Chemomechanical behaviors of layered cathode materials in alkali metal ion batteries

Xu, Zhengrui; Rahman, Muhammad Mominur; Mu, Linqin; Liu, Yijin; Lin, Feng

doi:10.1039/c8ta06875e

Title: Chemomechanical behaviors of layered cathode materials in alkali metal ion batteries

Journal Article · 21 October 2018 · Journal of Materials Chemistry. A

DOI: https://doi.org/10.1039/c8ta06875e · OSTI ID:1503597

Xu, Zhengrui ^[1]; Rahman, Muhammad Mominur ^[1]; Mu, Linqin ^[1];

^[2];

^[1]

Virginia Polytechnic Inst. and State Univ. (Virginia Tech), Blacksburg, VA (United States)
SLAC National Accelerator Lab. (SLAC), Menlo Park, CA (United States)

Layered cathode materials (LCMs), because of their high energy density and relatively stable performance, represent an important class of cathode materials for alkali metal ion (e.g., Li⁺ and Na⁺) batteries. Chemomechanical behaviors of LCMs, which affect battery performance dramatically, have drawn extensive attention in recent years. Most chemomechanical processes have some common chemical and structural origins that are at the center of materials chemistry, for example, defects and local bonding environments in the solid state. In this review, we first discuss the chemomechanical breakdown of LCMs by introducing their categories and negative effects on the battery performance. We then systematically analyze factors that govern the initiation and propagation of chemomechanical breakdown and summarize their formation mechanisms. Strategies that can enhance the chemomechanical properties of LCMs or reduce the destructive effects of chemomechanical breakdown are then discussed. Lastly, light is shed on the new state-of-the-art techniques that have been applied to study chemomechanical breakdown. This review virtually includes most aspects of the chemomechanical behaviors of LCMs and provides some insights into the important chemical motifs that determine the chemomechanical properties. Thus, we believe that advanced design protocols of LCMs can be developed to effectively address the chemomechanical breakdown issue of LCMs.

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Research Organization:: SLAC National Accelerator Lab. (SLAC), Menlo Park, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

Grant/Contract Number:: AC02-76SF00515

OSTI ID:: 1503597

Journal Information:: Journal of Materials Chemistry. A, Journal Name: Journal of Materials Chemistry. A Journal Issue: 44 Vol. 6; ISSN 2050-7488

Publisher:: Royal Society of ChemistryCopyright Statement

Country of Publication:: United States

Language:: English

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