Postirradiation examination on metallic fuel in the AFC-2 irradiation test series
Abstract
In this paper, irradiation experiments on metallic fuel alloys containing rare earth additions to simulate potential carry-over from pyro-metallurgical reprocessing and minor actinide additions were performed in the Idaho National Laboratory Advanced Test Reactor. These tests were designated AFC-2A and AFC-2B. Additionally irradiation experiments were also performed on metallic fuel alloys containing minor actinide additions that were fabricated by different techniques. These tests were designated AFC-2E. These pins were removed from the reactor after achieving burnups between 6 and 11% fission per initial heave metal atom. Examination of these pins revealed that they were unintentionally operated beyond their desired power and temperature conditions. Highlights from the postirradiation examination of these experiments is discussed. A variety of issue contributed to the poor performance of these irradiation tests including capsule design, reactor power variations and fabrication issues. While all the issues contributed, the major issue was determined to be unanticipated variations in reactor power. Through comparisons between these experiments and historical off-normal experiments, it was possible to conclude bound the operating temperatures of these experiments. There likely was some in-pile melting in the rare earth addition experiments (AFC-2A, AFC-2B), but it is not likely that there was in-pile melting in the fabricationmore »
- Authors:
-
- Idaho National Lab. (INL), Idaho Falls, ID (United States)
- Publication Date:
- Research Org.:
- Idaho National Lab. (INL), Idaho Falls, ID (United States)
- Sponsoring Org.:
- USDOE Office of Nuclear Energy (NE)
- OSTI Identifier:
- 1484472
- Alternate Identifier(s):
- OSTI ID: 1495279
- Report Number(s):
- INL-JOU-18-50163-Rev000
Journal ID: ISSN 0022-3115
- Grant/Contract Number:
- AC07-05ID14517
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Journal of Nuclear Materials
- Additional Journal Information:
- Journal Volume: 509; Journal Issue: C; Journal ID: ISSN 0022-3115
- Publisher:
- Elsevier
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS; AFC-2; postirradiation examination; metallic fast reactor fuel; lanthanide carry-over; ternary fuel
Citation Formats
Harp, Jason M., Capriotti, Luca, Chichester, Heather J. M., Medvedev, Pavel G., Porter, Douglas L., and Hayes, Steven L. Postirradiation examination on metallic fuel in the AFC-2 irradiation test series. United States: N. p., 2018.
Web. doi:10.1016/j.jnucmat.2018.07.019.
Harp, Jason M., Capriotti, Luca, Chichester, Heather J. M., Medvedev, Pavel G., Porter, Douglas L., & Hayes, Steven L. Postirradiation examination on metallic fuel in the AFC-2 irradiation test series. United States. https://doi.org/10.1016/j.jnucmat.2018.07.019
Harp, Jason M., Capriotti, Luca, Chichester, Heather J. M., Medvedev, Pavel G., Porter, Douglas L., and Hayes, Steven L. Wed .
"Postirradiation examination on metallic fuel in the AFC-2 irradiation test series". United States. https://doi.org/10.1016/j.jnucmat.2018.07.019. https://www.osti.gov/servlets/purl/1484472.
@article{osti_1484472,
title = {Postirradiation examination on metallic fuel in the AFC-2 irradiation test series},
author = {Harp, Jason M. and Capriotti, Luca and Chichester, Heather J. M. and Medvedev, Pavel G. and Porter, Douglas L. and Hayes, Steven L.},
abstractNote = {In this paper, irradiation experiments on metallic fuel alloys containing rare earth additions to simulate potential carry-over from pyro-metallurgical reprocessing and minor actinide additions were performed in the Idaho National Laboratory Advanced Test Reactor. These tests were designated AFC-2A and AFC-2B. Additionally irradiation experiments were also performed on metallic fuel alloys containing minor actinide additions that were fabricated by different techniques. These tests were designated AFC-2E. These pins were removed from the reactor after achieving burnups between 6 and 11% fission per initial heave metal atom. Examination of these pins revealed that they were unintentionally operated beyond their desired power and temperature conditions. Highlights from the postirradiation examination of these experiments is discussed. A variety of issue contributed to the poor performance of these irradiation tests including capsule design, reactor power variations and fabrication issues. While all the issues contributed, the major issue was determined to be unanticipated variations in reactor power. Through comparisons between these experiments and historical off-normal experiments, it was possible to conclude bound the operating temperatures of these experiments. There likely was some in-pile melting in the rare earth addition experiments (AFC-2A, AFC-2B), but it is not likely that there was in-pile melting in the fabrication technique experiments (AFC-2E).},
doi = {10.1016/j.jnucmat.2018.07.019},
journal = {Journal of Nuclear Materials},
number = C,
volume = 509,
place = {United States},
year = {Wed Jul 11 00:00:00 EDT 2018},
month = {Wed Jul 11 00:00:00 EDT 2018}
}
Web of Science
Works referenced in this record:
Irradiation of Minor Actinide–Bearing Uranium-Plutonium-Zirconium Alloys up to ˜2.5 at. %, ˜7 at. %, and ˜10 at. % Burnups
journal, April 2015
- Ohta, Hirokazu; Ogata, Takanari; Papaioannou, Dimitrios
- Nuclear Technology, Vol. 190, Issue 1
Electron probe microanalysis of a METAPHIX UPuZr metallic alloy fuel irradiated to 7.0 at.% burn-up
journal, November 2016
- Brémier, S.; Inagaki, K.; Capriotti, L.
