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Title: Experimental realization of two-dimensional Dirac nodal line fermions in monolayer Cu2Si

Journal Article · · Nature Communications

Topological nodal line semimetals, a novel quantum state of materials, possess topologically nontrivial valence and conduction bands that touch at a line near the Fermi level. The exotic band structure can lead to various novel properties, such as long-range Coulomb interaction and flat Landau levels. Recently, topological nodal lines have been observed in several bulk materials, such as PtSn4, ZrSiS, TlTaSe2 and PbTaSe2. However, in two-dimensional materials, experimental research on nodal line fermions is still lacking. Here, we report the discovery of two-dimensional Dirac nodal line fermions in monolayer Cu2Si based on combined theoretical calculations and angle-resolved photoemission spectroscopy measurements. The Dirac nodal lines in Cu2Si form two concentric loops centred around the Γ point and are protected by mirror reflection symmetry. In conclusion, our results establish Cu2Si as a platform to study the novel physical properties in two-dimensional Dirac materials and provide opportunities to realize high-speed low-dissipation devices.

Research Organization:
Univ. of Illinois, Chicago, IL (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division
Grant/Contract Number:
FG02-07ER46383
OSTI ID:
1499693
Journal Information:
Nature Communications, Vol. 8, Issue 1; ISSN 2041-1723
Publisher:
Nature Publishing GroupCopyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 209 works
Citation information provided by
Web of Science

References (25)

Topological nodal semimetals journal December 2011
Generalized Gradient Approximation Made Simple journal October 1996
Topological insulators and superconductors journal October 2011
Atomic structure of the Cu/Si(111) interface by high-energy core-level Auger electron diffraction journal July 1985
A NIXSW structural investigation of the (√3×√3)R30°-Cu2Si surface alloy phase formed by SiH4 reaction with Cu(111) journal September 2001
Graphene-Like Two-Dimensional Materials journal January 2013
Drumhead surface states and topological nodal-line fermions in TlTaSe 2 journal March 2016
Two-Dimensional Cu 2 Si Monolayer with Planar Hexacoordinate Copper and Silicon Bonding journal February 2015
Topological nodal-line fermions in spin-orbit metal PbTaSe2 journal February 2016
Dirac node arcs in PtSn4 journal April 2016
Methylsilane on Cu(111), a STM study of the R30°-Cu2Si surface silicide journal July 2005
Interaction of silane with Cu(111): Surface alloy and molecular chemisorbed phases journal April 1997
Dirac cone protected by non-symmorphic symmetry and three-dimensional Dirac line node in ZrSiS journal May 2016
Colloquium: Topological insulators journal November 2010
Observation of topological nodal fermion semimetal phase in ZrSiS journal May 2016
A simple tight-binding model of spin–orbit splitting of sp-derived surface states journal July 2000
Efficient iterative schemes for ab initio total-energy calculations using a plane-wave basis set journal October 1996
Discovery of a Three-Dimensional Topological Dirac Semimetal, Na3Bi journal January 2014
Microscopic structure, discommensurations, and tiling of Si(111)/Cu-‘‘5×5’’ journal July 1992
Two- and One-Dimensional Honeycomb Structures of Silicon and Germanium journal June 2009
The prediction of a family group of two-dimensional node-line semimetals journal January 2017
Deduction of a three-phase model for the (√3×√3)R30°-Cu2Si/Cu(111) surface alloy journal November 2009
Discovery of a Weyl fermion semimetal and topological Fermi arcs journal July 2015
Discovery of a Three-dimensional Topological Dirac Semimetal, Na3Bi text January 2013
Discovery of a Weyl Fermion Semimetal and Topological Fermi Arcs text January 2015

Cited By (35)

Epitaxial Growth of Honeycomb Monolayer CuSe with Dirac Nodal Line Fermions journal March 2018
Large‐Spin‐Gap Nodal‐Line Half‐Metal and High‐Temperature Ferromagnetic Semiconductor in Cr 2 X 3 (X=O,S,Se) Monolayers journal October 2019
Computational Prediction of the Low‐Temperature Ferromagnetic Semiconducting 2D SiN Monolayer journal September 2019
Low‐Energy GeP Monolayers with Natural Type‐II Homojunctions for SunLight‐Driven Water Splitting journal May 2019
Topological quantum catalyst: Dirac nodal line states and a potential electrocatalyst of hydrogen evolution in the TiSi family journal December 2017
Mixed topological semimetals driven by orbital complexity in two-dimensional ferromagnets journal July 2019
A two-dimensional CaSi monolayer with quasi-planar pentacoordinate silicon journal January 2018
Coexistence of open and closed type nodal line topological semimetals in two dimensional B 2 C journal January 2018
Discovery of a novel spin-polarized nodal ring in a two-dimensional HK lattice journal January 2018
Two-dimensional honeycomb borophene oxide: strong anisotropy and nodal loop transformation journal January 2019
Hydrogenated derivatives of hexacoordinated metallic Cu 2 Si monolayer journal January 2018
Discovery of cobweb-like MoC 6 and its application for nitrogen fixation journal January 2018
Predicting multiple Dirac-cones and ultrahigh Fermi velocity in perovskite Rc phase LaCuO 3 journal January 2018
Hexagonal M 2 C 3 (M = As, Sb, and Bi) monolayers: new functional materials with desirable band gaps and ultrahigh carrier mobility journal January 2018
Bipolar magnetism in a two-dimensional NbS 2 semiconductor with high Curie temperature journal January 2018
Perfect planar tetra-coordinated MC 6 monolayer: superior anode material for Li-ion battery journal January 2019
TMC (TM = Co, Ni, and Cu) monolayers with planar pentacoordinate carbon and their potential applications journal January 2019
Superconductivity in predicted two dimensional XB 6 (X = Ga, In) journal January 2020
Barrier tunneling of the loop-nodal semimetal in the hyperhoneycomb lattice journal April 2018
Isolated highly localized bands in YBi 2 monolayer caused by 4 f orbitals journal September 2018
Prediction of staggered stacking 2D BeP semiconductor with unique anisotropic electronic properties journal November 2019
Topological node line semimetal state in two-dimensional tetragonal allotrope of Ge and Sn journal March 2019
Ferromagnetic nodal-line metal in monolayer h -InC journal July 2019
Fully spin-polarized open and closed nodal lines in β -borophene by magnetic proximity effect journal September 2019
Dual topological insulator and insulator-semimetal transition in mirror-symmetric honeycomb materials journal November 2019
Plateaus of quantized conductance with high steps in topological nodal-line semimetals journal January 2020
Hourglasslike nodal net semimetal in Ag 2 BiO 3 journal August 2018
Spin-orbit-stable type-II nodal line band crossing in n -doped monolayer Mo X 2 ( X = S , Se,Te) journal December 2018
Monolayer Mg 2 C : Negative Poisson's ratio and unconventional two-dimensional emergent fermions journal October 2018
Dirac nodal lines protected against spin-orbit interaction in IrO 2 journal June 2019
Two-dimensional nodal-loop half-metal in monolayer MnN journal August 2019
Optical conductivity of three and two dimensional topological nodal line semimetals text January 2017
Isolated highly localized bands in $\mathrm{YbI_2}$ monolayer caused by $4f$ orbitals text January 2018
Two-dimensional honeycomb borophene oxide: Strong anisotropy and nodal loop transformation text January 2018
Two-dimensional nodal-loop half metal in monolayer MnN text January 2019

Figures / Tables (4)


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