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Title: Characterizing laser-plasma ion accelerators driving an intense neutron beam via nuclear signatures

Abstract

Compact, bright neutron sources are opening up several emerging applications including detection of nuclear materials for national security applications. At Los Alamos National Laboratory, we have used a short-pulse laser to accelerate deuterons in the relativistic transparency regime. These deuterons impinge on a beryllium converter to generate neutrons. During the initial experiments where these neutrons were used for active interrogation of uranium and plutonium, we observed β-delayed neutron production from decay of 9Li, formed by the high-energy deuteron bombardment of the beryllium converter. Analysis of the delayed neutrons provides novel evidence of the divergence of the highest energy portion of the deuterons (i.e., above 10 MeV/nucleon) from the laser axis, a documented feature of the breakout afterburner laser-plasma ion acceleration mechanism. Furthermore, these delayed neutrons form the basis of non-intrusive diagnostics for determining the features of deuteron acceleration as well as monitoring neutron production for the next generation of laser-driven neutron sources.

Authors:
ORCiD logo [1];  [2]; ORCiD logo [1];  [3];  [4]; ORCiD logo [1]; ORCiD logo [1]; ORCiD logo [1]; ORCiD logo [1];  [5]; ORCiD logo [1]; ORCiD logo [1]
  1. Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
  2. Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Spectral Sciences, Burlington, MA (United States)
  3. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
  4. ELI Beamlines, Prague (Czech Republic); Helmholtz-Zentrum Dresden-Rossendorf, Dresden (Germany)
  5. Technische Univ. Darmstadt, Darmstadt (Germany)
Publication Date:
Research Org.:
Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
Sponsoring Org.:
USDOE Laboratory Directed Research and Development (LDRD) Program
OSTI Identifier:
1496749
Report Number(s):
LA-UR-17-30568
Journal ID: ISSN 2045-2322
Grant/Contract Number:  
89233218CNA000001
Resource Type:
Accepted Manuscript
Journal Name:
Scientific Reports
Additional Journal Information:
Journal Volume: 9; Journal Issue: 1; Journal ID: ISSN 2045-2322
Publisher:
Nature Publishing Group
Country of Publication:
United States
Language:
English
Subject:
43 PARTICLE ACCELERATORS

Citation Formats

Favalli, Andrea, Guler, Nevzat, Henzlova, Daniela Constance, Croft, Stephen, Falk, K., Gautier, Daniel Cort, Ianakiev, Kiril Dimitrov, Iliev, Metodi, Palaniyappan, Sasikumar, Roth, Markus, Fernandez, Juan C., and Swinhoe, Martyn Thomas. Characterizing laser-plasma ion accelerators driving an intense neutron beam via nuclear signatures. United States: N. p., 2019. Web. doi:10.1038/s41598-019-39054-z.
Favalli, Andrea, Guler, Nevzat, Henzlova, Daniela Constance, Croft, Stephen, Falk, K., Gautier, Daniel Cort, Ianakiev, Kiril Dimitrov, Iliev, Metodi, Palaniyappan, Sasikumar, Roth, Markus, Fernandez, Juan C., & Swinhoe, Martyn Thomas. Characterizing laser-plasma ion accelerators driving an intense neutron beam via nuclear signatures. United States. https://doi.org/10.1038/s41598-019-39054-z
Favalli, Andrea, Guler, Nevzat, Henzlova, Daniela Constance, Croft, Stephen, Falk, K., Gautier, Daniel Cort, Ianakiev, Kiril Dimitrov, Iliev, Metodi, Palaniyappan, Sasikumar, Roth, Markus, Fernandez, Juan C., and Swinhoe, Martyn Thomas. Thu . "Characterizing laser-plasma ion accelerators driving an intense neutron beam via nuclear signatures". United States. https://doi.org/10.1038/s41598-019-39054-z. https://www.osti.gov/servlets/purl/1496749.
@article{osti_1496749,
title = {Characterizing laser-plasma ion accelerators driving an intense neutron beam via nuclear signatures},
author = {Favalli, Andrea and Guler, Nevzat and Henzlova, Daniela Constance and Croft, Stephen and Falk, K. and Gautier, Daniel Cort and Ianakiev, Kiril Dimitrov and Iliev, Metodi and Palaniyappan, Sasikumar and Roth, Markus and Fernandez, Juan C. and Swinhoe, Martyn Thomas},
abstractNote = {Compact, bright neutron sources are opening up several emerging applications including detection of nuclear materials for national security applications. At Los Alamos National Laboratory, we have used a short-pulse laser to accelerate deuterons in the relativistic transparency regime. These deuterons impinge on a beryllium converter to generate neutrons. During the initial experiments where these neutrons were used for active interrogation of uranium and plutonium, we observed β-delayed neutron production from decay of 9Li, formed by the high-energy deuteron bombardment of the beryllium converter. Analysis of the delayed neutrons provides novel evidence of the divergence of the highest energy portion of the deuterons (i.e., above 10 MeV/nucleon) from the laser axis, a documented feature of the breakout afterburner laser-plasma ion acceleration mechanism. Furthermore, these delayed neutrons form the basis of non-intrusive diagnostics for determining the features of deuteron acceleration as well as monitoring neutron production for the next generation of laser-driven neutron sources.},
doi = {10.1038/s41598-019-39054-z},
journal = {Scientific Reports},
number = 1,
volume = 9,
place = {United States},
year = {Thu Feb 14 00:00:00 EST 2019},
month = {Thu Feb 14 00:00:00 EST 2019}
}

