skip to main content
DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Well‐Dispersed Nickel‐ and Zinc‐Tailored Electronic Structure of a Transition Metal Oxide for Highly Active Alkaline Hydrogen Evolution Reaction

Authors:
 [1];  [2];  [3];  [2];  [4];  [5];  [5];  [2];  [2];  [6]; ORCiD logo [1]
  1. Key Laboratory for Advanced Ceramics and Machining Technology of Ministry of EducationTianjin Key Laboratory of Composite and Functional MaterialsSchool of Materials Science and EngineeringTianjin University Tianjin 300072 China, School of Chemical EngineeringThe University of Adelaide Adelaide SA 5005 Australia
  2. Key Laboratory for Advanced Ceramics and Machining Technology of Ministry of EducationTianjin Key Laboratory of Composite and Functional MaterialsSchool of Materials Science and EngineeringTianjin University Tianjin 300072 China
  3. Institute of Physical Science and Information TechnologyAnhui University Anhui 230601 China
  4. Beijing Synchrotron Radiation FacilityInstitute of High Energy PhysicsChinese Academy of Sciences Beijing 100049 China
  5. Department of ChemistryVirginia Tech Blacksburg VA 24061 USA
  6. School of Chemical EngineeringThe University of Adelaide Adelaide SA 5005 Australia
Publication Date:
Sponsoring Org.:
USDOE
OSTI Identifier:
1497740
Grant/Contract Number:  
DE‐AC02‐76SF00515
Resource Type:
Publisher's Accepted Manuscript
Journal Name:
Advanced Materials
Additional Journal Information:
Journal Name: Advanced Materials Journal Volume: 31 Journal Issue: 16; Journal ID: ISSN 0935-9648
Publisher:
Wiley Blackwell (John Wiley & Sons)
Country of Publication:
Germany
Language:
English

Citation Formats

Ling, Tao, Zhang, Tong, Ge, Binghui, Han, Lili, Zheng, Lirong, Lin, Feng, Xu, Zhengrui, Hu, Wen‐Bin, Du, Xi‐Wen, Davey, Kenneth, and Qiao, Shi‐Zhang. Well‐Dispersed Nickel‐ and Zinc‐Tailored Electronic Structure of a Transition Metal Oxide for Highly Active Alkaline Hydrogen Evolution Reaction. Germany: N. p., 2019. Web. doi:10.1002/adma.201807771.
Ling, Tao, Zhang, Tong, Ge, Binghui, Han, Lili, Zheng, Lirong, Lin, Feng, Xu, Zhengrui, Hu, Wen‐Bin, Du, Xi‐Wen, Davey, Kenneth, & Qiao, Shi‐Zhang. Well‐Dispersed Nickel‐ and Zinc‐Tailored Electronic Structure of a Transition Metal Oxide for Highly Active Alkaline Hydrogen Evolution Reaction. Germany. doi:10.1002/adma.201807771.
Ling, Tao, Zhang, Tong, Ge, Binghui, Han, Lili, Zheng, Lirong, Lin, Feng, Xu, Zhengrui, Hu, Wen‐Bin, Du, Xi‐Wen, Davey, Kenneth, and Qiao, Shi‐Zhang. Wed . "Well‐Dispersed Nickel‐ and Zinc‐Tailored Electronic Structure of a Transition Metal Oxide for Highly Active Alkaline Hydrogen Evolution Reaction". Germany. doi:10.1002/adma.201807771.
@article{osti_1497740,
title = {Well‐Dispersed Nickel‐ and Zinc‐Tailored Electronic Structure of a Transition Metal Oxide for Highly Active Alkaline Hydrogen Evolution Reaction},
author = {Ling, Tao and Zhang, Tong and Ge, Binghui and Han, Lili and Zheng, Lirong and Lin, Feng and Xu, Zhengrui and Hu, Wen‐Bin and Du, Xi‐Wen and Davey, Kenneth and Qiao, Shi‐Zhang},
abstractNote = {},
doi = {10.1002/adma.201807771},
journal = {Advanced Materials},
number = 16,
volume = 31,
place = {Germany},
year = {2019},
month = {2}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record
DOI: 10.1002/adma.201807771

