Magic high-order harmonics from a quasi-one-dimensional hexagonal solid
Abstract
High-order harmonic generation (HHG) from atoms is a coherent light source that opens up attosecond physics, but it is the application of HHG to solids that has brought much excitement in the last decade. Here in this paper we report a special kind of harmonics in a quasi-one-dimensional and hexagonal barium titanium sulfide: Under circularly polarized laser excitation, harmonics are generated only at first, fifth, seventh, and eleventh orders. These magic harmonics appear only with circularly polarized light, not with linearly polarized light. Neither cubic nor tetragonal cells have magic harmonics even with circularly polarized light. Through a careful group-theory analysis, we find that two subgroups of symmetry operations unique to the hexagonal symmetry cancel out third and ninth harmonics. This feature presents a rare opportunity to develop HHG into a crystal-structure characterization tool for phase transitions between hexagonal and nonhexagonal structures..
- Authors:
-
- Indiana State Univ. Terre Haute, IN (United States). Dept. of Physics
- Publication Date:
- Research Org.:
- Indiana State Univ. Terre Haute, IN (United States); Indiana State Univ., Terre Haute, IN (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division
- OSTI Identifier:
- 1503569
- Alternate Identifier(s):
- OSTI ID: 1593942
- Report Number(s):
- NA
Journal ID: ISSN 2469-9950; PRBMDO
- Grant/Contract Number:
- FG02-06ER46304; AC02-05CH11231
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Physical Review B
- Additional Journal Information:
- Journal Volume: 99; Journal Issue: 9; Journal ID: ISSN 2469-9950
- Publisher:
- American Physical Society (APS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 74 ATOMIC AND MOLECULAR PHYSICS; 36 MATERIALS SCIENCE
Citation Formats
Zhang, G. P., and Bai, Y. H. Magic high-order harmonics from a quasi-one-dimensional hexagonal solid. United States: N. p., 2019.
Web. doi:10.1103/PhysRevB.99.094313.
Zhang, G. P., & Bai, Y. H. Magic high-order harmonics from a quasi-one-dimensional hexagonal solid. United States. https://doi.org/10.1103/PhysRevB.99.094313
Zhang, G. P., and Bai, Y. H. Thu .
"Magic high-order harmonics from a quasi-one-dimensional hexagonal solid". United States. https://doi.org/10.1103/PhysRevB.99.094313. https://www.osti.gov/servlets/purl/1503569.
@article{osti_1503569,
title = {Magic high-order harmonics from a quasi-one-dimensional hexagonal solid},
author = {Zhang, G. P. and Bai, Y. H.},
abstractNote = {High-order harmonic generation (HHG) from atoms is a coherent light source that opens up attosecond physics, but it is the application of HHG to solids that has brought much excitement in the last decade. Here in this paper we report a special kind of harmonics in a quasi-one-dimensional and hexagonal barium titanium sulfide: Under circularly polarized laser excitation, harmonics are generated only at first, fifth, seventh, and eleventh orders. These magic harmonics appear only with circularly polarized light, not with linearly polarized light. Neither cubic nor tetragonal cells have magic harmonics even with circularly polarized light. Through a careful group-theory analysis, we find that two subgroups of symmetry operations unique to the hexagonal symmetry cancel out third and ninth harmonics. This feature presents a rare opportunity to develop HHG into a crystal-structure characterization tool for phase transitions between hexagonal and nonhexagonal structures..},
doi = {10.1103/PhysRevB.99.094313},
journal = {Physical Review B},
number = 9,
volume = 99,
place = {United States},
year = {Thu Mar 28 00:00:00 EDT 2019},
month = {Thu Mar 28 00:00:00 EDT 2019}
}
Free Publicly Available Full Text
Publisher's Version of Record
Other availability
Search WorldCat to find libraries that may hold this journal
Cited by: 10 works
Citation information provided by
Web of Science
Web of Science
Save to My Library
You must Sign In or Create an Account in order to save documents to your library.
Works referenced in this record:
Transformation of Cubic Boron Nitride to a Graphitic Form of Hexagonal Boron Nitride
journal, August 1959
- Milledge, H. Judith; Nave, E.; Weller, F. H.
- Nature, Vol. 184, Issue 4687
Observation of multiple-harmonic radiation induced from a gold surface by picosecond neodymium-doped yttrium aluminum garnet laser pulses
journal, October 1992
- Farkas, Gy.; Tóth, Cs.; Moustaizis, S. D.
- Physical Review A, Vol. 46, Issue 7
Giant optical anisotropy in a quasi-one-dimensional crystal
journal, June 2018
- Niu, Shanyuan; Joe, Graham; Zhao, Huan
- Nature Photonics, Vol. 12, Issue 7
Generalized Gradient Approximation Made Simple
journal, October 1996
- Perdew, John P.; Burke, Kieron; Ernzerhof, Matthias
- Physical Review Letters, Vol. 77, Issue 18, p. 3865-3868
Identification of optical transitions in cubic and hexagonal GaN by spatially resolved cathodoluminescence
journal, January 1996
- Menniger, J.; Jahn, U.; Brandt, O.
- Physical Review B, Vol. 53, Issue 4
Colloquium : Strong-field phenomena in periodic systems
journal, April 2018
- Kruchinin, Stanislav Yu.; Krausz, Ferenc; Yakovlev, Vladislav S.
- Reviews of Modern Physics, Vol. 90, Issue 2
Anisotropic exchange interaction between nonmagnetic europium cations in Eu O
journal, July 2011
- Concas, G.; Dewhurst, J. K.; Sanna, A.
