Controlling 3-D Morphology of Ni-Fe-Based Nanocatalysts for Oxygen Evolution Reaction

Manso, Ryan H.; Zhu, Yimei; Acharya, Prashant; Deng, Shiqing; Crane, Cameron C.; Reinhart, Benjamin; Lee, Sungsik; Tong, Xiao; Zhu, Jing; Greenlee, Lauren F.; Chen, Jingyi

doi:10.1039/C8NR10138H

Title: Controlling 3-D Morphology of Ni-Fe-Based Nanocatalysts for Oxygen Evolution Reaction

Journal Article · 18 February 2019 · Nanoscale

DOI: https://doi.org/10.1039/C8NR10138H · OSTI ID:1494044

Manso, Ryan H. ^[1];

^[2]; Acharya, Prashant ^[1]; Deng, Shiqing ^[3]; Crane, Cameron C. ^[1]; Reinhart, Benjamin ^[4]; Lee, Sungsik ^[4]; Tong, Xiao ^[2]; Zhu, Jing ^[5]; Greenlee, Lauren F. ^[1]; Chen, Jingyi ^[1]

Univ. of Arkansas, Fayetteville, AR (United States)
Brookhaven National Lab. (BNL), Upton, NY (United States)
Brookhaven National Lab. (BNL), Upton, NY (United States); Tsinghua Univ., Beijing (People's Republic of China)
Argonne National Lab. (ANL), Lemont, IL (United States)
Tsinghua Univ., Beijing (People's Republic of China)

Here, controlling the 3-D morphology of nanocatalysts is one of the underexplored but important approaches for improving the sluggish kinetics of oxygen evolution reaction (OER) in water electrolysis. This work reports a scalable, oil-based method based on thermal decomposition or organometallic complexes to yield highly uniform Ni-Fe-based nanocatalysts with well-defined morphology (i.e., Ni-Fe core-shell, Ni/Fe alloy, and Fe-Ni core shell).

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Research Organization:: Brookhaven National Laboratory (BNL), Upton, NY (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

Grant/Contract Number:: SC0012704

OSTI ID:: 1494044

Report Number(s):: BNL--211253-2019-JAAM

Journal Information:: Nanoscale, Journal Name: Nanoscale Journal Issue: 17 Vol. 11; ISSN 2040-3364

Publisher:: Royal Society of ChemistryCopyright Statement

Country of Publication:: United States

Language:: English

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