The Role of Secondary Ice Processes in Midlatitude Continental Clouds

Zipori, Assaf; Reicher, Naama; Erel, Yigal; Rosenfeld, Daniel; Sandler, Amir; Knopf, Daniel A.; Rudich, Yinon

doi:10.1029/2018JD029146

Title: The Role of Secondary Ice Processes in Midlatitude Continental Clouds

Journal Article · 08 October 2018 · Journal of Geophysical Research: Atmospheres

DOI: https://doi.org/10.1029/2018JD029146 · OSTI ID:1500174

Zipori, Assaf ^[1];

^[2]; Erel, Yigal ^[3];

^[3]; Sandler, Amir ^[4];

^[5];

^[2]

Weizmann Inst. of Science, Rehovot (Israel); Hebrew Univ. of Jerusalem (Israel); Stony Brook University
Weizmann Inst. of Science, Rehovot (Israel)
Hebrew Univ. of Jerusalem (Israel)
Geological Survey of Israel, Jerusalem (Israel)
Stony Brook Univ., NY (United States)

Clouds contribute very large uncertainties to our understanding of Earth's climate system. This is partly attributed to the insufficient predictive abilities of ice formation processes in clouds and the ramifications for the hydrological cycle and climate. To improve predictions of ice particle concentrations in clouds, a better understanding of the relative contributions of ice nucleating particles and secondary ice processes (SIPs) is needed. To address this challenging question, we combine ice nucleation measurements via immersion freezing of particles filtered from rainwater, with satellite-retrieved cloud top glaciation temperatures of the same clouds, while considering the chemical composition of the rainwater, the particles, and the particles' mass loads. In addition, laboratory-derived ice nucleation parameterization of K-feldspar was implemented in an ice nucleation model in order to reconstruct cloud glaciation temperatures considering primary ice nucleation only. Our laboratory and modeling results suggest that SIPs play a major role in glaciating the investigated clouds system. Furthermore, we show that SIP is controlled by cloud droplet sizes. In summary, our results suggest that the effect of SIP on cloud glaciation temperatures and therefore on Earth's radiation budget, may be significant.

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Research Organization:: Stony Brook Univ., NY (United States)

Sponsoring Organization:: USDOE; USDOE Office of Science (SC), Biological and Environmental Research (BER) (SC-23). Climate and Environmental Sciences Division

Grant/Contract Number:: SC0016370

OSTI ID:: 1500174

Journal Information:: Journal of Geophysical Research: Atmospheres, Journal Name: Journal of Geophysical Research: Atmospheres Journal Issue: 22 Vol. 123; ISSN 2169-897X

