Nonequilibrium Pair Breaking in Ba(Fe1-xCox)2As2 Superconductors: Evidence for Formation of a Photoinduced Excitonic State

Yang, X.; Luo, L.; Mootz, M.; Patz, A.; Bud’ko, S. L.; Canfield, P. C.; Perakis, I. E.; Wang, J.

doi:10.1103/PhysRevLett.121.267001

Title: Nonequilibrium Pair Breaking in $Ba ({Fe}_{1 - x} {Co}_{x})_{2} {As}_{2}$ Superconductors: Evidence for Formation of a Photoinduced Excitonic State

Journal Article · 26 December 2018 · Physical Review Letters

DOI: https://doi.org/10.1103/PhysRevLett.121.267001 · OSTI ID:1492059

Yang, X. ^[1]; Luo, L. ^[1]; Mootz, M. ^[2]; Patz, A. ^[1]; Bud’ko, S. L. ^[1]; Canfield, P. C. ^[1]; Perakis, I. E. ^[2]; Wang, J. ^[1]

Ames Lab. and Iowa State Univ., Ames, IA (United States). Dept. of Physics and Astronomy
Univ. of Alabama, Birmingham, AL (United States). Dept. of Physics

Ultrafast terahertz (THz) pump-probe spectroscopy reveals an unusual out-of-equilibrium Cooper pair nonlinear dynamics and a nonequilibrium state driven by femtosecond (fs) photoexcitation of superconductivity (SC) in iron pnictides. Following fast SC quench via hot-phonon scattering, a second, abnormally slow (many hundreds of picoseconds), SC quench regime is observed prior to any recovery. Importantly, a nonlinear pump fluence dependence is identified for this remarkably long prebottleneck dynamics that are sensitive to both doping and temperature. Here, using quantum kinetic modeling we argue that the buildup of excitonic interpocket correlation between electron-hole (e-h) quasiparticles (QP) quenches SC after fs photoexcitation leading to a long-lived, many-QP excitonic state.

View Accepted Manuscript (DOE)

View Accepted Manuscript (Publisher)

Cite

Export

Save

Research Organization:: Ames Laboratory (AMES), Ames, IA (United States); Univ. of Alabama, Birmingham, AL (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: W911NF-15-1-0135; SC0019137; AC02-07CH11358

OSTI ID:: 1492059

Alternate ID(s):: OSTI ID: 1488904; OSTI ID: 1971747

Report Number(s):: IS-J-9790

Journal Information:: Physical Review Letters, Vol. 121, Issue 26; ISSN 0031-9007

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

Citation Metrics:

Cited by: 25 works

Citation information provided by
Web of Science

References (42)

