Toward Environmentally Friendly Lithium Sulfur Batteries: Probing the Role of Electrode Design in MoS2-Containing Li–S Batteries with a Green Electrolyte

Wang, Lei; Abraham, Alyson; Lutz, Diana M.; Quilty, Calvin D.; Takeuchi, Esther S.; Takeuchi, Kenneth J.; Marschilok, Amy C.

doi:10.1021/acssuschemeng.8b06141

Title: Toward Environmentally Friendly Lithium Sulfur Batteries: Probing the Role of Electrode Design in MoS₂-Containing Li–S Batteries with a Green Electrolyte

Journal Article · 03 February 2019 · ACS Sustainable Chemistry & Engineering

DOI: https://doi.org/10.1021/acssuschemeng.8b06141 · OSTI ID:1496231

^[1]; Abraham, Alyson ^[2];

^[2]; Quilty, Calvin D. ^[2];

^[3];

^[2];

^[3]

State Univ. of New York at Stony Brook, Stony Brook, NY (United States); Stony Brook University
State Univ. of New York at Stony Brook, Stony Brook, NY (United States)
State Univ. of New York at Stony Brook, Stony Brook, NY (United States); Brookhaven National Lab. (BNL), Upton, NY (United States)

While lithium sulfur batteries (Li–S) hold promise as future high energy density low cost energy storage systems, barriers to implementation include low sulfur loading, limited cycle life, and the use of toxic electrolyte solvents. A comprehensive study of Li–S cells in the environmentally benign di(propylene glycol) dimethyl ether (DPGDME)-based electrolyte, using as-prepared MoS₂ nanosheets derived from a facile aqueous microwave synthesis as polysulfide trapping agents, is reported herein for the first time. Conventional coated foil electrodes and binder-free electrodes (BFEs) with various structures are systematically generated and tested to correlate electrode design with the resulting electrochemical behavior. Significantly improved Li–S electrochemistry is demonstrated through the synergy of MoS₂ chemistry and binder-free electrode engineering. In the coating configuration, the MoS₂-containing cell evinced better rate performance and more stable cyclability than the cell without MoS₂. In comparison with the coating counterparts, the BFE cells exhibited excellent cycle stability and superior rate capability (10-fold capacities and energy density per electrode weight with 20% higher retention rate) despite 2X higher areal sulfur loading. As a result, the BFE cell improvement can be attributed to the synergistic effect of the i) interconnected macroporous structure of CNT interlayers, providing a conductive framework, and ii) the efficient polysulfide trapping by the MoS₂ nanosheets.

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Research Organization:: Brookhaven National Lab. (BNL), Upton, NY (United States); Stony Brook Univ., Stony Brook, NY (United States)

Sponsoring Organization:: USDOE; USDOE Office of Energy Efficiency and Renewable Energy (EERE)

Grant/Contract Number:: EE0008208; SC0012704

OSTI ID:: 1496231

Report Number(s):: BNL--211467-2019-JAAM

Journal Information:: ACS Sustainable Chemistry & Engineering, Journal Name: ACS Sustainable Chemistry & Engineering Journal Issue: 5 Vol. 7; ISSN 2168-0485

Publisher:: American Chemical Society (ACS)Copyright Statement

Country of Publication:: United States

Language:: English

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Defect Control in the Synthesis of 2 D MoS ₂ Nanosheets: Polysulfide Trapping in Composite Sulfur Cathodes for Li–S Batteries Abraham, Alyson; Wang, Lei; Quilty, Calvin D. ChemSusChem, Vol. 13, Issue 6 https://doi.org/10.1002/cssc.201903028	journal	March 2020
Encapsulation of Few-Layer MoS2 in the Pores of Mesoporous Carbon Hollow Spheres for Lithium-Sulfur Batteries Zhao, Yunyan; Zhuang, Qianyu; Li, Wenda Nanomaterials, Vol. 9, Issue 9 https://doi.org/10.3390/nano9091247	journal	September 2019

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Title: Toward Environmentally Friendly Lithium Sulfur Batteries: Probing the Role of Electrode Design in MoS2-Containing Li–S Batteries with a Green Electrolyte

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Title: Toward Environmentally Friendly Lithium Sulfur Batteries: Probing the Role of Electrode Design in MoS₂-Containing Li–S Batteries with a Green Electrolyte