Publisher:: American Geophysical UnionCopyright Statement

Country of Publication:: United States

Language:: English

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Ice nucleation by fertile soil dusts: relative importance of mineral and biogenic components O'Sullivan, D.; Murray, B. J.; Malkin, T. L. Atmospheric Chemistry and Physics, Vol. 14, Issue 4 https://doi.org/10.5194/acp-14-1853-2014	journal	January 2014
High ice water content at low radar reflectivity near deep convection – Part 2: Evaluation of microphysical pathways in updraft parcel simulations Ackerman, A. S.; Fridlind, A. M.; Grandin, A. Atmospheric Chemistry and Physics, Vol. 15, Issue 20 https://doi.org/10.5194/acp-15-11729-2015	journal	January 2015
A comparative study of K-rich and Na/Ca-rich feldspar ice-nucleating particles in a nanoliter droplet freezing assay Peckhaus, Andreas; Kiselev, Alexei; Hiron, Thibault Atmospheric Chemistry and Physics, Vol. 16, Issue 18 https://doi.org/10.5194/acp-16-11477-2016	journal	January 2016
Effects of mineral dust on global atmospheric nitrate concentrations Karydis, V. A.; Tsimpidi, A. P.; Pozzer, A. Atmospheric Chemistry and Physics, Vol. 16, Issue 3 https://doi.org/10.5194/acp-16-1491-2016	journal	January 2016
Analysis of isothermal and cooling-rate-dependent immersion freezing by a unifying stochastic ice nucleation model Alpert, Peter A.; Knopf, Daniel A. Atmospheric Chemistry and Physics, Vol. 16, Issue 4 https://doi.org/10.5194/acp-16-2083-2016	journal	January 2016
Comparing model and measured ice crystal concentrations in orographic clouds during the INUPIAQ campaign Farrington, Robert J.; Connolly, Paul J.; Lloyd, Gary Atmospheric Chemistry and Physics, Vol. 16, Issue 8 https://doi.org/10.5194/acp-16-4945-2016	journal	January 2016
Observations of cloud microphysics and ice formation during COPE Taylor, J. W.; Choularton, T. W.; Blyth, A. M. Atmospheric Chemistry and Physics, Vol. 16, Issue 2 https://doi.org/10.5194/acp-16-799-2016	journal	January 2016
Comparing contact and immersion freezing from continuous flow diffusion chambers Nagare, Baban; Marcolli, Claudia; Welti, André Atmospheric Chemistry and Physics, Vol. 16, Issue 14 https://doi.org/10.5194/acp-16-8899-2016	journal	January 2016
Partitioning the primary ice formation modes in large eddy simulations of mixed-phase clouds Hande, Luke B.; Hoose, Corinna Atmospheric Chemistry and Physics, Vol. 17, Issue 22 https://doi.org/10.5194/acp-17-14105-2017	journal	January 2017
Further evidence for CCN aerosol concentrations determining the height of warm rain and ice initiation in convective clouds over the Amazon basin Braga, Ramon Campos; Rosenfeld, Daniel; Weigel, Ralf Atmospheric Chemistry and Physics, Vol. 17, Issue 23 https://doi.org/10.5194/acp-17-14433-2017	journal	January 2017
Contribution of feldspar and marine organic aerosols to global ice nucleating particle concentrations Vergara-Temprado, Jesús; Murray, Benjamin J.; Wilson, Theodore W. Atmospheric Chemistry and Physics, Vol. 17, Issue 5 https://doi.org/10.5194/acp-17-3637-2017	journal	January 2017
Initiation of secondary ice production in clouds Sullivan, Sylvia C.; Hoose, Corinna; Kiselev, Alexei Atmospheric Chemistry and Physics, Vol. 18, Issue 3 https://doi.org/10.5194/acp-18-1593-2018	journal	January 2018
Global indirect aerosol effects: a review Lohmann, U.; Feichter, J. Atmospheric Chemistry and Physics, Vol. 5, Issue 3 https://doi.org/10.5194/acp-5-715-2005	journal	January 2005
Cloud microphysics and aerosol indirect effects in the global climate model ECHAM5-HAM Lohmann, U.; Stier, P.; Hoose, C. Atmospheric Chemistry and Physics, Vol. 7, Issue 13 https://doi.org/10.5194/acp-7-3425-2007	journal	January 2007
Efficiency of immersion mode ice nucleation on surrogates of mineral dust Marcolli, C.; Gedamke, S.; Peter, T. Atmospheric Chemistry and Physics, Vol. 7, Issue 19 https://doi.org/10.5194/acp-7-5081-2007	journal	January 2007
