Soft Magnetic Multilayered FeSiCrB–Fe$_{x}$N Metallic Glass Composites Fabricated by Spark Plasma Sintering

Monson, Todd C.; Zheng, Baolong; Delany, Robert E.; Pearce, Charles Joseph; Langlois, Eric D.; Lepkowski, Stefan Mark; Stevens, Tyler Eugene; Zhou, Yizhang; Atcitty, Stanley; Lavernia, Enrique J.

doi:10.1109/LMAG.2019.2906832

Title: Soft Magnetic Multilayered FeSiCrB–Fe$$_{x}$$N Metallic Glass Composites Fabricated by Spark Plasma Sintering

Full Record
Other Related Research

Abstract

Novel multilayered FeSiCrB–Fe $$_{x}$$ N ( x = 2–4) metallic glass composites were fabricated using spark plasma sintering of FeSiCrB amorphous ribbons (Metglas 2605SA3 alloy) and Fe $$_{x}$$ N ( x = 2–4) powder. Crystalline Fe $$_{x}$$ N can serve as a high magnetic moment, high electrical resistance binder, and lamination material in the consolidation of amorphous and nanocrystalline ribbons, mitigating eddy currents while boosting magnetic performance and stacking factor in both wound and stacked soft magnetic cores. Stacking factors of nearly 100% can be achieved in an amorphous ribbon/iron nitride composite. FeSiCrB–Fe $$_{x}$$ N multilayered metallic glass composites prepared by spark plasma sintering have the potential to serve as a next-generation soft magnetic material in power electronics and electrical machines.

Authors:

^[1]; Zheng, Baolong ^[2]; Delany, Robert E. ^[1];

^[1]; Langlois, Eric D. ^[1]; Lepkowski, Stefan Mark ^[1];

^[1]; Zhou, Yizhang ^[2]; Atcitty, Stanley ^[1];

^[2]

Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
Univ. of California, Irvine, CA (United States)

Publication Date:: 2019-03-27

Research Org.:: Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)

Sponsoring Org.:: USDOE Office of Electricity (OE)

OSTI Identifier:: 1507518

Report Number(s):: SAND-2019-3014J
Journal ID: ISSN 1949-307X; 673533

Grant/Contract Number:: AC04-94AL85000

Resource Type:: Accepted Manuscript

Journal Name:: IEEE Magnetics Letters

Additional Journal Information:: Journal Volume: 10; Journal ID: ISSN 1949-307X

Publisher:: IEEE

Country of Publication:: United States

Language:: English

Subject:: 36 MATERIALS SCIENCE; soft magnetic materials; amorphous alloys; composites; iron nitride; soft magnets; spark plasma sintering

Citation Formats


                    Monson, Todd C., Zheng, Baolong, Delany, Robert E., Pearce, Charles Joseph, Langlois, Eric D., Lepkowski, Stefan Mark, Stevens, Tyler Eugene, Zhou, Yizhang, Atcitty, Stanley, and Lavernia, Enrique J.. Soft Magnetic Multilayered FeSiCrB–Fe$_{x}$N Metallic Glass Composites Fabricated by Spark Plasma Sintering.  United States: N. p., 2019. 
Web.  doi:10.1109/LMAG.2019.2906832.

Copy to clipboard


                    Monson, Todd C., Zheng, Baolong, Delany, Robert E., Pearce, Charles Joseph, Langlois, Eric D., Lepkowski, Stefan Mark, Stevens, Tyler Eugene, Zhou, Yizhang, Atcitty, Stanley, & Lavernia, Enrique J.. Soft Magnetic Multilayered FeSiCrB–Fe$_{x}$N Metallic Glass Composites Fabricated by Spark Plasma Sintering.  United States.  https://doi.org/10.1109/LMAG.2019.2906832

Copy to clipboard


                    Monson, Todd C., Zheng, Baolong, Delany, Robert E., Pearce, Charles Joseph, Langlois, Eric D., Lepkowski, Stefan Mark, Stevens, Tyler Eugene, Zhou, Yizhang, Atcitty, Stanley, and Lavernia, Enrique J.. Wed .  
"Soft Magnetic Multilayered FeSiCrB–Fe$_{x}$N Metallic Glass Composites Fabricated by Spark Plasma Sintering".  United States.  https://doi.org/10.1109/LMAG.2019.2906832.  https://www.osti.gov/servlets/purl/1507518.

Copy to clipboard


                    
@article{osti_1507518,

  title        = {Soft Magnetic Multilayered FeSiCrB–Fe$_{x}$N Metallic Glass Composites Fabricated by Spark Plasma Sintering},

  author       = {Monson, Todd C. and Zheng, Baolong and Delany, Robert E. and Pearce, Charles Joseph and Langlois, Eric D. and Lepkowski, Stefan Mark and Stevens, Tyler Eugene and Zhou, Yizhang and Atcitty, Stanley and Lavernia, Enrique J.},

  abstractNote = {Novel multilayered FeSiCrB–Fe $_{x}$ N ( x = 2–4) metallic glass composites were fabricated using spark plasma sintering of FeSiCrB amorphous ribbons (Metglas 2605SA3 alloy) and Fe $_{x}$ N ( x = 2–4) powder. Crystalline Fe $_{x}$ N can serve as a high magnetic moment, high electrical resistance binder, and lamination material in the consolidation of amorphous and nanocrystalline ribbons, mitigating eddy currents while boosting magnetic performance and stacking factor in both wound and stacked soft magnetic cores. Stacking factors of nearly 100% can be achieved in an amorphous ribbon/iron nitride composite. FeSiCrB–Fe $_{x}$ N multilayered metallic glass composites prepared by spark plasma sintering have the potential to serve as a next-generation soft magnetic material in power electronics and electrical machines.},

  doi          = {10.1109/LMAG.2019.2906832},

  journal      = {IEEE Magnetics Letters},

  number       = ,

  volume       = 10,

  place        = {United States},

  year         = {2019},

  month        = {3}

}

Copy to clipboard

Journal Article:

Free Publicly Available Full Text

Accepted Manuscript (DOE)

Publisher's Version of Record

https://doi.org/10.1109/LMAG.2019.2906832

Other availability

Search WorldCat to find libraries that may hold this journal

Citation Metrics:

Cited by: 3 works

Citation information provided by
Web of Science

Save / Share:

Export Metadata

Save to My Library

Similar Records in DOE PAGES and OSTI.GOV collections:

Phase stability and magnetic and electronic properties of a spark plasma sintered CoFe – P soft magnetic alloy

Journal Article Belcher, Calvin H. ; Zheng, Baolong ; Dickens, Sara M. ; ... - Journal of Alloys and Compounds

More efficient power conversion devices are able to transmit greater electrical power across larger distances to satisfy growing global electrical needs. A critical requirement to achieve more efficient power conversion are the soft magnetic materials used as core materials in transformers, inductors, and motors. To that effect it is well known that the use of non-equilibrium microstructures, which are, for example, nanocrystalline or consist of single phase solid solutions, can yield high saturation magnetic polarization and high electrical resistivity necessary for more efficient soft magnetic materials. In this work, we synthesized CoFe – P soft magnetic alloys containing nanocrystalline, singlemore »« less
https://doi.org/10.1016/j.jallcom.2022.166756

Full Text Available
Synthesis and behavior of bulk iron nitride soft magnets via high-pressure spark plasma sintering

Journal Article Monson, Todd C. ; Zheng, Baolong ; Delaney, Robert E. ; ... - Journal of Materials Research

Abstract In this study, dense bulk iron nitrides (Fe _x N) were synthesized for the first time ever using spark plasma sintering (SPS) of Fe _x N powders. The Fe ₄ N phase of iron nitride in particular has significant potential to serve as a new soft magnetic material in both transformer and inductor cores and electrical machines. The density of SPSed Fe _x N increased with SPS temperature and pressure. The microstructure of the consolidated bulk Fe _x N was characterized with X-ray diffraction (XRD), scanning electron microscopy (SEM), transmission electronmore »« less
https://doi.org/10.1557/s43578-021-00379-z
Nanocrystallization in spark plasma sintered Fe{sub 48}Cr{sub 15}Mo{sub 14}Y{sub 2}C{sub 15}B{sub 6} bulk amorphous alloy

Journal Article Singh, Ashish ; Harimkar, Sandip P. ; Katakam, Shravana ; ... - Journal of Applied Physics

Spark plasma sintering (SPS) is evolving as an attractive process for the processing of multi-component Fe-based bulk amorphous alloys and their in-situ nanocomposites with controlled primary nanocrystallization. Extended Q-range small angle neutron scattering (EQ-SANS) analysis, complemented by x-ray diffraction and transmission electron microscopy, was performed to characterize nanocrystallization behavior of SPS sintered Fe-based bulk amorphous alloys. The SANS experiments show significant scattering for the samples sintered in the supercooled region indicating local structural/compositional changes associated with the profuse nucleation of nanoclusters (∼4 nm). For the samples spark plasma sintered near and above crystallization temperature (>653 °C), the SANS data showmore »« less
https://doi.org/10.1063/1.4817379
Magnetic properties of Nd-Fe-Ti-C-B nanocomposite magnets produced by spark plasma sintering method

Journal Article Saito, Tetsuji - Journal of Applied Physics

Amorphous melt-spun ribbons of a Nd{sub 9}Fe{sub 73}Ti{sub 4}C{sub 1}B{sub 13} alloy were consolidated into bulk materials by the spark plasma sintering method. The resultant bulk material was amorphous when the ribbons were consolidated at 773 K. The amorphous bulk material showed a low coercivity, as would be expected for amorphous Nd-Fe-B materials. On the other hand, the bulk materials produced at 873 K and above consisted of {alpha}-Fe and Nd{sub 2}Fe{sub 14}B phases. The resultant nanocomposite magnets showed high coercivity values exceeding 10 kOe. The bulk material produced at 973 K showed a high remanence of 8.4 kG withmore »« less
https://doi.org/10.1063/1.2172907
The investigation of order–disorder transition process of ZSM-5 induced by spark plasma sintering

Journal Article Wang, Liang ; Wang, Lianjun ; Jiang, Wan ; ... - Journal of Solid State Chemistry

Based on the amorphization of zeolites, an order–disorder transition method was used to prepare silica glass via Spark Plasma Sintering (SPS). In order to get a better understanding about the mechanism of amorphization induced by SPS, the intermediate products in this process were prepared and characterized by different characterization techniques. X-ray diffraction and High-energy synchrotron X-ray scattering show a gradual transformation from ordered crystal to glass. Local structural changes in glass network including Si–O bond length, O–Si–O bond angle, size of rings, coordination were detected by Infrared spectroscopy and {sup 29}Si magic-angle spinning nuclear magnetic resonance (NMR) spectroscopy. Topologically ordered,more »« less
https://doi.org/10.1016/J.JSSC.2014.01.024

Similar Records