- Journal of Nuclear Materials, Vol. 480
Characterization of metallic fuel for minor actinides transmutation in fast reactor
journal, January 2017
- Capriotti, L.; Brémier, S.; Inagaki, K.
- Progress in Nuclear Energy, Vol. 94
Fabrication and evaluation of rare-earth-bearing fuel slugs for sodium-cooled fast reactors
journal, October 2014
- Kim, Jong Hwan; Song, Hoon; Kim, Ki Hwan
- Journal of Radioanalytical and Nuclear Chemistry, Vol. 303, Issue 1
A US perspective on fast reactor fuel fabrication technology and experience part I: metal fuels and assembly design
journal, June 2009
- Burkes, Douglas E.; Fielding, Randall S.; Porter, Douglas L.
- Journal of Nuclear Materials, Vol. 389, Issue 3
Metallic fast reactor fuels
journal, January 1997
- Hofman, G. L.; Walters, L. C.; Bauer, T. H.
- Progress in Nuclear Energy, Vol. 31, Issue 1-2
As-cast microstructures in U–Pu–Zr alloy fuel pins with 5–8wt.% minor actinides and 0–1.5wt% rare-earth elements
journal, November 2010
- Janney, Dawn E.; Kennedy, J. Rory
- Materials Characterization, Vol. 61, Issue 11
Hardening neutron spectrum for advanced actinide transmutation experiments in the ATR
journal, December 2005
- Chang, G. S.; Ambrosek, R. G.
- Radiation Protection Dosimetry, Vol. 115, Issue 1-4
Testing fast reactor fuels in a thermal reactor
journal, March 2018
- Medvedev, Pavel; Hayes, Steven; Bays, Samuel
- Nuclear Engineering and Design, Vol. 328
Metallography and fuel cladding chemical interaction in fast flux test facility irradiated metallic U-10Zr MFF-3 and MFF-5 fuel pins
journal, May 2016
- Carmack, W. J.; Chichester, H. M.; Porter, D. L.
- Journal of Nuclear Materials, Vol. 473
Verification of the BISON fuel performance code
journal, September 2014
- Hales, J. D.; Novascone, S. R.; Spencer, B. W.
- Annals of Nuclear Energy, Vol. 71
Validating the BISON fuel performance code to integral LWR experiments
journal, May 2016
- Williamson, R. L.; Gamble, K. A.; Perez, D. M.
- Nuclear Engineering and Design, Vol. 301
Tensile Properties of Martensitic Stainless Steels at Elevated Temperatures
journal, May 2005
- Roy, A. K.; Kukatla, S. R.; Yarlagadda, B.
- Journal of Materials Engineering and Performance, Vol. 14, Issue 2
Fuel/cladding compatibility in U-19Pu-10Zr/HT9-clad fuel at elevated temperatures
journal, September 1993
- Cohen, A. B.; Tsai, H.; Neimark, L. A.
- Journal of Nuclear Materials, Vol. 204
Behavior of EBR-II Mk-V-type fuel elements in simulated loss-of-flow tests
journal, September 1993
- Liu, Y. Y.; Tsai, H.; Billone, M. C.
- Journal of Nuclear Materials, Vol. 204
Full-length U–xPu–10Zr (x=0, 8, 19wt.%) fast reactor fuel test in FFTF
journal, August 2012
- Porter, D. L.; Tsai, Hanchung
- Journal of Nuclear Materials, Vol. 427, Issue 1-3
Swelling behavior of U-Pu-Zr fuel
journal, February 1990
- Hofman, Gerard L.; Pahl, R. G.; Lahm, C. E.
- Metallurgical Transactions A, Vol. 21, Issue 2
Fuel-Cladding Chemical Interaction in U-Pu-Zr Metallic Fuels: A Critical Review
journal, June 2017
- Matthews, Christopher; Unal, Cetin; Galloway, Jack
- Nuclear Technology, Vol. 198, Issue 3
Temperature gradient driven constituent redistribution in UZr alloys
journal, January 1996
- Hofman, G. L.; Hayes, S. L.; Petri, M. C.
- Journal of Nuclear Materials, Vol. 227, Issue 3
Works referencing / citing this record:
Advanced Postirradiation Characterization of Nuclear Fuels Using Pulsed Neutrons
journal, November 2019
- Vogel, Sven C.; Bourke, Mark A. M.; Craft, Aaron E.
- JOM, Vol. 72, Issue 1