Citation Metrics:
Cited by: 26 works
Citation information provided by
Web of Science

Save / Share:

Works referenced in this record:

Activating and optimizing MoS2 basal planes for hydrogen evolution through the formation of strained sulphur vacancies
journal, November 2015

  • Li, Hong; Tsai, Charlie; Koh, Ai Leen
  • Nature Materials, Vol. 15, Issue 1
  • DOI: 10.1038/nmat4465

Metal/Oxide Interface Nanostructures Generated by Surface Segregation for Electrocatalysis
journal, October 2015


An overview of hydrogen production technologies
journal, January 2009


A rhodium/silicon co-electrocatalyst design concept to surpass platinum hydrogen evolution activity at high overpotentials
journal, July 2016

  • Zhu, Lili; Lin, Haiping; Li, Youyong
  • Nature Communications, Vol. 7, Issue 1
  • DOI: 10.1038/ncomms12272

Metal–air batteries: from oxygen reduction electrochemistry to cathode catalysts
journal, January 2012

  • Cheng, Fangyi; Chen, Jun
  • Chemical Society Reviews, Vol. 41, Issue 6, p. 2172-2192
  • DOI: 10.1039/c1cs15228a

Metal–Organic Framework Derived Hybrid Co 3 O 4 -Carbon Porous Nanowire Arrays as Reversible Oxygen Evolution Electrodes
journal, September 2014

  • Ma, Tian Yi; Dai, Sheng; Jaroniec, Mietek
  • Journal of the American Chemical Society, Vol. 136, Issue 39
  • DOI: 10.1021/ja5082553

Double perovskites as a family of highly active catalysts for oxygen evolution in alkaline solution
journal, September 2013

  • Grimaud, Alexis; May, Kevin J.; Carlton, Christopher E.
  • Nature Communications, Vol. 4, Issue 1
  • DOI: 10.1038/ncomms3439

Enhancing Hydrogen Evolution Activity in Water Splitting by Tailoring Li+-Ni(OH)2-Pt Interfaces
journal, December 2011


Enhancing Electrocatalytic Oxygen Reduction on MnO 2 with Vacancies
journal, January 2013

  • Cheng, Fangyi; Zhang, Tianran; Zhang, Yi
  • Angewandte Chemie International Edition, Vol. 52, Issue 9
  • DOI: 10.1002/anie.201208582

Engineering surface atomic structure of single-crystal cobalt (II) oxide nanorods for superior electrocatalysis
journal, September 2016

  • Ling, Tao; Yan, Dong-Yang; Jiao, Yan
  • Nature Communications, Vol. 7, Issue 1
  • DOI: 10.1038/ncomms12876

Engineering water dissociation sites in MoS 2 nanosheets for accelerated electrocatalytic hydrogen production
journal, January 2016

  • Zhang, Jian; Wang, Tao; Liu, Pan
  • Energy & Environmental Science, Vol. 9, Issue 9
  • DOI: 10.1039/C6EE01786J

Co3O4 nanocrystals on graphene as a synergistic catalyst for oxygen reduction reaction
journal, August 2011

  • Liang, Yongye; Li, Yanguang; Wang, Hailiang
  • Nature Materials, Vol. 10, Issue 10, p. 780-786
  • DOI: 10.1038/nmat3087

Oxygen Reduction Electrocatalyst Based on Strongly Coupled Cobalt Oxide Nanocrystals and Carbon Nanotubes
journal, September 2012

  • Liang, Yongye; Wang, Hailiang; Diao, Peng
  • Journal of the American Chemical Society, Vol. 134, Issue 38
  • DOI: 10.1021/ja305623m

Nanoscale nickel oxide/nickel heterostructures for active hydrogen evolution electrocatalysis
journal, August 2014