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Figure 1 Figure 1: Experimental setup at Trident facility (not in scale).

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Works referenced in this record:

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Bright Laser-Driven Neutron Source Based on the Relativistic Transparency of Solids
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Improved yield and control of spectra from high-intensity laser-generated neutron beams
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Ion acceleration by superintense laser-plasma interaction
text, January 2013


Efficient quasi-monoenergetic ion beams from laser-driven relativistic plasmas
journal, December 2015

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  • Nature Communications, Vol. 6, Issue 1
  • DOI: 10.1038/ncomms10170

Dynamics of relativistic transparency and optical shuttering in expanding overdense plasmas
journal, August 2012

  • Palaniyappan, Sasi; Hegelich, B. Manuel; Wu, Hui-Chun
  • Nature Physics, Vol. 8, Issue 10
  • DOI: 10.1038/nphys2390

Monoenergetic and GeV ion acceleration from the laser breakout afterburner using ultrathin targets
journal, May 2007

  • Yin, L.; Albright, B. J.; Hegelich, B. M.
  • Physics of Plasmas, Vol. 14, Issue 5
  • DOI: 10.1063/1.2436857

TRIDENT high-energy-density facility experimental capabilities and diagnostics
journal, October 2008

  • Batha, S. H.; Aragonez, R.; Archuleta, F. L.
  • Review of Scientific Instruments, Vol. 79, Issue 10
  • DOI: 10.1063/1.2972020

Break-out afterburner ion acceleration in the longer laser pulse length regime
journal, June 2011

  • Yin, L.; Albright, B. J.; Jung, D.
  • Physics of Plasmas, Vol. 18, Issue 6
  • DOI: 10.1063/1.3596555

Neutron imaging with the short-pulse laser driven neutron source at the Trident laser facility
journal, October 2016

  • Guler, N.; Volegov, P.; Favalli, A.
  • Journal of Applied Physics, Vol. 120, Issue 15
  • DOI: 10.1063/1.4964248

Laser-plasmas in the relativistic-transparency regime: Science and applications
journal, May 2017

  • Fernández, Juan C.; Cort Gautier, D.; Huang, Chengkung
  • Physics of Plasmas, Vol. 24, Issue 5
  • DOI: 10.1063/1.4983991

Experimental demonstration of particle energy, conversion efficiency and spectral shape required for ion-based fast ignition
journal, July 2011


Fast ignition with laser-driven proton and ion beams
journal, April 2014


Figures/Tables have been extracted from DOE-funded journal article accepted manuscripts.