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Title: Real-time thermomechanical property monitoring during ion beam irradiation using in situ transient grating spectroscopy

Abstract

A facility for continuously monitoring the thermal and elastic performance of materials under exposure to ion beam irradiation has been designed and commissioned. By coupling an all-optical, non-contact, non-destructive measurement technique known as transient grating spectroscopy (TGS) to a 6 MV tandem ion accelerator, bulk material properties may be measured at high fidelity as a function of irradiation exposure and temperature. Ion beam energies and optical parameters may be tuned to ensure that only the properties of the ion-implanted surface layer are interrogated. This facility provides complementary capabilities to the set of facilities worldwide which have the ability to study the evolution of microstructure in situ during radiation exposure, but lack the ability to measure bulk-like properties. Here, the measurement physics of TGS, design of the experimental facility, and initial results using both light and heavy ion exposures are described. Lastly, several short- and long-term upgrades are discussed which will further increase the capabilities of this diagnostic.

Authors:
 [1];  [2];  [2];  [1]
  1. Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States)
  2. Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
Publication Date:
Research Org.:
Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
Sponsoring Org.:
USDOE Office of Science (SC)
OSTI Identifier:
1492374
Report Number(s):
SAND-2018-12137J
Journal ID: ISSN 0168-583X; 669047
Grant/Contract Number:  
AC04-94AL85000
Resource Type:
Accepted Manuscript
Journal Name:
Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms
Additional Journal Information:
Journal Volume: 440; Journal Issue: C; Journal ID: ISSN 0168-583X
Publisher:
Elsevier
Country of Publication:
United States
Language:
English
Subject:
46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND TECHNOLOGY; Ion beam; Transient grating; Irradiation; Photoacoustics; Surface acoustic wave; Radiation damage

Citation Formats

Dennett, Cody A., Buller, Daniel L., Hattar, Khalid Mikhiel, and Short, Michael P. Real-time thermomechanical property monitoring during ion beam irradiation using in situ transient grating spectroscopy. United States: N. p., 2018. Web. https://doi.org/10.1016/j.nimb.2018.10.025.
Dennett, Cody A., Buller, Daniel L., Hattar, Khalid Mikhiel, & Short, Michael P. Real-time thermomechanical property monitoring during ion beam irradiation using in situ transient grating spectroscopy. United States. https://doi.org/10.1016/j.nimb.2018.10.025
Dennett, Cody A., Buller, Daniel L., Hattar, Khalid Mikhiel, and Short, Michael P. Mon . "Real-time thermomechanical property monitoring during ion beam irradiation using in situ transient grating spectroscopy". United States. https://doi.org/10.1016/j.nimb.2018.10.025. https://www.osti.gov/servlets/purl/1492374.
@article{osti_1492374,
title = {Real-time thermomechanical property monitoring during ion beam irradiation using in situ transient grating spectroscopy},
author = {Dennett, Cody A. and Buller, Daniel L. and Hattar, Khalid Mikhiel and Short, Michael P.},
abstractNote = {A facility for continuously monitoring the thermal and elastic performance of materials under exposure to ion beam irradiation has been designed and commissioned. By coupling an all-optical, non-contact, non-destructive measurement technique known as transient grating spectroscopy (TGS) to a 6 MV tandem ion accelerator, bulk material properties may be measured at high fidelity as a function of irradiation exposure and temperature. Ion beam energies and optical parameters may be tuned to ensure that only the properties of the ion-implanted surface layer are interrogated. This facility provides complementary capabilities to the set of facilities worldwide which have the ability to study the evolution of microstructure in situ during radiation exposure, but lack the ability to measure bulk-like properties. Here, the measurement physics of TGS, design of the experimental facility, and initial results using both light and heavy ion exposures are described. Lastly, several short- and long-term upgrades are discussed which will further increase the capabilities of this diagnostic.},
doi = {10.1016/j.nimb.2018.10.025},
journal = {Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms},
number = C,
volume = 440,
place = {United States},
year = {2018},
month = {12}
}

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Cited by: 5 works
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Works referenced in this record:

Deformation mode maps for tensile deformation of neutron-irradiated structural alloys
journal, December 2004


Void swelling and microstructure evolution at very high damage level in self-ion irradiated ferritic-martensitic steels
journal, November 2016


Emulation of reactor irradiation damage using ion beams
journal, October 2014


Cascade fragmentation: deviation from power law in primary radiation damage
journal, February 2017


