Polymer morphology and interfacial charge transfer dominate over energy-dependent scattering in organic-inorganic thermoelectrics
Abstract
Hybrid (organic-inorganic) materials have emerged as a promising class of thermoelectric materials, achieving power factors (S2σ) exceeding those of either constituent. The mechanism of this enhancement is still under debate, and pinpointing the underlying physics has proven difficult. In this work, we combine transport measurements with theoretical simulations and first principles calculations on a prototypical PEDOT:PSS-Te(Cux) nanowire hybrid material system to understand the effect of templating and charge redistribution on the thermoelectric performance. Further, we apply the recently developed Kang-Snyder charge transport model to show that scattering of holes in the hybrid system, defined by the energy-dependent scattering parameter, remains the same as in the host polymer matrix; performance is instead dictated by polymer morphology manifested in an energy-independent transport coefficient. We build upon this language to explain thermoelectric behavior in a variety of PEDOT and P3HT based hybrids acting as a guide for future work in multiphase materials.
- Authors:
-
- Institute of Materials Research and Engineering (Singapore)
- Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Univ. of California, Berkeley, CA (United States)
- Institute of High Performance Computing (Singapore)
- Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
- Publication Date:
- Research Org.:
- Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1493278
- Grant/Contract Number:
- AC02-05CH11231
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Communications
- Additional Journal Information:
- Journal Volume: 9; Journal Issue: 1; Journal ID: ISSN 2041-1723
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; 36 MATERIALS SCIENCE
Citation Formats
Kumar, Pawan, Zaia, Edmond W., Yildirim, Erol, Repaka, D. V. Maheswar, Yang, Shuo-Wang, Urban, Jeffrey J., and Hippalgaonkar, Kedar. Polymer morphology and interfacial charge transfer dominate over energy-dependent scattering in organic-inorganic thermoelectrics. United States: N. p., 2018.
Web. doi:10.1038/s41467-018-07435-z.
Kumar, Pawan, Zaia, Edmond W., Yildirim, Erol, Repaka, D. V. Maheswar, Yang, Shuo-Wang, Urban, Jeffrey J., & Hippalgaonkar, Kedar. Polymer morphology and interfacial charge transfer dominate over energy-dependent scattering in organic-inorganic thermoelectrics. United States. https://doi.org/10.1038/s41467-018-07435-z
Kumar, Pawan, Zaia, Edmond W., Yildirim, Erol, Repaka, D. V. Maheswar, Yang, Shuo-Wang, Urban, Jeffrey J., and Hippalgaonkar, Kedar. Mon .
"Polymer morphology and interfacial charge transfer dominate over energy-dependent scattering in organic-inorganic thermoelectrics". United States. https://doi.org/10.1038/s41467-018-07435-z. https://www.osti.gov/servlets/purl/1493278.
@article{osti_1493278,
title = {Polymer morphology and interfacial charge transfer dominate over energy-dependent scattering in organic-inorganic thermoelectrics},
author = {Kumar, Pawan and Zaia, Edmond W. and Yildirim, Erol and Repaka, D. V. Maheswar and Yang, Shuo-Wang and Urban, Jeffrey J. and Hippalgaonkar, Kedar},
abstractNote = {Hybrid (organic-inorganic) materials have emerged as a promising class of thermoelectric materials, achieving power factors (S2σ) exceeding those of either constituent. The mechanism of this enhancement is still under debate, and pinpointing the underlying physics has proven difficult. In this work, we combine transport measurements with theoretical simulations and first principles calculations on a prototypical PEDOT:PSS-Te(Cux) nanowire hybrid material system to understand the effect of templating and charge redistribution on the thermoelectric performance. Further, we apply the recently developed Kang-Snyder charge transport model to show that scattering of holes in the hybrid system, defined by the energy-dependent scattering parameter, remains the same as in the host polymer matrix; performance is instead dictated by polymer morphology manifested in an energy-independent transport coefficient. We build upon this language to explain thermoelectric behavior in a variety of PEDOT and P3HT based hybrids acting as a guide for future work in multiphase materials.},
doi = {10.1038/s41467-018-07435-z},
journal = {Nature Communications},
number = 1,
volume = 9,
place = {United States},
year = {Mon Dec 17 00:00:00 EST 2018},
month = {Mon Dec 17 00:00:00 EST 2018}
}
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Figures / Tables:
Fig. 1: Morphology of hybrids and alignment of PEDOT:PSS at the inorganic interface (a, b) False-color scanning electron microscope (SEM) images of (a) PEDOT:PSS-Te and (b) PEDOT:PSS-Cu1.75Te films illustrate the overall morphology of the hybrid films – inorganic nanowires in a PEDOT:PSS matrix. The green color shows the surface nanowiresmore »
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