Impact of Modular Total Absorption Spectrometer measurements of decay of fission products on the decay heat and reactor flux calculation
- Univ. of Warsaw, Warsaw (Poland); Rutgers Univ., New Brunswick, NJ (United States); Univ. of Tennessee, Knoxville, TN (United States)
- Univ. of Warsaw, Warsaw (Poland); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
- Univ. of Tennessee, Knoxville, TN (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Louisiana State Univ., Baton Rouge, LA (United States)
- Univ. of Tennessee, Knoxville, TN (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
- Univ. of Tennessee, Knoxville, TN (United States)
- Univ. of Warsaw, Warsaw (Poland)
- Oak Ridge Associated Univ., Oak Ridge, TN (United States)
- Vanderbilt Univ., Nashville, TN (United States)
- Louisiana State Univ., Baton Rouge, LA (United States)
Here, we report the results of a β-decay study of fission products 86Br, 89Kr, 89Rb, 90gsRb, 90mRb, 90Kr, 92Rb, 139Xe, and 142Cs performed with the Modular Total Absorption Spectrometer (MTAS) and on-line mass-separated ion beams. These radioactivities were assessed by the Nuclear Energy Agency as having high priority for decay heat analysis during a nuclear fuel cycle. We observe a substantial increase in β feeding to high excited states in all daughter isotopes in comparison to earlier data. This increases the average γ-ray energy emitted by the decay of fission fragments during the first 10 000 s after fission of 235U and 239Pu by approximately 2% and 1%, respectively, improving agreement between results of calculations and direct observations. New MTAS results reduce the reference reactor ¯νe flux used to analyze reactor ¯νe interaction with detector matter. The reduction determined by the ab initio method for the four nuclear fuel components, 235U, 238U, 239Pu, and 241Pu, amounts to 0.976, 0.986, 0.983, and 0.984, respectively.
- Research Organization:
- Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
- Sponsoring Organization:
- USDOE Office of Science (SC), Nuclear Physics (NP); USDOE
- Grant/Contract Number:
- AC05-00OR22725; FG02-96ER40983; NA0002132; FG02-96ER40978; FG02-96ER41006; FG05-88ER40407
- OSTI ID:
- 1492173
- Alternate ID(s):
- OSTI ID: 1373799
- Journal Information:
- Physical Review Letters, Vol. 119, Issue 5; ISSN 0031-9007
- Publisher:
- American Physical Society (APS)Copyright Statement
- Country of Publication:
- United States
- Language:
- English
Web of Science
Total Absorption Spectroscopy
|
journal | April 2018 |
Review on the progress in nuclear fission—experimental methods and theoretical descriptions
|
journal | September 2018 |
Large Impact of the Decay of Niobium Isomers on the Reactor ν ¯ e Summation Calculations
|
journal | January 2019 |
First-forbidden transitions in the reactor anomaly | text | January 2019 |
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