A review of transmission electron microscopes with in situ ion irradiation
journal, December 2009

  • Hinks, J. A.
  • Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 267, Issue 23-24
  • DOI: 10.1016/j.nimb.2009.09.014

Concurrent in situ ion irradiation transmission electron microscope
journal, November 2014

  • Hattar, K.; Bufford, D. C.; Buller, D. L.
  • Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 338
  • DOI: 10.1016/j.nimb.2014.08.002

Monitoring of the microstructure of ion-irradiated nuclear ceramics by in situ Raman spectroscopy : Microstructure of ion-irradiated nuclear ceramics
journal, December 2015

  • Miro, S.; Bordas, E.; Thomé, L.
  • Journal of Raman Spectroscopy, Vol. 47, Issue 4
  • DOI: 10.1002/jrs.4837

Nanoindentation and in situ microcompression in different dose regimes of proton beam irradiated 304 SS
journal, April 2017


Comparison of swelling and irradiation creep behavior of fcc-austenitic and bcc-ferritic/martensitic alloys at high neutron exposure
journal, January 2000


Applications of Transient Grating Spectroscopy to Radiation Materials Science
journal, June 2015


Materials aging at the mesoscale: Kinetics of thermal, stress, radiation activations
journal, August 2015


Bridging the gap to mesoscale radiation materials science with transient grating spectroscopy
journal, December 2016


Optical Generation and Characterization of Acoustic Waves in Thin Films: Fundamentals and Applications
journal, August 2000


Direct Measurement of Room-Temperature Nondiffusive Thermal Transport Over Micron Distances in a Silicon Membrane
journal, January 2013


Interaction of a Contact Resonance of Microspheres with Surface Acoustic Waves
journal, July 2013


Non-Contact Measurement of Thermal Diffusivity in Ion-Implanted Nuclear Materials
journal, November 2015

  • Hofmann, F.; Mason, D. R.; Eliason, J. K.
  • Scientific Reports, Vol. 5, Issue 1
  • DOI: 10.1038/srep16042

Increase in elastic anisotropy of single crystal tungsten upon He-ion implantation measured with laser-generated surface acoustic waves
journal, October 2016

  • Duncan, R. A.; Hofmann, F.; Vega-Flick, A.
  • Applied Physics Letters, Vol. 109, Issue 15
  • DOI: 10.1063/1.4964709

Detecting self-ion irradiation-induced void swelling in pure copper using transient grating spectroscopy
journal, February 2018


Time-resolved, dual heterodyne phase collection transient grating spectroscopy
journal, May 2017

  • Dennett, Cody A.; Short, Michael P.
  • Applied Physics Letters, Vol. 110, Issue 21
  • DOI: 10.1063/1.4983716

Thermal diffusivity determination using heterodyne phase insensitive transient grating spectroscopy
journal, June 2018

  • Dennett, Cody A.; Short, Michael P.
  • Journal of Applied Physics, Vol. 123, Issue 21
  • DOI: 10.1063/1.5026429

Evaluation of radiation damage using nonlinear ultrasound
journal, March 2012

  • Matlack, K. H.; Wall, J. J.; Kim, J. -Y.
  • Journal of Applied Physics, Vol. 111, Issue 5
  • DOI: 10.1063/1.3692086

Sensitivity of ultrasonic nonlinearity to irradiated, annealed, and re-irradiated microstructure changes in RPV steels
journal, May 2014


Development of a nondestructive inspection method for irradiation-induced microstructural evolution of thick 304 stainless steel blocks
journal, September 2013


Measurement of thermal conductivity in proton irradiated silicon
journal, April 2014

  • Khafizov, Marat; Yablinsky, Clarissa; Allen, Todd R.
  • Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 325
  • DOI: 10.1016/j.nimb.2014.02.003

Thermal conductivity measurements via time-domain thermoreflectance for the characterization of radiation induced damage
journal, May 2015

  • Cheaito, Ramez; Gorham, Caroline S.; Misra, Amit
  • Journal of Materials Research, Vol. 30, Issue 9
  • DOI: 10.1557/jmr.2015.11

Optical heterodyne detection of laser-induced gratings
journal, January 1998

  • Maznev, A. A.; Nelson, K. A.; Rogers, J. A.
  • Optics Letters, Vol. 23, Issue 16
  • DOI: 10.1364/OL.23.001319

Bulk and surface acoustic wave phenomena in crystals: Observation and interpretation
journal, December 2013


