pH-Dependent structure of water-exposed surfaces of CdSe quantum dots
Abstract
Weakly-bound ligands in dynamic exchange expose the surface of CdSe quantum dots to pH-dependent modification.
- Authors:
-
- Department of Chemistry, Northwestern University, Evanston, USA
- Department of Biomedical Engineering and Chemistry of Life Processes Institute, Northwestern University, Evanston, USA
- Department of Chemistry, Northwestern University, Evanston, USA, Department of Biomedical Engineering and Chemistry of Life Processes Institute
- Publication Date:
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1507597
- Grant/Contract Number:
- SC0000989
- Resource Type:
- Publisher's Accepted Manuscript
- Journal Name:
- ChemComm
- Additional Journal Information:
- Journal Name: ChemComm Journal Volume: 55 Journal Issue: 38; Journal ID: ISSN 1359-7345
- Publisher:
- Royal Society of Chemistry (RSC)
- Country of Publication:
- United Kingdom
- Language:
- English
Citation Formats
Westmoreland, Dana E., Nap, Rikkert J., Arcudi, Francesca, Szleifer, Igal, and Weiss, Emily A. pH-Dependent structure of water-exposed surfaces of CdSe quantum dots. United Kingdom: N. p., 2019.
Web. doi:10.1039/C9CC01339C.
Westmoreland, Dana E., Nap, Rikkert J., Arcudi, Francesca, Szleifer, Igal, & Weiss, Emily A. pH-Dependent structure of water-exposed surfaces of CdSe quantum dots. United Kingdom. https://doi.org/10.1039/C9CC01339C
Westmoreland, Dana E., Nap, Rikkert J., Arcudi, Francesca, Szleifer, Igal, and Weiss, Emily A. Tue .
"pH-Dependent structure of water-exposed surfaces of CdSe quantum dots". United Kingdom. https://doi.org/10.1039/C9CC01339C.
@article{osti_1507597,
title = {pH-Dependent structure of water-exposed surfaces of CdSe quantum dots},
author = {Westmoreland, Dana E. and Nap, Rikkert J. and Arcudi, Francesca and Szleifer, Igal and Weiss, Emily A.},
abstractNote = {Weakly-bound ligands in dynamic exchange expose the surface of CdSe quantum dots to pH-dependent modification.},
doi = {10.1039/C9CC01339C},
journal = {ChemComm},
number = 38,
volume = 55,
place = {United Kingdom},
year = {Tue May 07 00:00:00 EDT 2019},
month = {Tue May 07 00:00:00 EDT 2019}
}
Free Publicly Available Full Text
Publisher's Version of Record
https://doi.org/10.1039/C9CC01339C
https://doi.org/10.1039/C9CC01339C
Other availability
Cited by: 11 works
Citation information provided by
Web of Science
Web of Science
Save to My Library
You must Sign In or Create an Account in order to save documents to your library.
Works referenced in this record:
Redox shuttle mechanism enhances photocatalytic H2 generation on Ni-decorated CdS nanorods
journal, August 2014
- Simon, Thomas; Bouchonville, Nicolas; Berr, Maximilian J.
- Nature Materials, Vol. 13, Issue 11
Enhancing the Rate of Quantum-Dot-Photocatalyzed Carbon–Carbon Coupling by Tuning the Composition of the Dot’s Ligand Shell
journal, March 2017
- Zhang, Zhengyi; Edme, Kedy; Lian, Shichen
- Journal of the American Chemical Society, Vol. 139, Issue 12
Mechanisms for Adsorption of Methyl Viologen on CdS Quantum Dots
journal, February 2014
- Peterson, Mark D.; Jensen, Stephen C.; Weinberg, David J.
- ACS Nano, Vol. 8, Issue 3
Preparation of compact biocompatible quantum dots using multicoordinating molecular-scale ligands based on a zwitterionic hydrophilic motif and lipoic acid anchors
journal, May 2015
- Zhan, Naiqian; Palui, Goutam; Mattoussi, Hedi
- Nature Protocols, Vol. 10, Issue 6
Molecularly imprinted polymer coated quantum dots for fluorescence sensing of acetaminophen
journal, December 2018
- Montaseri, Hanieh; Forbes, Patricia B. C.
- Materials Today Communications, Vol. 17
Organic Surfactant-Controlled Composition of the Surfaces of CdSe Quantum Dots
journal, March 2010
- Morris-Cohen, Adam J.; Frederick, Matthew T.; Lilly, G. Daniel
- The Journal of Physical Chemistry Letters, Vol. 1, Issue 7
Geochemical behavior of antimony, arsenic, cadmium and thallium: EhpH diagrams for 25°C, 1-bar pressure
journal, February 1986
- Brookins, Douglas G.
- Chemical Geology, Vol. 54, Issue 3-4
Use of potential determining ions to control energetics and photochemical charge transfer of a nanoscale water splitting photocatalyst
journal, January 2014
- Chamousis, Rachel L.; Osterloh, Frank E.
- Energy Environ. Sci., Vol. 7, Issue 2
Strategies for interfacing inorganic nanocrystals with biological systems based on polymer-coating
journal, January 2015
- Palui, Goutam; Aldeek, Fadi; Wang, Wentao
- Chemical Society Reviews, Vol. 44, Issue 1
Primary Reactions in the Photocorrosion of CdSe Through Photocapacitance Measurements
journal, January 1991
- Allongue, Ph.
