Consequences of exchange-site heterogeneity and dynamics on the UV-visible spectrum of Cu-exchanged SSZ-13
Abstract
Theory and experiment reveal relationships between observed UV-visible spectra and ion exchange site types, ion nuclearity, and finite-temperature dynamics in Cu exchanged chabazite (SSZ-13) zeolites.
- Authors:
-
[1];
[2];
[3];
[4];
[3];
[3];
[3];
[1]
- Department of Chemical and Biomolecular Engineering, University of Notre Dame, Notre Dame, USA
- Department of Chemical and Biomolecular Engineering, University of Notre Dame, Notre Dame, USA, Department of Chemical Engineering
- Charles D. Davidson School of Chemical Engineering, Purdue University, West Lafayette, USA
- Department of Chemical and Biological Engineering, University of Wisconsin-Madison, Madison, USA
- Publication Date:
- Research Org.:
- Purdue Univ., West Lafayette, IN (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- Contributing Org.:
- Center for Research Computing at Notre Dame; EMSL, a DOE Office of Science User Facility sponsored by the Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory
- OSTI Identifier:
- 1490127
- Alternate Identifier(s):
- OSTI ID: 1495316; OSTI ID: 1835585
- Grant/Contract Number:
- SC0019026
- Resource Type:
- Published Article
- Journal Name:
- Chemical Science
- Additional Journal Information:
- Journal Name: Chemical Science Journal Volume: 10 Journal Issue: 8; Journal ID: ISSN 2041-6520
- Publisher:
- Royal Society of Chemistry (RSC)
- Country of Publication:
- United Kingdom
- Language:
- English
- Subject:
- 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; 36 MATERIALS SCIENCE
Citation Formats
Li, Hui, Paolucci, Christopher, Khurana, Ishant, Wilcox, Laura N., Göltl, Florian, Albarracin-Caballero, Jonatan D., Shih, Arthur J., Ribeiro, Fabio H., Gounder, Rajamani, and Schneider, William F. Consequences of exchange-site heterogeneity and dynamics on the UV-visible spectrum of Cu-exchanged SSZ-13. United Kingdom: N. p., 2019.
Web. doi:10.1039/C8SC05056B.
Li, Hui, Paolucci, Christopher, Khurana, Ishant, Wilcox, Laura N., Göltl, Florian, Albarracin-Caballero, Jonatan D., Shih, Arthur J., Ribeiro, Fabio H., Gounder, Rajamani, & Schneider, William F. Consequences of exchange-site heterogeneity and dynamics on the UV-visible spectrum of Cu-exchanged SSZ-13. United Kingdom. https://doi.org/10.1039/C8SC05056B
Li, Hui, Paolucci, Christopher, Khurana, Ishant, Wilcox, Laura N., Göltl, Florian, Albarracin-Caballero, Jonatan D., Shih, Arthur J., Ribeiro, Fabio H., Gounder, Rajamani, and Schneider, William F. Wed .
"Consequences of exchange-site heterogeneity and dynamics on the UV-visible spectrum of Cu-exchanged SSZ-13". United Kingdom. https://doi.org/10.1039/C8SC05056B.
@article{osti_1490127,
title = {Consequences of exchange-site heterogeneity and dynamics on the UV-visible spectrum of Cu-exchanged SSZ-13},
author = {Li, Hui and Paolucci, Christopher and Khurana, Ishant and Wilcox, Laura N. and Göltl, Florian and Albarracin-Caballero, Jonatan D. and Shih, Arthur J. and Ribeiro, Fabio H. and Gounder, Rajamani and Schneider, William F.},
abstractNote = {Theory and experiment reveal relationships between observed UV-visible spectra and ion exchange site types, ion nuclearity, and finite-temperature dynamics in Cu exchanged chabazite (SSZ-13) zeolites.},
doi = {10.1039/C8SC05056B},
journal = {Chemical Science},
number = 8,
volume = 10,
place = {United Kingdom},
year = {Wed Feb 20 00:00:00 EST 2019},
month = {Wed Feb 20 00:00:00 EST 2019}
}
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Figures / Tables:
Fig. 1: UV-visible spectra collected at 300 K of samples containing predominantly (a) Z2Cu (Si/Al = 5, Cu/Al = 0.21), (b) ZCuOH (Si/Al = 15, Cu/Al = 0.24) and (c) ZCuOH (Si/Al = 15, Cu/Al = 0.15), after 20% O2 treatment at 673 K (black), and 5% CO treatment atmore »
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