Phase-controlled, heterodyne laser-induced transient grating measurements of thermal transport properties in opaque material
journal, January 2012

  • Johnson, Jeremy A.; Maznev, Alexei A.; Bulsara, Mayank T.
  • Journal of Applied Physics, Vol. 111, Issue 2
  • DOI: 10.1063/1.3675467

Surface acoustic wave depth profiling of a functionally graded material
journal, September 2007

  • Goossens, Jozefien; Leclaire, Philippe; Xu, Xiaodong
  • Journal of Applied Physics, Vol. 102, Issue 5
  • DOI: 10.1063/1.2774002

Rayleigh wave velocity and displacement in orthorhombic, tetragonal, hexagonal, and cubic crystals
journal, November 1984

  • Royer, D.; Dieulesaint, E.
  • The Journal of the Acoustical Society of America, Vol. 76, Issue 5
  • DOI: 10.1121/1.391427

Transient thermal gratings at surfaces for thermal characterization of bulk materials and thin films
journal, September 1995

  • K�ding, O. W.; Skurk, H.; Maznev, A. A.
  • Applied Physics A Materials Science & Processing, Vol. 61, Issue 3
  • DOI: 10.1007/BF01538190

Elastic Constants of Tantalum, Tungsten, and Molybdenum
journal, May 1963


Single‐Crystal Elastic Properties of Tungsten from 24° to 1800°C
journal, October 1967

  • Lowrie, Robert; Gonas, A. M.
  • Journal of Applied Physics, Vol. 38, Issue 11
  • DOI: 10.1063/1.1709158

Elastic Constants of Single‐Crystal Mo and W between 77° and 500°K
journal, July 1962

  • Bolef, D. I.; De Klerk, J.
  • Journal of Applied Physics, Vol. 33, Issue 7
  • DOI: 10.1063/1.1728952

The elastic constants of nickel-copper alloy single crystals
journal, May 1965


SRIM – The stopping and range of ions in matter (2010)
journal, June 2010

  • Ziegler, James F.; Ziegler, M. D.; Biersack, J. P.
  • Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 268, Issue 11-12
  • DOI: 10.1016/j.nimb.2010.02.091

On the use of SRIM for computing radiation damage exposure
journal, September 2013

  • Stoller, R. E.; Toloczko, M. B.; Was, G. S.
  • Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 310
  • DOI: 10.1016/j.nimb.2013.05.008

Temperature dependent magnetic contributions to the high field elastic constants of nickel and an Fe-Ni alloy
journal, May 1960

  • Alers, G. A.; Neighbours, J. R.; Sato, H.
  • Journal of Physics and Chemistry of Solids, Vol. 13, Issue 1-2
  • DOI: 10.1016/0022-3697(60)90125-6

High-temperature thermal expansion of six metallic elements measured by dilatation method and X-ray diffraction
journal, February 1988

  • Suh, In-Kook; Ohta, H.; Waseda, Y.
  • Journal of Materials Science, Vol. 23, Issue 2
  • DOI: 10.1007/BF01174717

Recent advances in modeling and simulation of the exposure and response of tungsten to fusion energy conditions
journal, June 2017

  • Marian, Jaime; Becquart, Charlotte S.; Domain, Christophe
  • Nuclear Fusion, Vol. 57, Issue 9
  • DOI: 10.1088/1741-4326/aa5e8d

Helium-induced hardening effect in polycrystalline tungsten
journal, September 2017

  • Kong, Fanhang; Qu, Miao; Yan, Sha
  • Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 406
  • DOI: 10.1016/j.nimb.2017.02.029

Effects of sequential tungsten and helium ion implantation on nano-indentation hardness of tungsten
journal, June 2013

  • Armstrong, D. E. J.; Edmondson, P. D.; Roberts, S. G.
  • Applied Physics Letters, Vol. 102, Issue 25
  • DOI: 10.1063/1.4811825

Helium bubble formation in ultrafine and nanocrystalline tungsten under different extreme conditions
journal, March 2015


Dose rate effects in nickel-ion-irradiated nickel
journal, January 1975


The influence of ion beam rastering on the swelling of self-ion irradiated pure iron at 450 °C
journal, October 2015


Effect of triple ion beams in ferritic/martensitic steel on swelling behavior
journal, December 2002


    Works referencing / citing this record:

    Listening to Radiation Damage In Situ: Passive and Active Acoustic Techniques
    journal, November 2019