Ice nucleating particles in the marine boundary layer in the Canadian Arctic during summer 2014
Abstract
Ice nucleating particles (INPs) in the Arctic can influence climateand precipitation in the region; yet our understanding of the concentrations and sourcesof INPs in this region remain uncertain. In the following, we (1) measured concentrationsof INPs in the immersion mode in the Canadian Arctic marine boundary layer duringsummer 2014 on board the CCGS Amundsen, (2) determined ratios of surface areasof mineral dust aerosol to sea spray aerosol, and (3) investigated the source region ofthe INPs using particle dispersion modelling. Average concentrations of INPs at -15,-20, and -25-C were 0.005, 0.044, and 0.154L-1,respectively. These concentrations fall within the range of INP concentrations measuredin other marine environments. For the samples investigated the ratio of mineral dustsurface area to sea spray surface area ranged from 0.03 to 0.09. Based on these ratiosand the ice active surface site densities of mineral dust and sea spray aerosoldetermined in previous laboratory studies, our results suggest that mineral dust is amore important contributor to the INP population than sea spray aerosol for the samplesanalysed. Based on particle dispersion modelling, the highest concentrations of INPs wereoften associated with lower-latitude source regions such as the Hudson Bay area, easternGreenland, or north-western continental Canada. On the other hand, the lowestconcentrations were often associated with regionsmore »
- Authors:
-
[2];
[3];
[1];
[2];
[2];
[7];
[1]
- Univ. of British Columbia, Vancouver, BC (Canada)
- Univ. of Toronto, ON (Canada)
- Pacific Northwest National Lab. (PNNL), Richland, WA (United States)
- Univ. Grenoble Alpes (France); Univ. Pierre et Marie Curie, Paris (France)
- Environment and Climate Change Canada, Toronto, ON (United States)
- Univ. of Quebec (Canada)
- Purdue Univ., West Lafayette, IN (United States)
- Publication Date:
- Research Org.:
- Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1501757
- Report Number(s):
- PNNL-SA-138062
Journal ID: ISSN 1680-7324
- Grant/Contract Number:
- AC05-76RL01830
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Atmospheric Chemistry and Physics (Online)
- Additional Journal Information:
- Journal Name: Atmospheric Chemistry and Physics (Online); Journal Volume: 19; Journal Issue: 2; Journal ID: ISSN 1680-7324
- Publisher:
- European Geosciences Union
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 54 ENVIRONMENTAL SCIENCES
Citation Formats
Irish, Victoria E., Hanna, Sarah J., Willis, Megan D., China, Swarup, Thomas, Jennie L., Wentzell, Jeremy J. B., Cirisan, Ana, Si, Meng, Leaitch, W. Richard, Murphy, Jennifer G., Abbatt, Jonathan P. D., Laskin, Alexander, Girard, Eric, and Bertram, Allan K. Ice nucleating particles in the marine boundary layer in the Canadian Arctic during summer 2014. United States: N. p., 2019.
Web. doi:10.5194/acp-19-1027-2019.
Irish, Victoria E., Hanna, Sarah J., Willis, Megan D., China, Swarup, Thomas, Jennie L., Wentzell, Jeremy J. B., Cirisan, Ana, Si, Meng, Leaitch, W. Richard, Murphy, Jennifer G., Abbatt, Jonathan P. D., Laskin, Alexander, Girard, Eric, & Bertram, Allan K. Ice nucleating particles in the marine boundary layer in the Canadian Arctic during summer 2014. United States. https://doi.org/10.5194/acp-19-1027-2019
Irish, Victoria E., Hanna, Sarah J., Willis, Megan D., China, Swarup, Thomas, Jennie L., Wentzell, Jeremy J. B., Cirisan, Ana, Si, Meng, Leaitch, W. Richard, Murphy, Jennifer G., Abbatt, Jonathan P. D., Laskin, Alexander, Girard, Eric, and Bertram, Allan K. Fri .
"Ice nucleating particles in the marine boundary layer in the Canadian Arctic during summer 2014". United States. https://doi.org/10.5194/acp-19-1027-2019. https://www.osti.gov/servlets/purl/1501757.
@article{osti_1501757,
title = {Ice nucleating particles in the marine boundary layer in the Canadian Arctic during summer 2014},
author = {Irish, Victoria E. and Hanna, Sarah J. and Willis, Megan D. and China, Swarup and Thomas, Jennie L. and Wentzell, Jeremy J. B. and Cirisan, Ana and Si, Meng and Leaitch, W. Richard and Murphy, Jennifer G. and Abbatt, Jonathan P. D. and Laskin, Alexander and Girard, Eric and Bertram, Allan K.},
abstractNote = {Ice nucleating particles (INPs) in the Arctic can influence climateand precipitation in the region; yet our understanding of the concentrations and sourcesof INPs in this region remain uncertain. In the following, we (1) measured concentrationsof INPs in the immersion mode in the Canadian Arctic marine boundary layer duringsummer 2014 on board the CCGS Amundsen, (2) determined ratios of surface areasof mineral dust aerosol to sea spray aerosol, and (3) investigated the source region ofthe INPs using particle dispersion modelling. Average concentrations of INPs at -15,-20, and -25-C were 0.005, 0.044, and 0.154L-1,respectively. These concentrations fall within the range of INP concentrations measuredin other marine environments. For the samples investigated the ratio of mineral dustsurface area to sea spray surface area ranged from 0.03 to 0.09. Based on these ratiosand the ice active surface site densities of mineral dust and sea spray aerosoldetermined in previous laboratory studies, our results suggest that mineral dust is amore important contributor to the INP population than sea spray aerosol for the samplesanalysed. Based on particle dispersion modelling, the highest concentrations of INPs wereoften associated with lower-latitude source regions such as the Hudson Bay area, easternGreenland, or north-western continental Canada. On the other hand, the lowestconcentrations were often associated with regions further north of the sampling sites andover Baffin Bay. A weak correlation was observed between INP concentrations and the timethe air mass spent over bare land, and a weak negative correlation was observed betweenINP concentrations and the time the air mass spent over ice and open water. Thesecombined results suggest that mineral dust from local sources is an important contributorto the INP population in the Canadian Arctic marine boundary layer during summer 2014.},
doi = {10.5194/acp-19-1027-2019},
journal = {Atmospheric Chemistry and Physics (Online)},
number = 2,
volume = 19,
place = {United States},
year = {Fri Jan 25 00:00:00 EST 2019},
month = {Fri Jan 25 00:00:00 EST 2019}
}
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Sea spray aerosol as a unique source of ice nucleating particles
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Dust and Biological Aerosols from the Sahara and Asia Influence Precipitation in the Western U.S.