- Physical Review B, Vol. 84, Issue 1
Energy- and crystal momentum-resolved study of laser-induced femtosecond magnetism
journal, December 2009
- Zhang, G. P.; Bai, Yihua; George, Thomas F.
- Physical Review B, Vol. 80, Issue 21
Ultrafast Spin Dynamics in Ferromagnetic Nickel
journal, May 1996
- Beaurepaire, E.; Merle, J. -C.; Daunois, A.
- Physical Review Letters, Vol. 76, Issue 22
Observation of high-order harmonic generation in a bulk crystal
journal, December 2010
- Ghimire, Shambhu; DiChiara, Anthony D.; Sistrunk, Emily
- Nature Physics, Vol. 7, Issue 2
Anisotropic high-harmonic generation in bulk crystals
journal, November 2016
- You, Yong Sing; Reis, David A.; Ghimire, Shambhu
- Nature Physics, Vol. 13, Issue 4
Paradigm of the time-resolved magneto-optical Kerr effect for femtosecond magnetism
journal, June 2009
- Zhang, G. P.; Hübner, W.; Lefkidis, Georgios
- Nature Physics, Vol. 5, Issue 7
The spatial symmetric forms of third-order nonlinear susceptibility
journal, February 1987
- Shang, C.; Hsu, H.
- IEEE Journal of Quantum Electronics, Vol. 23, Issue 2
Third-order optical susceptibilities of liquids and solids
journal, January 1977
- Hellwarth, R. W.
- Progress in Quantum Electronics, Vol. 5
Initial growth of hexagonal and cubic boron nitride: A theoretical study
journal, August 2003
- Olander, J.; Larsson, K.
- Physical Review B, Vol. 68, Issue 7
Electron correlation decides the stability of cubic versus hexagonal boron nitride
journal, January 2011
- Halo, Migen; Pisani, Cesare; Maschio, Lorenzo
- Physical Review B, Vol. 83, Issue 3
Identification of the cubic-to-hexagonal phase transition for the production of stable zinc oxynitride layers
journal, January 2018
- Gómez-Castaño, M.; Pau, J. L.; Redondo-Cubero, A.
- CrystEngComm, Vol. 20, Issue 26
Generating high-order optical and spin harmonics from ferromagnetic monolayers
journal, August 2018
- Zhang, G. P.; Si, M. S.; Murakami, M.
- Nature Communications, Vol. 9, Issue 1
Notizen: Die Kristallstruktur von BaTiS3/Crystal Structure of BaTiS3
journal, June 1980
- Huster, Jürgen
- Zeitschrift für Naturforschung B, Vol. 35, Issue 6
Harmonic generation by a one-dimensional conductor: Exact results
journal, August 1994
- Pronin, Kirill A.; Bandrauk, André D.; Ovchinnikov, Alexander A.
- Physical Review B, Vol. 50, Issue 5
Catalyzing Cubic-to-Hexagonal Phase Transition in NaYF 4 via Ligand Enhanced Surface Ordering
journal, July 2018
- Saha, Sulay; Pala, Raj Ganesh S.; Sivakumar, Sri
- Crystal Growth & Design, Vol. 18, Issue 9
Optical High Harmonic Generation in
journal, July 2005
- Zhang, G. P.
- Physical Review Letters, Vol. 95, Issue 4
Hexagonal to cubic crystal structure transformation during aerosol deposition of aluminum nitride
journal, February 2005
- Iwata, Atsushi; Akedo, Jun
- Journal of Crystal Growth, Vol. 275, Issue 1-2
Structural aspects of the metal-insulator transition in BaVS3
journal, June 2005
- Fagot, S.; Foury-Leylekian, P.; Ravy, S.
- Solid State Sciences, Vol. 7, Issue 6
All-Optical Reconstruction of Crystal Band Structure
journal, November 2015
- Vampa, G.; Hammond, T. J.; Thiré, N.
- Physical Review Letters, Vol. 115, Issue 19
Nonlinear optical properties of one-dimensional semiconductors and conjugated polymers
journal, January 1978
- Agrawal, G. P.; Cojan, C.; Flytzanis, C.
- Physical Review B, Vol. 17, Issue 2
Ellipticity dependence of optical harmonic generation in
journal, August 2006
- Zhang, G. P.; George, Thomas F.
- Physical Review A, Vol. 74, Issue 2
Cubic to hexagonal phase transition in CdTe polycrystalline thin films by oxygen incorporation
journal, January 1997
- Arizpe-Chávez, H.; Espinoza-Beltrán, F. J.; Ramírez-Bon, R.
- Solid State Communications, Vol. 101, Issue 1
Frequency dependence of scaling exponents of hyperpolarizability in polyenes: A density-matrix renormalization-group approach
journal, October 1999
- Zhang, G. P.
- Physical Review B, Vol. 60, Issue 16
Ab initio study of the cubic-to-hexagonal phase transition promoted by interstitial hydrogen in iron
journal, September 2011
- Castedo, A.; Sanchez, J.; Fullea, J.
- Physical Review B, Vol. 84, Issue 9
Higher-Order Harmonic Generation from Fullerene by Means of the Plasma Harmonic Method
journal, January 2009
- Ganeev, R. A.; Bom, L. B. Elouga; Abdul-Hadi, J.
- Physical Review Letters, Vol. 102, Issue 1
Structural aspects of the metal–insulator transition in BaVS3
journal, April 2005
- Fagot, S.; Foury, P.; Ravy, S.
- Physica B: Condensed Matter, Vol. 359-361