Improved high temperature radiation damage tolerance in a three-phase ceramic with heterointerfaces
Abstract
Abstract Radiation damage tolerance for a variety of ceramics at high temperatures depends on the material’s resistance to nucleation and growth of extended defects. Such processes are prevalent in ceramics employed for space, nuclear fission/fusion and nuclear waste environments. This report shows that random heterointerfaces in materials with sub-micron grains can act as highly efficient sinks for point defects compared to grain boundaries in single-phase materials. The concentration of dislocation loops in a radiation damage-prone phase (Al 2 O 3 ) is significantly reduced when Al 2 O 3 is a component of a composite system as opposed to a single-phase system. These results present a novel method for designing exceptionally radiation damage tolerant ceramics at high temperatures with a stable grain size, without requiring extensive interfacial engineering or production of nanocrystalline materials.
- Publication Date:
- Research Org.:
- Univ. of California, Irvine, CA (United States)
- Sponsoring Org.:
- USDOE Office of Nuclear Energy (NE); National Science Foundation (NSF)
- OSTI Identifier:
- 1469740
- Alternate Identifier(s):
- OSTI ID: 1499998
- Grant/Contract Number:
- NE0000711; DMR 1611457
- Resource Type:
- Published Article
- Journal Name:
- Scientific Reports
- Additional Journal Information:
- Journal Name: Scientific Reports Journal Volume: 8 Journal Issue: 1; Journal ID: ISSN 2045-2322
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United Kingdom
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; ceramics; composites
Citation Formats
Ohtaki, Kenta K., Patel, Maulik K., Crespillo, Miguel L., Karandikar, Keyur K., Zhang, Yanwen, Graeve, Olivia A., and Mecartney, Martha L. Improved high temperature radiation damage tolerance in a three-phase ceramic with heterointerfaces. United Kingdom: N. p., 2018.
Web. doi:10.1038/s41598-018-31721-x.
Ohtaki, Kenta K., Patel, Maulik K., Crespillo, Miguel L., Karandikar, Keyur K., Zhang, Yanwen, Graeve, Olivia A., & Mecartney, Martha L. Improved high temperature radiation damage tolerance in a three-phase ceramic with heterointerfaces. United Kingdom. https://doi.org/10.1038/s41598-018-31721-x
Ohtaki, Kenta K., Patel, Maulik K., Crespillo, Miguel L., Karandikar, Keyur K., Zhang, Yanwen, Graeve, Olivia A., and Mecartney, Martha L. Tue .
"Improved high temperature radiation damage tolerance in a three-phase ceramic with heterointerfaces". United Kingdom. https://doi.org/10.1038/s41598-018-31721-x.
@article{osti_1469740,
title = {Improved high temperature radiation damage tolerance in a three-phase ceramic with heterointerfaces},
author = {Ohtaki, Kenta K. and Patel, Maulik K. and Crespillo, Miguel L. and Karandikar, Keyur K. and Zhang, Yanwen and Graeve, Olivia A. and Mecartney, Martha L.},
abstractNote = {Abstract Radiation damage tolerance for a variety of ceramics at high temperatures depends on the material’s resistance to nucleation and growth of extended defects. Such processes are prevalent in ceramics employed for space, nuclear fission/fusion and nuclear waste environments. This report shows that random heterointerfaces in materials with sub-micron grains can act as highly efficient sinks for point defects compared to grain boundaries in single-phase materials. The concentration of dislocation loops in a radiation damage-prone phase (Al 2 O 3 ) is significantly reduced when Al 2 O 3 is a component of a composite system as opposed to a single-phase system. These results present a novel method for designing exceptionally radiation damage tolerant ceramics at high temperatures with a stable grain size, without requiring extensive interfacial engineering or production of nanocrystalline materials.},
doi = {10.1038/s41598-018-31721-x},
journal = {Scientific Reports},
number = 1,
volume = 8,
place = {United Kingdom},
year = {Tue Sep 18 00:00:00 EDT 2018},
month = {Tue Sep 18 00:00:00 EDT 2018}
}
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https://doi.org/10.1038/s41598-018-31721-x
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Cited by: 11 works
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Figures / Tables:
Figure 1: Cross section TEM bright field images of irradiated single crystals of YSZ, MgAl2O4 and Al2O3 from top surface to irradiated interior with Stopping and Range of Ions in Matter (SRIM) calculation29. SRIM calculations predict that the damage peak lies at ~1.6 μm from the irradiated surface and themore »
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Works referenced in this record:
Oxygen ion diffusivity in strained yttria stabilized zirconia: where is the fastest strain?
journal, January 2010
- Kushima, Akihiro; Yildiz, Bilge
- Journal of Materials Chemistry, Vol. 20, Issue 23
Radiation damage in nanostructured materials
journal, July 2018
- Zhang, Xinghang; Hattar, Khalid; Chen, Youxing
- Progress in Materials Science, Vol. 96
Effect of grain boundary character on sink efficiency
journal, October 2012
- Han, W. Z.; Demkowicz, M. J.; Fu, E. G.
- Acta Materialia, Vol. 60, Issue 18
Design of Radiation Tolerant Materials Via Interface Engineering
journal, September 2013
- Han, Weizhong; Demkowicz, Michael J.; Mara, Nathan A.
- Advanced Materials, Vol. 25, Issue 48
New ion beam materials laboratory for materials modification and irradiation effects research
journal, November 2014
- Zhang, Y.; Crespillo, M. L.; Xue, H.
- Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 338
Defect production in ceramics
journal, November 1997
- Zinkle, S. J.; Kinoshita, C.