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- Schnell, R. C.; Vali, G.
- Tellus, Vol. 27, Issue 3
Long-term trends of black carbon and sulphate aerosol in the Arctic: changes in atmospheric transport and source region emissions
journal, January 2010
- Hirdman, D.; Burkhart, J. F.; Sodemann, H.
- Atmospheric Chemistry and Physics, Vol. 10, Issue 19
Ice nucleation by fertile soil dusts: relative importance of mineral and biogenic components
journal, January 2014
- O'Sullivan, D.; Murray, B. J.; Malkin, T. L.
- Atmospheric Chemistry and Physics, Vol. 14, Issue 4
Ice-nucleating particles in Canadian Arctic sea-surface microlayer and bulk seawater
journal, January 2017
- Irish, Victoria E.; Elizondo, Pablo; Chen, Jessie
- Atmospheric Chemistry and Physics, Vol. 17, Issue 17
Effect of sea breeze circulation on aerosol mixing state and radiative properties in a desert setting
journal, January 2017
- Derimian, Yevgeny; Choël, Marie; Rudich, Yinon
- Atmospheric Chemistry and Physics, Vol. 17, Issue 18
Marine and terrestrial influences on ice nucleating particles during continuous springtime measurements in an Arctic oilfield location
journal, January 2018
- Creamean, Jessie M.; Kirpes, Rachel M.; Pratt, Kerri A.
- Atmospheric Chemistry and Physics, Vol. 18, Issue 24
Ice-nucleating particle concentrations unaffected by urban air pollution in Beijing, China
journal, January 2018
- Chen, Jie; Wu, Zhijun; Augustin-Bauditz, Stefanie
- Atmospheric Chemistry and Physics, Vol. 18, Issue 5
Ice nucleation activity of agricultural soil dust aerosols from Mongolia, Argentina, and Germany
text, January 2016
- Steinke, I.; Funk, R.; Busse, J.
- Karlsruhe
Heterogeneous ice nucleation on dust particles sourced from nine deserts worldwide - Part 1: Immersion freezing
text, January 2016
- Boose, Y.; Welti, A.; Atkinson, J.
- Karlsruhe
Heterogeneous ice nucleation on atmospheric aerosols: a review of results from laboratory experiments
text, January 2012
- Hoose, C.; Möhler, O.
- Karlsruhe
Works referencing / citing this record:
Bioaerosol field measurements: Challenges and perspectives in outdoor studies
journal, November 2019
- Šantl-Temkiv, Tina; Sikoparija, Branko; Maki, Teruya
- Aerosol Science and Technology, Vol. 54, Issue 5
Overview paper: New insights into aerosol and climate in the Arctic
journal, January 2019
- Abbatt, Jonathan P. D.; Leaitch, W. Richard; Aliabadi, Amir A.
- Atmospheric Chemistry and Physics, Vol. 19, Issue 4
Concentrations, composition, and sources of ice-nucleating particles in the Canadian High Arctic during spring 2016
journal, January 2019
- Si, Meng; Evoy, Erin; Yun, Jingwei
- Atmospheric Chemistry and Physics, Vol. 19, Issue 5
Annual variability of ice-nucleating particle concentrations at different Arctic locations
journal, January 2019
- Wex, Heike; Huang, Lin; Zhang, Wendy
- Atmospheric Chemistry and Physics, Vol. 19, Issue 7
Ice-nucleating particles in a coastal tropical site
journal, January 2019
- Ladino, Luis A.; Raga, Graciela B.; Alvarez-Ospina, Harry
- Atmospheric Chemistry and Physics, Vol. 19, Issue 9
Revisiting properties and concentrations of ice-nucleating particles in the sea surface microlayer and bulk seawater in the Canadian Arctic during summer
journal, January 2019
- Irish, Victoria E.; Hanna, Sarah J.; Xi, Yu
- Atmospheric Chemistry and Physics, Vol. 19, Issue 11
Characterization of aerosol particles at Cabo Verde close to sea level and at the cloud level – Part 2: Ice-nucleating particles in air, cloud and seawater
journal, January 2020
- Gong, Xianda; Wex, Heike; van Pinxteren, Manuela
- Atmospheric Chemistry and Physics, Vol. 20, Issue 3
Spatial and temporal variability in the ice-nucleating ability of alpine snowmelt and extension to frozen cloud fraction
journal, January 2020
- Brennan, Killian P.; David, Robert O.; Borduas-Dedekind, Nadine
- Atmospheric Chemistry and Physics, Vol. 20, Issue 1