF Research Lab, Wright-Patterson AFB, OH (United States)
- National Energy Technology Lab. (NETL), Albany, OR (United States)
- Univ. of Science and Technology Beijing, Beijing (People's Republic of China)
- Publication Date:
- Research Org.:
- National Energy Technology Laboratory (NETL), Pittsburgh, PA, Morgantown, WV, and Albany, OR (United States)
- Sponsoring Org.:
- FE; USDOE
- OSTI Identifier:
- 1509730
- Report Number(s):
- CONTR-PUB-478
Journal ID: ISSN 0884-2914
- Grant/Contract Number:
- FE0004000
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Journal of Materials Research
- Additional Journal Information:
- Journal Volume: 33; Journal Issue: 19; Journal ID: ISSN 0884-2914
- Publisher:
- Materials Research Society
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE
Citation Formats
Gao, Michael C., Miracle, Daniel B., Maurice, David, Yan, Xuehui, Zhang, Yong, and Hawk, Jeffrey A. High-entropy functional materials. United States: N. p., 2018.
Web. doi:10.1557/jmr.2018.323.
Gao, Michael C., Miracle, Daniel B., Maurice, David, Yan, Xuehui, Zhang, Yong, & Hawk, Jeffrey A. High-entropy functional materials. United States. https://doi.org/10.1557/jmr.2018.323
Gao, Michael C., Miracle, Daniel B., Maurice, David, Yan, Xuehui, Zhang, Yong, and Hawk, Jeffrey A. Thu .
"High-entropy functional materials". United States. https://doi.org/10.1557/jmr.2018.323. https://www.osti.gov/servlets/purl/1509730.
@article{osti_1509730,
title = {High-entropy functional materials},
author = {Gao, Michael C. and Miracle, Daniel B. and Maurice, David and Yan, Xuehui and Zhang, Yong and Hawk, Jeffrey A.},
abstractNote = {While most papers on high-entropy alloys (HEAs) focus on the microstructure and mechanical properties for structural materials applications, there has been growing interest in developing high-entropy functional materials. The objective of this paper is to provide a brief, timely review on select functional properties of HEAs, including soft magnetic, magnetocaloric, physical, thermoelectric, superconducting, and hydrogen storage. Comparisons of functional properties between HEAs and conventional low- and medium-entropy materials are provided, and examples are illustrated using computational modeling and tuning the composition of existing functional materials through substitutional or interstitial mixing. Extending the concept of high configurational entropy to a wide range of materials such as intermetallics, ceramics, and semiconductors through the isostructural design approach is discussed. As a result, perspectives are offered in designing future high-performance functional materials utilizing the high-entropy concepts and high-throughput predictive computational modeling.},
doi = {10.1557/jmr.2018.323},
journal = {Journal of Materials Research},
number = 19,
volume = 33,
place = {United States},
year = {Thu Sep 20 00:00:00 EDT 2018},
month = {Thu Sep 20 00:00:00 EDT 2018}
}
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Figures / Tables:
Table I: Part 1: Measured saturation magnetization (Ms, T) versus coercivity (Hc, A/m) for high entropy alloys reported in the literature.
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Magnetic properties of the CrMnFeCoNi high-entropy alloy
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Hybrid Monte Carlo/Molecular Dynamics Simulation of a Refractory Metal High Entropy Alloy
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- Carnegie Mellon University
Prediction of A2 to B2 Phase Transition in the High Entropy Alloy MoNbTaW
text, January 2013
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Works referencing / citing this record:
Semiconducting SiGeSn high-entropy alloy: A density functional theory study
journal, December 2019
- Wang, Duo; Liu, Lei; Huang, Wenjiang
- Journal of Applied Physics, Vol. 126, Issue 22
High entropy Sr((Zr 0.94 Y 0.06 ) 0.2 Sn 0.2 Ti 0.2 Hf 0.2 Mn 0.2 )O 3− x perovskite synthesis by reactive spark plasma sintering
journal, March 2019
- Biesuz, Mattia; Fu, Shuai; Dong, Jian
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TiVZrNb Multi-Principal-Element Alloy: Synthesis Optimization, Structural, and Hydrogen Sorption Properties
journal, July 2019
- Montero, Jorge; Zlotea, Claudia; Ek, Gustav
- Molecules, Vol. 24, Issue 15
Unveiling the mechanism of abnormal magnetic behavior of FeNiCoMnCu high-entropy alloys through a joint experimental-theoretical study
journal, January 2020
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Compositional Design of Soft Magnetic High Entropy Alloys by Minimizing Magnetostriction Coefficient in (Fe0.3Co0.5Ni0.2)100−x(Al1/3Si2/3)x System
journal, March 2019
- Zhang, Yong; Zhang, Min; Li, Dongyue
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High entropy alloys as a bold step forward in alloy development
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Transition from high-entropy to Cu-based (TiZrNbNi) 1− x Cu x metallic glasses
journal, October 2019
- Ristić, Ramir; Figueroa, Ignacio A.; Lachová, Andrea
- Journal of Applied Physics, Vol. 126, Issue 15
The AC Soft Magnetic Properties of FeCoNixCuAl (1.0 ≤ x ≤ 1.75) High-Entropy Alloys
journal, December 2019
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TiVZrNb Multi-Principal-Element Alloy: Synthesis Optimization, Structural, and Hydrogen Sorption Properties
journal, July 2019
- Montero, Jorge; Zlotea, Claudia; Ek, Gustav
- Molecules, Vol. 24, Issue 15
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