  • Gong, Ming; Zhou, Wu; Tsai, Mon-Che
  • Nature Communications, Vol. 5, Issue 1
  • DOI: 10.1038/ncomms5695

Bifunctional non-noble metal oxide nanoparticle electrocatalysts through lithium-induced conversion for overall water splitting
journal, June 2015

  • Wang, Haotian; Lee, Hyun-Wook; Deng, Yong
  • Nature Communications, Vol. 6, Issue 1
  • DOI: 10.1038/ncomms8261

Ultrathin platinum nanowires grown on single-layered nickel hydroxide with high hydrogen evolution activity
journal, March 2015

  • Yin, Huajie; Zhao, Shenlong; Zhao, Kun
  • Nature Communications, Vol. 6, Issue 1
  • DOI: 10.1038/ncomms7430

What Are Batteries, Fuel Cells, and Supercapacitors?
journal, October 2004

  • Winter, Martin; Brodd, Ralph J.
  • Chemical Reviews, Vol. 104, Issue 10, p. 4245-4270
  • DOI: 10.1021/cr020730k

Gas-Phase Cation Exchange toward Porous Single-Crystal CoO Nanorods for Catalytic Hydrogen Production
journal, December 2014

  • Zhang, Hao; Ling, Tao; Du, Xi-Wen
  • Chemistry of Materials, Vol. 27, Issue 1
  • DOI: 10.1021/cm504076n

Functional links between stability and reactivity of strontium ruthenate single crystals during oxygen evolution
journal, June 2014

  • Chang, Seo Hyoung; Danilovic, Nemanja; Chang, Kee-Chul
  • Nature Communications, Vol. 5, Issue 1
  • DOI: 10.1038/ncomms5191

Advancing the Electrochemistry of the Hydrogen-Evolution Reaction through Combining Experiment and Theory
journal, November 2014

  • Zheng, Yao; Jiao, Yan; Jaroniec, Mietek
  • Angewandte Chemie International Edition, Vol. 54, Issue 1
  • DOI: 10.1002/anie.201407031

Homogeneously dispersed multimetal oxygen-evolving catalysts
journal, March 2016


Cation exchange on the nanoscale: an emerging technique for new material synthesis, device fabrication, and chemical sensing
journal, January 2013

  • Rivest, Jessy B.; Jain, Prashant K.
  • Chem. Soc. Rev., Vol. 42, Issue 1
  • DOI: 10.1039/C2CS35241A

Gold-supported cerium-doped NiOx catalysts for water oxidation
journal, April 2016

  • Ng, Jia Wei Desmond; García-Melchor, Max; Bajdich, Michal
  • Nature Energy, Vol. 1, Issue 5
  • DOI: 10.1038/nenergy.2016.53

Solar Water Splitting Cells
journal, November 2010

  • Walter, Michael G.; Warren, Emily L.; McKone, James R.
  • Chemical Reviews, Vol. 110, Issue 11, p. 6446-6473
  • DOI: 10.1021/cr1002326

Activating cobalt(II) oxide nanorods for efficient electrocatalysis by strain engineering
journal, November 2017


Atomic-level structure engineering of metal oxides for high-rate oxygen intercalation pseudocapacitance
journal, October 2018


High Electrocatalytic Hydrogen Evolution Activity of an Anomalous Ruthenium Catalyst
journal, December 2016

  • Zheng, Yao; Jiao, Yan; Zhu, Yihan
  • Journal of the American Chemical Society, Vol. 138, Issue 49
  • DOI: 10.1021/jacs.6b11291

Ni–Mo Nanopowders for Efficient Electrochemical Hydrogen Evolution
journal, January 2013

  • McKone, James R.; Sadtler, Bryce F.; Werlang, Caroline A.
  • ACS Catalysis, Vol. 3, Issue 2
  • DOI: 10.1021/cs300691m

Solar Energy Supply and Storage for the Legacy and Nonlegacy Worlds
journal, November 2010

