Lead halide perovskites: Crystal-liquid duality, phonon glass electron crystals, and large polaron formation
Abstract
Lead halide perovskites have been demonstrated as high performance materials in solar cells and light-emitting devices. These materials are characterized by coherent band transport expected from crystalline semiconductors, but dielectric responses and phonon dynamics typical of liquids. This “crystal-liquid” duality implies that lead halide perovskites belong to phonon glass electron crystals, a class of materials believed to make the most efficient thermoelectrics. We show that the crystal-liquid duality and the resulting dielectric response are responsible for large polaron formation and screening of charge carriers, leading to defect tolerance, moderate charge carrier mobility, and radiative recombination properties. Large polaron formation, along with the phonon glass character, may also explain the marked reduction in hot carrier cooling rates in these materials.
- Publication Date:
- Research Org.:
- Columbia Univ., New York, NY (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1499930
- Grant/Contract Number:
- SC0010692
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Science Advances
- Additional Journal Information:
- Journal Volume: 3; Journal Issue: 10; Journal ID: ISSN 2375-2548
- Publisher:
- AAAS
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; 14 SOLAR ENERGY
Citation Formats
Miyata, Kiyoshi, Atallah, Timothy L., and Zhu, X. -Y.. Lead halide perovskites: Crystal-liquid duality, phonon glass electron crystals, and large polaron formation. United States: N. p., 2017.
Web. doi:10.1126/sciadv.1701469.
Miyata, Kiyoshi, Atallah, Timothy L., & Zhu, X. -Y.. Lead halide perovskites: Crystal-liquid duality, phonon glass electron crystals, and large polaron formation. United States. https://doi.org/10.1126/sciadv.1701469
Miyata, Kiyoshi, Atallah, Timothy L., and Zhu, X. -Y.. Fri .
"Lead halide perovskites: Crystal-liquid duality, phonon glass electron crystals, and large polaron formation". United States. https://doi.org/10.1126/sciadv.1701469. https://www.osti.gov/servlets/purl/1499930.
@article{osti_1499930,
title = {Lead halide perovskites: Crystal-liquid duality, phonon glass electron crystals, and large polaron formation},
author = {Miyata, Kiyoshi and Atallah, Timothy L. and Zhu, X. -Y.},
abstractNote = {Lead halide perovskites have been demonstrated as high performance materials in solar cells and light-emitting devices. These materials are characterized by coherent band transport expected from crystalline semiconductors, but dielectric responses and phonon dynamics typical of liquids. This “crystal-liquid” duality implies that lead halide perovskites belong to phonon glass electron crystals, a class of materials believed to make the most efficient thermoelectrics. We show that the crystal-liquid duality and the resulting dielectric response are responsible for large polaron formation and screening of charge carriers, leading to defect tolerance, moderate charge carrier mobility, and radiative recombination properties. Large polaron formation, along with the phonon glass character, may also explain the marked reduction in hot carrier cooling rates in these materials.},
doi = {10.1126/sciadv.1701469},
journal = {Science Advances},
number = 10,
volume = 3,
place = {United States},
year = {2017},
month = {10}
}
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Figures / Tables:
Fig. 1: Structure of CH3NH3PbX3 perovskite. It consists of a framework of corner-sharing lead (gray) halide (purple) octahedrals and the CH3NH3⁺ cation (black, blue, and white) in the nanocage.
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- Alberti, Alessandra; Bongiorno, Corrado; Smecca, Emanuele
- Nature Communications, Vol. 10, Issue 1
Enhancing ferroelectric photovoltaic effect by polar order engineering
journal, July 2018
- You, Lu; Zheng, Fan; Fang, Liang
- Science Advances, Vol. 4, Issue 7
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