- Journal of The Electrochemical Society, Vol. 138, Issue 1
A Ligand System for the Flexible Functionalization of Quantum Dots via Click Chemistry
journal, March 2018
- Chen, Yue; Cordero, Jose M.; Wang, Hua
- Angewandte Chemie International Edition, Vol. 57, Issue 17
Organic-to-Aqueous Phase Transfer of Cadmium Chalcogenide Quantum Dots Using a Sulfur-Free Ligand for Enhanced Photoluminescence and Oxidative Stability
journal, September 2016
- Calzada, Raul; Thompson, Christopher M.; Westmoreland, Dana E.
- Chemistry of Materials, Vol. 28, Issue 18
Semiconductor Nanocrystals as Fluorescent Biological Labels
patent, September 1998
- Bruchez Jr., Marcel; Moronne, Mario Moronne; Gin, Peter Gin
- Science, Vol. 281, Issue 5385, p. 2013-2016
Characterization of Photochemical Processes for H 2 Production by CdS Nanorod–[FeFe] Hydrogenase Complexes
journal, March 2012
- Brown, Katherine A.; Wilker, Molly B.; Boehm, Marko
- Journal of the American Chemical Society, Vol. 134, Issue 12
One-pot, low-temperature synthesis of self-doped NaTaO3 nanoclusters for visible-light-driven photocatalysis
journal, January 2013
- Wang, Jianqiang; Su, Shuangyue; Liu, Bing
- Chemical Communications, Vol. 49, Issue 71
Size-Dependent Dissociation pH of Thiolate Ligands from Cadmium Chalcogenide Nanocrystals
journal, February 2005
- Aldana, Jose; Lavelle, Natasha; Wang, Yunjun
- Journal of the American Chemical Society, Vol. 127, Issue 8
Electrostatic Control of Excitonic Energies and Dynamics in a CdS Quantum Dot through Reversible Protonation of Its Ligands
journal, September 2016
- Thompson, Christopher M.; Kodaimati, Mohamad; Westmoreland, Dana
- The Journal of Physical Chemistry Letters, Vol. 7, Issue 19
Selective Photocatalytic Oxidation of Benzyl Alcohol to Benzaldehyde or C–C Coupled Products by Visible-Light-Absorbing Quantum Dots
journal, October 2018
- McClelland, Kevin P.; Weiss, Emily A.
- ACS Applied Energy Materials, Vol. 2, Issue 1
Solar-driven reforming of lignocellulose to H2 with a CdS/CdOx photocatalyst
journal, March 2017
- Wakerley, David W.; Kuehnel, Moritz F.; Orchard, Katherine L.
- Nature Energy, Vol. 2, Issue 4
Photocatalytic Conversion of Nitrobenzene to Aniline through Sequential Proton-Coupled One-Electron Transfers from a Cadmium Sulfide Quantum Dot
journal, January 2016
- Jensen, Stephen C.; Bettis Homan, Stephanie; Weiss, Emily A.
- Journal of the American Chemical Society, Vol. 138, Issue 5
Electrochemical equilibria of cadmium and water and the dissolution of cadmium as a function of pH
journal, January 1975
- Tomlinson, W. J.; Wardle, N.
- Corrosion Science, Vol. 15, Issue 6-12
Morphology and Capacity of a Cadmium Electrode
journal, January 1973
- Will, F. G.; Hess, H. J.
- Journal of The Electrochemical Society, Vol. 120, Issue 1
Highly luminescent core–shell InP/ZnX (X = S, Se) quantum dots prepared via a phosphine synthetic route
journal, January 2017
- Mordvinova, Natalia; Vinokurov, Alexander; Kuznetsova, Tatiana
- Dalton Transactions, Vol. 46, Issue 4
General and Efficient C–C Bond Forming Photoredox Catalysis with Semiconductor Quantum Dots
journal, March 2017
- Caputo, Jill A.; Frenette, Leah C.; Zhao, Norman
- Journal of the American Chemical Society, Vol. 139, Issue 12
Size and zeta potential of CdS nanoparticles in stable aqueous solution of EDTA and NaCl
journal, February 2015
- Kuznetsova, Yu. V.; Rempel, A. A.
- Inorganic Materials, Vol. 51, Issue 3
Binding of Phosphonic Acids to CdSe Quantum Dots: A Solution NMR Study
journal, January 2011
- Gomes, Raquel; Hassinen, Antti; Szczygiel, Agnieszka
- The Journal of Physical Chemistry Letters, Vol. 2, Issue 3
Synthesis and Properties of Biocompatible Water-Soluble Silica-Coated CdSe/ZnS Semiconductor Quantum Dots †
journal, September 2001
- Gerion, Daniele; Pinaud, Fabien; Williams, Shara C.
- The Journal of Physical Chemistry B, Vol. 105, Issue 37
Ligand Exchange and the Stoichiometry of Metal Chalcogenide Nanocrystals: Spectroscopic Observation of Facile Metal-Carboxylate Displacement and Binding
journal, November 2013
- Anderson, Nicholas C.; Hendricks, Mark P.; Choi, Joshua J.
- Journal of the American Chemical Society, Vol. 135, Issue 49, p. 18536-18548
L-cysteine and 3-mercaptopropionic acid capped cadmium selenide quantum dots based metal ion probes
journal, July 2017
- Sajwan, Reena K.; Bagbi, Yana; Sharma, Purnima
- Journal of Luminescence, Vol. 187