  • Cook, Timothy R.; Dogutan, Dilek K.; Reece, Steven Y.
  • Chemical Reviews, Vol. 110, Issue 11
  • DOI: 10.1021/cr100246c

Advanced zinc-air batteries based on high-performance hybrid electrocatalysts
journal, May 2013

  • Li, Yanguang; Gong, Ming; Liang, Yongye
  • Nature Communications, Vol. 4, Issue 1
  • DOI: 10.1038/ncomms2812

Design principles for oxygen-reduction activity on perovskite oxide catalysts for fuel cells and metal–air batteries
journal, June 2011

  • Suntivich, Jin; Gasteiger, Hubert A.; Yabuuchi, Naoaki
  • Nature Chemistry, Vol. 3, Issue 7, p. 546-550
  • DOI: 10.1038/nchem.1069

Towards the computational design of solid catalysts
journal, April 2009

  • Nørskov, J.; Bligaard, T.; Rossmeisl, J.
  • Nature Chemistry, Vol. 1, Issue 1, p. 37-46
  • DOI: 10.1038/nchem.121

A Perovskite Oxide Optimized for Oxygen Evolution Catalysis from Molecular Orbital Principles
journal, October 2011


Hierarchical Zn x Co 3– x O 4 Nanoarrays with High Activity for Electrocatalytic Oxygen Evolution
journal, February 2014

  • Liu, Xijun; Chang, Zheng; Luo, Liang
  • Chemistry of Materials, Vol. 26, Issue 5
  • DOI: 10.1021/cm4040903

A mini review on nickel-based electrocatalysts for alkaline hydrogen evolution reaction
journal, December 2015


Spontaneous Superlattice Formation in Nanorods Through Partial Cation Exchange
journal, July 2007

  • Robinson, R. D.; Sadtler, B.; Demchenko, D. O.
  • Science, Vol. 317, Issue 5836, p. 355-358
  • DOI: 10.1126/science.1142593

A metal-free bifunctional electrocatalyst for oxygen reduction and oxygen evolution reactions
journal, April 2015

  • Zhang, Jintao; Zhao, Zhenghang; Xia, Zhenhai
  • Nature Nanotechnology, Vol. 10, Issue 5
  • DOI: 10.1038/nnano.2015.48

O-K and Co-L XANES Study on Oxygen Intercalation in Perovskite SrCoO3-δ
journal, January 2010

  • Karvonen, Lassi; Valkeapaa, Markus; Liu, Ru-Shi
  • Chemistry of Materials, Vol. 22, Issue 1, p. 70-76
  • DOI: 10.1021/cm9021563

A comprehensive review on PEM water electrolysis
journal, April 2013

  • Carmo, Marcelo; Fritz, David L.; Mergel, Jürgen
  • International Journal of Hydrogen Energy, Vol. 38, Issue 12, p. 4901-4934
  • DOI: 10.1016/j.ijhydene.2013.01.151

In Situ and Theoretical Studies for the Dissociation of Water on an Active Ni/CeO 2 Catalyst: Importance of Strong Metal-Support Interactions for the Cleavage of O-H Bonds
journal, February 2015

  • Carrasco, Javier; López-Durán, David; Liu, Zongyuan
  • Angewandte Chemie International Edition, Vol. 54, Issue 13
  • DOI: 10.1002/anie.201410697

Evidence of substitutional Co ion clusters in Zn 1 x Co x O dilute magnetic semiconductors
journal, June 2008


Versatile nanoporous bimetallic phosphides towards electrochemical water splitting
journal, January 2016

  • Tan, Yongwen; Wang, Hao; Liu, Pan
  • Energy & Environmental Science, Vol. 9, Issue 7
  • DOI: 10.1039/C6EE01109H

Multiscale Structural Engineering of Ni-Doped CoO Nanosheets for Zinc-Air Batteries with High Power Density
journal, October 2018


Atomically and Electronically Coupled Pt and CoO Hybrid Nanocatalysts for Enhanced Electrocatalytic Performance
journal, December 2016