Breakdown of magnons in a strongly spin-orbital coupled magnet
Abstract
The description of quantized collective excitations stands as a landmark in the quantum theory of condensed matter. A prominent example occurs in conventional magnets, which support bosonic magnons - quantized harmonic fluctuations of the ordered spins. In striking contrast is the recent discovery that strongly spin-orbital coupled magnets, such as α-RuCl3, may display a broad excitation continuum inconsistent with conventional magnons. Due to incomplete knowledge of the underlying interactions unraveling the nature of this continuum remains challenging. The most discussed explanation refers to a coherent continuum of fractional excitations analogous to the celebrated Kitaev spin liquid. Here we present a more general scenario. We propose that the observed continuum represents incoherent excitations originating from strong magnetic anharmoniticity that naturally occurs in such materials. This scenario fully explains the observed inelastic magnetic response of α-RuCl3 and reveals the presence of nontrivial excitations in such materials extending well beyond the Kitaev state.
- Authors:
-
[1];
[3];
- Goethe-Universität Frankfurt (Germany)
- Univ. of California, Irvine, CA (United States)
- Université de Cergy-Pontoise (France)
- Publication Date:
- Research Org.:
- Univ. of California, Irvine, CA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1499928
- Alternate Identifier(s):
- OSTI ID: 1784335
- Grant/Contract Number:
- FG02-04ER46174
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Communications
- Additional Journal Information:
- Journal Volume: 8; Journal Issue: 1; Journal ID: ISSN 2041-1723
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY
Citation Formats
Winter, Stephen M., Riedl, Kira, Maksimov, Pavel A., Chernyshev, Alexander L., Honecker, Andreas, and Valentí, Roser. Breakdown of magnons in a strongly spin-orbital coupled magnet. United States: N. p., 2017.
Web. doi:10.1038/s41467-017-01177-0.
Winter, Stephen M., Riedl, Kira, Maksimov, Pavel A., Chernyshev, Alexander L., Honecker, Andreas, & Valentí, Roser. Breakdown of magnons in a strongly spin-orbital coupled magnet. United States. https://doi.org/10.1038/s41467-017-01177-0
Winter, Stephen M., Riedl, Kira, Maksimov, Pavel A., Chernyshev, Alexander L., Honecker, Andreas, and Valentí, Roser. Fri .
"Breakdown of magnons in a strongly spin-orbital coupled magnet". United States. https://doi.org/10.1038/s41467-017-01177-0. https://www.osti.gov/servlets/purl/1499928.
@article{osti_1499928,
title = {Breakdown of magnons in a strongly spin-orbital coupled magnet},
author = {Winter, Stephen M. and Riedl, Kira and Maksimov, Pavel A. and Chernyshev, Alexander L. and Honecker, Andreas and Valentí, Roser},
abstractNote = {The description of quantized collective excitations stands as a landmark in the quantum theory of condensed matter. A prominent example occurs in conventional magnets, which support bosonic magnons - quantized harmonic fluctuations of the ordered spins. In striking contrast is the recent discovery that strongly spin-orbital coupled magnets, such as α-RuCl3, may display a broad excitation continuum inconsistent with conventional magnons. Due to incomplete knowledge of the underlying interactions unraveling the nature of this continuum remains challenging. The most discussed explanation refers to a coherent continuum of fractional excitations analogous to the celebrated Kitaev spin liquid. Here we present a more general scenario. We propose that the observed continuum represents incoherent excitations originating from strong magnetic anharmoniticity that naturally occurs in such materials. This scenario fully explains the observed inelastic magnetic response of α-RuCl3 and reveals the presence of nontrivial excitations in such materials extending well beyond the Kitaev state.},
doi = {10.1038/s41467-017-01177-0},
journal = {Nature Communications},
number = 1,
volume = 8,
place = {United States},
year = {2017},
month = {10}
}
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Figures / Tables:
Fig. 1 : From material to model. Within the honeycomb ab-layer of $α$-RuCl3 are illustrated the RuCl6 octahedra, magnetic zigzag ordering pattern, and definition of the underlying magnetic interactions. Crystal axes are labeled with respect to the C2/m structure
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