Clouds-Aerosols-Precipitation Satellite Analysis Tool (CAPSAT) Lensky, I. M.; Rosenfeld, D. Atmospheric Chemistry and Physics, Vol. 8, Issue 22 https://doi.org/10.5194/acp-8-6739-2008	journal	January 2008
On the importance of small ice crystals in tropical anvil cirrus Jensen, E. J.; Lawson, P.; Baker, B. Atmospheric Chemistry and Physics, Vol. 9, Issue 15 https://doi.org/10.5194/acp-9-5519-2009	journal	January 2009
Sensitivity studies of different aerosol indirect effects in mixed-phase clouds Lohmann, U.; Hoose, C. Atmospheric Chemistry and Physics, Vol. 9, Issue 22 https://doi.org/10.5194/acp-9-8917-2009	journal	January 2009
Heterogeneous ice nucleation on atmospheric aerosols: a review of results from laboratory experiments Hoose, C.; Möhler, O. Atmospheric Chemistry and Physics Discussions, Vol. 12, Issue 5 https://doi.org/10.5194/acpd-12-12531-2012	journal	January 2012
Effects of mineral dust on global atmospheric nitrate concentrations Karydis, V. A.; Tsimpidi, A. P.; Pozzer, A. Atmospheric Chemistry and Physics Discussions, Vol. 15, Issue 8 https://doi.org/10.5194/acpd-15-11525-2015	journal	January 2015
Global indirect aerosol effects: a review Lohmann, U.; Feichter, J. Atmospheric Chemistry and Physics Discussions, Vol. 4, Issue 6 https://doi.org/10.5194/acpd-4-7561-2004	journal	January 2004
Cloud microphysics and aerosol indirect effects in the global climate model ECHAM5-HAM Lohmann, U.; Stier, P.; Hoose, C. Atmospheric Chemistry and Physics Discussions, Vol. 7, Issue 2 https://doi.org/10.5194/acpd-7-3719-2007	journal	January 2007
Clouds-Aerosols-Precipitation Satellite Analysis Tool (CAPSAT) Lensky, I. M.; Rosenfeld, D. Atmospheric Chemistry and Physics Discussions, Vol. 8, Issue 2 https://doi.org/10.5194/acpd-8-4765-2008	journal	January 2008
The WeIzmann Supercooled Droplets Observation on a Microarray (WISDOM) and application for ambient dust Reicher, Naama; Segev, Lior; Rudich, Yinon Atmospheric Measurement Techniques, Vol. 11, Issue 1 https://doi.org/10.5194/amt-11-233-2018	journal	January 2018
Experimental quantification of contact freezing in an electrodynamic balance Hoffmann, N.; Kiselev, A.; Rzesanke, D. Atmospheric Measurement Techniques, Vol. 6, Issue 9 https://doi.org/10.5194/amt-6-2373-2013	journal	January 2013
Experimental quantification of contact freezing in an electrodynamic balance Hoffmann, N.; Kiselev, A.; Rzesanke, D. Karlsruhe https://doi.org/10.5445/ir/1000038393	text	January 2013
Heterogeneous ice nucleation on atmospheric aerosols: a review of results from laboratory experiments Hoose, Corinna; Möhler, Ottmar Karlsruhe https://doi.org/10.5445/ir/1000038466	text	January 2012
Ice nuclei in marine air: Biogenic particles or dust? Burrows, S. M.; Hoose, C.; Pöschl, U. Karlsruhe https://doi.org/10.5445/ir/1000041600	text	January 2013
Initiation of secondary ice production in clouds Sullivan, Sylvia C.; Hoose, Corinna; Kiselev, Alexei Karlsruhe https://doi.org/10.5445/ir/1000080418	text	January 2018
Heterogeneous ice nucleation on atmospheric aerosols: a review of results from laboratory experiments Hoose, C.; Möhler, O. Karlsruhe https://doi.org/10.5445/ir/110089633	text	January 2012

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Cloud history can change water–ice–surface interactions of oxide mineral aerosols: a case study on silica Abdelmonem, Ahmed; Ratnayake, Sanduni; Toner, Jonathan D. Atmospheric Chemistry and Physics, Vol. 20, Issue 2 https://doi.org/10.5194/acp-20-1075-2020	journal	January 2020
Spatial and temporal variability in the ice-nucleating ability of alpine snowmelt and extension to frozen cloud fraction Brennan, Killian P.; David, Robert O.; Borduas-Dedekind, Nadine Atmospheric Chemistry and Physics, Vol. 20, Issue 1 https://doi.org/10.5194/acp-20-163-2020	journal	January 2020

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