- Journal of Nuclear Materials, Vol. 251
10MeV Au ion irradiation effects in an MgO–HfO2 ceramic–ceramic (CERCER) composite
journal, August 2009
- Valdez, J. A.; Usov, I. O.; Won, J.
- Journal of Nuclear Materials, Vol. 393, Issue 1
Enhanced radiation tolerance in nanocrystalline MgGa2O4
journal, June 2007
- Shen, Tong D.; Feng, Shihai; Tang, Ming
- Applied Physics Letters, Vol. 90, Issue 26
Radiation endurance in Al2O3 nanoceramics
journal, September 2016
- García Ferré, F.; Mairov, A.; Ceseracciu, L.
- Scientific Reports, Vol. 6, Issue 1
Defect-interface interactions
journal, October 2015
- Beyerlein, I. J.; Demkowicz, M. J.; Misra, A.
- Progress in Materials Science, Vol. 74
Achieving Radiation Tolerance through Non-Equilibrium Grain Boundary Structures
journal, September 2017
- Vetterick, Gregory A.; Gruber, Jacob; Suri, Pranav K.
- Scientific Reports, Vol. 7, Issue 1
Amorphous intergranular films act as ultra-efficient point defect sinks during collision cascades
journal, January 2016
- Ludy, Joseph E.; Rupert, Timothy J.
- Scripta Materialia, Vol. 110
The radiation damage tolerance of ultra-high strength nanolayered composites
journal, September 2007
- Misra, A.; Demkowicz, M. J.; Zhang, X.
- JOM, Vol. 59, Issue 9
Strained Ionic Interfaces: Effect on Oxygen Diffusivity from Atomistic Simulations
journal, February 2014
- Aidhy, Dilpuneet S.; Zhang, Yanwen; Weber, William J.
- The Journal of Physical Chemistry C, Vol. 118, Issue 8
Threshold displacement energy in yttria-stabilized zirconia
journal, March 2007
- Costantini, Jean-Marc; Beuneu, François
- physica status solidi (c), Vol. 4, Issue 3
Radiation effects in ceramics
journal, October 1994
- Hobbs, Linn W.; Clinard, Frank W.; Zinkle, Steven J.
- Journal of Nuclear Materials, Vol. 216
Effects of neutron irradiation of Ti3SiC2 and Ti3AlC2 in the 121–1085 °C temperature range
journal, February 2017
- Tallman, Darin J.; He, Lingfeng; Gan, Jian
- Journal of Nuclear Materials, Vol. 484
Interface Structure and Radiation Damage Resistance in Cu-Nb Multilayer Nanocomposites
journal, April 2008
- Demkowicz, M. J.; Hoagland, R. G.; Hirth, J. P.
- Physical Review Letters, Vol. 100, Issue 13
Grain growth and phase stability of nanocrystalline cubic zirconia under ion irradiation
journal, November 2010
- Zhang, Yanwen; Jiang, Weilin; Wang, Chongmin
- Physical Review B, Vol. 82, Issue 18
Why is magnesia spinel a radiation-resistant material?
journal, March 1995
- Kinoshita, C.; Fukumoto, K.; Fukuda, K.
- Journal of Nuclear Materials, Vol. 219
Synthesis and Consolidation of BaAl 2 Si 2 O 8 :Eu: Development of an Integrated Process for Luminescent Smart Ceramic Materials
journal, November 2009
- Sinha, Kaustav; Pearson, Brett; Casolco, Said R.
- Journal of the American Ceramic Society, Vol. 92, Issue 11
SRIM – The stopping and range of ions in matter (2010)
journal, June 2010
- Ziegler, James F.; Ziegler, M. D.; Biersack, J. P.
- Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 268, Issue 11-12
Microstructural defects in SiC neutron irradiated at very high temperatures
journal, December 2008
- Kondo, S.; Katoh, Y.; Snead, L. L.
- Journal of Nuclear Materials, Vol. 382, Issue 2-3
On the use of SRIM for computing radiation damage exposure
journal, September 2013
- Stoller, R. E.; Toloczko, M. B.; Was, G. S.
- Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 310
Design of α-Al 2 O 3 /Cr 2 O 3 nano-multilayered composite films with enhanced irradiation tolerance prepared by epitaxial growth at low temperature
journal, September 2017
- Zou, Jianxiong; Dong, Yuming; Liu, Bo
- Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 406
Effect of irradiation spectrum on the microstructural evolution in ceramic insulators
journal, March 1995
- Zinkle, S. J.
- Journal of Nuclear Materials, Vol. 219
Radiation Tolerance of Nanocrystalline Ceramics: Insights from Yttria Stabilized Zirconia
journal, January 2015
- Dey, Sanchita; Drazin, John W.; Wang, Yongqiang
- Scientific Reports, Vol. 5, Issue 1
Radiation damage tolerant nanomaterials
journal, November 2013
- Beyerlein, I. J.; Caro, A.; Demkowicz, M. J.
- Materials Today, Vol. 16, Issue 11
Enhanced radiation tolerance of YSZ/Al2O3 multilayered nanofilms with pre-existing nanovoids
journal, February 2018
- Wang, Hui; Ren, Feng; Tang, Jun
- Acta Materialia, Vol. 144
Microstructure of Al2O3 and MgAl2O4 irradiated at low temperatures
journal, March 1998
- Zinkle, S. J.; Pells, G. P.
- Journal of Nuclear Materials, Vol. 253, Issue 1-3
A high-strain-rate superplastic ceramic
journal, September 2001
- Kim, B. -N.; Hiraga, K.; Morita, K.
- Nature, Vol. 413, Issue 6853
Figures / Tables found in this record:
Figures/Tables have been extracted from DOE-funded journal article accepted manuscripts.