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Title: Removing Cs within a continuous flow set-up by an ionic exchanger material transformable into a final waste form

Abstract

Silica monoliths loaded with hexacyanoferrate (HCF) nanoparticles were designed and synthesized to selectively remove Cs + ions from an aqueous saline solution within a continuous flow set-up. The decontamination and hydrodynamic efficiency of this smart material was compared to other granularly supported HCF. Finally, a thermal treatment was applied to transform the HCF functionalized monolith into a final waste form matrix.

Authors:
 [1];  [1];  [2];  [3];  [4];  [5];  [6]; ORCiD logo [1]
  1. Univ. Montpellier, Bagnols‑sur‑Cèze, France). Lab. of Supercritical and Decontamination Processes
  2. PSL Univ., Fontainebleau (France). Centre de Géosciences; MINES Paris Tech, Paris (France)
  3. Brookhaven National Lab. (BNL), Upton, NY (United States). Nuclear Science and Technology Dept.
  4. Brookhaven National Lab. (BNL), Upton, NY (United States). Photon Division
  5. Univ. Montpellier, Bagnols‑sur‑Cèze, France). Lab. of Supercritical and Decontamination Processes, and Research Lab. for the Development of Conditioning Matrices
  6. Univ. Montpellier, Bagnols‑sur‑Cèze, France). Research Lab. for the Development of Conditioning Matrices
Publication Date:
Research Org.:
Brookhaven National Lab. (BNL), Upton, NY (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Nuclear Physics (NP) (SC-26)
OSTI Identifier:
1503230
Report Number(s):
BNL-211451-2019-JAAM
Journal ID: ISSN 0929-5607
Grant/Contract Number:  
SC0012704
Resource Type:
Accepted Manuscript
Journal Name:
Adsorption
Additional Journal Information:
Journal Volume: none; Journal Issue: none; Journal ID: ISSN 0929-5607
Publisher:
Springer Nature
Country of Publication:
United States
Language:
English
Subject:
73 NUCLEAR PHYSICS AND RADIATION PHYSICS; Ionic exchanger; Monoliths; Continuous flow; Cs decontamination; Densification

Citation Formats

Cabaud, Clément, Barré, Yves, De Windt, Laurent, Gill, Simerjeet, Dooryhée, Eric, Moloney, Mícheál P., Massoni, Nicolas, and Grandjean, Agnès. Removing Cs within a continuous flow set-up by an ionic exchanger material transformable into a final waste form. United States: N. p., 2019. Web. doi:10.1007/s10450-019-00040-6.
Cabaud, Clément, Barré, Yves, De Windt, Laurent, Gill, Simerjeet, Dooryhée, Eric, Moloney, Mícheál P., Massoni, Nicolas, & Grandjean, Agnès. Removing Cs within a continuous flow set-up by an ionic exchanger material transformable into a final waste form. United States. doi:10.1007/s10450-019-00040-6.
Cabaud, Clément, Barré, Yves, De Windt, Laurent, Gill, Simerjeet, Dooryhée, Eric, Moloney, Mícheál P., Massoni, Nicolas, and Grandjean, Agnès. Fri . "Removing Cs within a continuous flow set-up by an ionic exchanger material transformable into a final waste form". United States. doi:10.1007/s10450-019-00040-6.
@article{osti_1503230,
title = {Removing Cs within a continuous flow set-up by an ionic exchanger material transformable into a final waste form},
author = {Cabaud, Clément and Barré, Yves and De Windt, Laurent and Gill, Simerjeet and Dooryhée, Eric and Moloney, Mícheál P. and Massoni, Nicolas and Grandjean, Agnès},
abstractNote = {Silica monoliths loaded with hexacyanoferrate (HCF) nanoparticles were designed and synthesized to selectively remove Cs+ ions from an aqueous saline solution within a continuous flow set-up. The decontamination and hydrodynamic efficiency of this smart material was compared to other granularly supported HCF. Finally, a thermal treatment was applied to transform the HCF functionalized monolith into a final waste form matrix.},
doi = {10.1007/s10450-019-00040-6},
journal = {Adsorption},
number = none,
volume = none,
place = {United States},
year = {2019},
month = {3}
}

Journal Article:
Free Publicly Available Full Text
This content will become publicly available on March 1, 2020
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