Electrochemically activated spinel manganese oxide for rechargeable aqueous aluminum battery
Abstract
Aluminum is a naturally abundant, trivalent charge carrier with high theoretical specific capacity and volumetric energy density, rendering aluminum-ion batteries a technology of choice for future large-scale energy storage. Nonetheless, the frequent collapse of the host structure of the cathode materials and sluggish kinetics of aluminum ion diffusion have thus far hampered the realization of practical battery devices. Here, we synthesize AlxMnO2•nH2O by an in-situ electrochemical transformation reaction to be used as a cathode material for an aluminum-ion battery with a configuration of Al/Al(OTF)3-H2O/AlxMnO2•nH2O. This cell is not only based on aqueous electrolyte chemistry but also delivers a high specific capacity of 467 mAh g-1 and a record high energy density of 481 Wh kg-1. The high safety of aqueous electrolyte, facile cell assembly and the low cost of materials suggest that this aqueous aluminum-ion battery holds promise for large-scale energy applications.
- Authors:
-
[4];
[4]
- Beijing Inst. of Technology, Beijing (China); Collaborative Innovation Center of Electric Vehicles in Beijing, Beijing (China)
- Beijing Inst. of Technology, Beijing (China)
- Chinese Academy of Sciences (CAS), Beijing (China)
- Argonne National Laboratory (ANL), Lemont, IL (United States)
- Publication Date:
- Research Org.:
- Argonne National Laboratory (ANL), Argonne, IL (United States)
- Sponsoring Org.:
- USDOE Office of Energy Efficiency and Renewable Energy (EERE), Vehicle Technologies Office (EE-3V)
- OSTI Identifier:
- 1504227
- Grant/Contract Number:
- AC02-06CH11357
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Communications
- Additional Journal Information:
- Journal Volume: 10; Journal Issue: 1; Journal ID: ISSN 2041-1723
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 25 ENERGY STORAGE
Citation Formats
Wu, Chuan, Gu, Sichen, Zhang, Qinghua, Bai, Ying, Li, Matthew, Yuan, Yifei, Wang, Huali, Liu, Xinyu, Yuan, Yanxia, Zhu, Na, Wu, Feng, Li, Hong, Gu, Lin, and Lu, Jun. Electrochemically activated spinel manganese oxide for rechargeable aqueous aluminum battery. United States: N. p., 2019.
Web. doi:10.1038/s41467-018-07980-7.
Wu, Chuan, Gu, Sichen, Zhang, Qinghua, Bai, Ying, Li, Matthew, Yuan, Yifei, Wang, Huali, Liu, Xinyu, Yuan, Yanxia, Zhu, Na, Wu, Feng, Li, Hong, Gu, Lin, & Lu, Jun. Electrochemically activated spinel manganese oxide for rechargeable aqueous aluminum battery. United States. https://doi.org/10.1038/s41467-018-07980-7
Wu, Chuan, Gu, Sichen, Zhang, Qinghua, Bai, Ying, Li, Matthew, Yuan, Yifei, Wang, Huali, Liu, Xinyu, Yuan, Yanxia, Zhu, Na, Wu, Feng, Li, Hong, Gu, Lin, and Lu, Jun. Tue .
"Electrochemically activated spinel manganese oxide for rechargeable aqueous aluminum battery". United States. https://doi.org/10.1038/s41467-018-07980-7. https://www.osti.gov/servlets/purl/1504227.
@article{osti_1504227,
title = {Electrochemically activated spinel manganese oxide for rechargeable aqueous aluminum battery},
author = {Wu, Chuan and Gu, Sichen and Zhang, Qinghua and Bai, Ying and Li, Matthew and Yuan, Yifei and Wang, Huali and Liu, Xinyu and Yuan, Yanxia and Zhu, Na and Wu, Feng and Li, Hong and Gu, Lin and Lu, Jun},
abstractNote = {Aluminum is a naturally abundant, trivalent charge carrier with high theoretical specific capacity and volumetric energy density, rendering aluminum-ion batteries a technology of choice for future large-scale energy storage. Nonetheless, the frequent collapse of the host structure of the cathode materials and sluggish kinetics of aluminum ion diffusion have thus far hampered the realization of practical battery devices. Here, we synthesize AlxMnO2•nH2O by an in-situ electrochemical transformation reaction to be used as a cathode material for an aluminum-ion battery with a configuration of Al/Al(OTF)3-H2O/AlxMnO2•nH2O. This cell is not only based on aqueous electrolyte chemistry but also delivers a high specific capacity of 467 mAh g-1 and a record high energy density of 481 Wh kg-1. The high safety of aqueous electrolyte, facile cell assembly and the low cost of materials suggest that this aqueous aluminum-ion battery holds promise for large-scale energy applications.},
doi = {10.1038/s41467-018-07980-7},
journal = {Nature Communications},
number = 1,
volume = 10,
place = {United States},
year = {Tue Jan 08 00:00:00 EST 2019},
month = {Tue Jan 08 00:00:00 EST 2019}
}
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