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Title: Understanding inks for porous-electrode formation

Scalable manufacturing of high-aspect-ratio multi-material electrodes are important for advanced energy storage and conversion systems. Such technologies often rely on solution-based processing methods where the active material is dispersed in a colloidal ink. To date, ink formulation has primarily focused on macro-scale process-specific optimization (i.e. viscosity and surface/interfacial tension), and been optimized mainly empirically. Thus, there is a further need to understand nano- and mesoscale interactions and how they can be engineered for controlled macroscale properties and structures related to performance, durability, and material utilization in electrochemical systems.
Authors:
ORCiD logo [1] ;  [1] ;  [2] ; ORCiD logo [2]
  1. Vanderbilt Univ., Nashville, TN (United States)
  2. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
Publication Date:
Grant/Contract Number:
AC02-05CH11231
Type:
Accepted Manuscript
Journal Name:
Journal of Materials Chemistry. A
Additional Journal Information:
Journal Volume: 5; Journal Issue: 39; Journal ID: ISSN 2050-7488
Publisher:
Royal Society of Chemistry
Research Org:
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
Sponsoring Org:
USDOE Office of Energy Efficiency and Renewable Energy (EERE), Fuel Cell Technologies Office (EE-3F)
Country of Publication:
United States
Language:
English
Subject:
42 ENGINEERING
OSTI Identifier:
1506265

Hatzell, Kelsey B., Dixit, Marm B., Berlinger, Sarah A., and Weber, Adam Z.. Understanding inks for porous-electrode formation. United States: N. p., Web. doi:10.1039/c7ta07255d.
Hatzell, Kelsey B., Dixit, Marm B., Berlinger, Sarah A., & Weber, Adam Z.. Understanding inks for porous-electrode formation. United States. doi:10.1039/c7ta07255d.
Hatzell, Kelsey B., Dixit, Marm B., Berlinger, Sarah A., and Weber, Adam Z.. 2017. "Understanding inks for porous-electrode formation". United States. doi:10.1039/c7ta07255d. https://www.osti.gov/servlets/purl/1506265.
@article{osti_1506265,
title = {Understanding inks for porous-electrode formation},
author = {Hatzell, Kelsey B. and Dixit, Marm B. and Berlinger, Sarah A. and Weber, Adam Z.},
abstractNote = {Scalable manufacturing of high-aspect-ratio multi-material electrodes are important for advanced energy storage and conversion systems. Such technologies often rely on solution-based processing methods where the active material is dispersed in a colloidal ink. To date, ink formulation has primarily focused on macro-scale process-specific optimization (i.e. viscosity and surface/interfacial tension), and been optimized mainly empirically. Thus, there is a further need to understand nano- and mesoscale interactions and how they can be engineered for controlled macroscale properties and structures related to performance, durability, and material utilization in electrochemical systems.},
doi = {10.1039/c7ta07255d},
journal = {Journal of Materials Chemistry. A},
number = 39,
volume = 5,
place = {United States},
year = {2017},
month = {9}
}

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