Spin excitations in the excitonic spin-density-wave state of the iron pnictides Brydon, P. M. R.; Timm, C. arXiv https://doi.org/10.48550/arxiv.0909.1222	text	January 2009
Measurement of Recombination Lifetimes in Superconductors Rothwarf, Allen; Taylor, B. N. Physical Review Letters, Vol. 19, Issue 1 https://doi.org/10.1103/PhysRevLett.19.27	journal	July 1967
Energy-Gap Dynamics of Superconducting NbN Thin Films Studied by Time-Resolved Terahertz Spectroscopy Beck, M.; Klammer, M.; Lang, S. Physical Review Letters, Vol. 107, Issue 17 https://doi.org/10.1103/PhysRevLett.107.177007	journal	October 2011
Excitons and Plasmons in Superconductors Bardasis, A.; Schrieffer, J. R. Physical Review, Vol. 121, Issue 4 https://doi.org/10.1103/PhysRev.121.1050	journal	February 1961
Light-Induced Superconductivity in a Stripe-Ordered Cuprate Fausti, D.; Tobey, R. I.; Dean, N. Science, Vol. 331, Issue 6014 https://doi.org/10.1126/science.1197294	journal	January 2011
Bose condensation in an attractive fermion gas: From weak to strong coupling superconductivity Nozi�res, P.; Schmitt-Rink, S. Journal of Low Temperature Physics, Vol. 59, Issue 3-4 https://doi.org/10.1007/BF00683774	journal	May 1985
Reversible modulation and ultrafast dynamics of terahertz resonances in strongly photoexcited metamaterials Chatzakis, I.; Luo, L.; Wang, J. Physical Review B, Vol. 86, Issue 12 https://doi.org/10.1103/PhysRevB.86.125110	journal	September 2012
Correlating quasiparticle excitations with quantum femtosecond magnetism in photoexcited nonequilibrium states of insulating antiferromagnetic manganites Lingos, P. C.; Patz, A.; Li, T. Physical Review B, Vol. 95, Issue 22 https://doi.org/10.1103/PhysRevB.95.224432	journal	June 2017
Iron-Based Layered Superconductor La[O _1- _x F _x ]FeAs ( x = 0.05−0.12) with T _c = 26 K Kamihara, Yoichi; Watanabe, Takumi; Hirano, Masahiro Journal of the American Chemical Society, Vol. 130, Issue 11 https://doi.org/10.1021/ja800073m	journal	March 2008
Pair-Breaking and Superconducting State Recovery Dynamics in M g B 2 Demsar, J.; Averitt, R. D.; Taylor, A. J. Physical Review Letters, Vol. 91, Issue 26 https://doi.org/10.1103/PhysRevLett.91.267002	journal	December 2003
Broadband terahertz generation from metamaterials Luo, Liang; Chatzakis, Ioannis; Wang, Jigang arXiv https://doi.org/10.48550/arxiv.1402.5203	text	January 2014
Ultrafast softening in InMnAs Wang, J.; Khodaparast, G. A.; Kono, J. Physica E: Low-dimensional Systems and Nanostructures, Vol. 20, Issue 3-4 https://doi.org/10.1016/j.physe.2003.08.048	journal	January 2004
Semiconductor Quantum Optics Kira, Mackillo; Koch, Stephan W. Cambridge University Press https://doi.org/10.1017/CBO9781139016926	book	January 2011
Pair-excitation energetics of highly correlated many-body states Mootz, M.; Kira, M.; Koch, S. W. arXiv https://doi.org/10.48550/arxiv.1307.7599	text	January 2013
Spin excitations in the excitonic spin-density-wave state of the iron pnictides Brydon, P. M. R.; Timm, C. Physical Review B, Vol. 80, Issue 17 https://doi.org/10.1103/PhysRevB.80.174401	journal	November 2009
Kinetics of a Superconductor Excited with a Femtosecond Optical Pulse Kabanov, V. V.; Demsar, J.; Mihailovic, D. Physical Review Letters, Vol. 95, Issue 14 https://doi.org/10.1103/PhysRevLett.95.147002	journal	September 2005
Ultrafast transient generation of spin-density-wave order in the normal state of BaFe2As2 driven by coherent lattice vibrations Kim, K. W.; Pashkin, A.; Schäfer, H. Nature Materials, Vol. 11, Issue 6 https://doi.org/10.1038/nmat3294	journal	April 2012
Electrodynamics of electron-doped iron pnictide superconductors: Normal-state properties Barišić, N.; Wu, D.; Dressel, M. Physical Review B, Vol. 82, Issue 5 https://doi.org/10.1103/PhysRevB.82.054518	journal	August 2010
Critical speeding up of nonequilibrium electronic relaxation near nematic phase transition in unstrained Ba( Fe 1 − x Co x ) 2 As 2 Patz, A.; Li, T.; Luo, L. Physical Review B, Vol. 95, Issue 16 https://doi.org/10.1103/PhysRevB.95.165122	journal	April 2017
Ultrafast terahertz snapshots of excitonic Rydberg states and electronic coherence in an organometal halide perovskite Luo, Liang; Men, Long; Liu, Zhaoyu Nature Communications, Vol. 8, Issue 1 https://doi.org/10.1038/ncomms15565	journal	June 2017
Ultrafast transient generation of spin-densitywave order in the normal state of BaFe2As2 driven by coherent lattice vibrations Kim, K. W.; Pashkin, A.; Schäfer, H. arXiv https://doi.org/10.48550/arxiv.1207.3987	text	January 2012
Theory of nonequilibrium dynamics of multiband superconductors Akbari, Alireza; Schnyder, Andreas P.; Manske, Dirk EPL (Europhysics Letters), Vol. 101, Issue 1 https://doi.org/10.1209/0295-5075/101/17002	journal	January 2013
Ultrafast terahertz probes of interacting dark excitons in chirality-specific semiconducting single-walled carbon nanotubes Luo, Liang; Chatzakis, Ioannis; Patz, Aaron arXiv https://doi.org/10.48550/arxiv.1406.6135	text	January 2014
Ultrafast observation of critical nematic fluctuations and giant magnetoelastic coupling in iron pnictides Patz, Aaron; Li, Tianqi; Ran, Sheng Nature Communications, Vol. 5, Issue 1 https://doi.org/10.1038/ncomms4229	journal	February 2014
Superconductivity and spin-density waves in multiband metals Vorontsov, A. B.; Vavilov, M. G.; Chubukov, A. V. Physical Review B, Vol. 81, Issue 17 https://doi.org/10.1103/PhysRevB.81.174538	journal	May 2010
Energy-gap dynamics of superconducting NbN thin films studied by time-resolved terahertz spectroscopy Beck, M.; Klammer, M.; Lang, S. arXiv https://doi.org/10.48550/arxiv.1102.5616	text	January 2011
Pair-excitation energetics of highly correlated many-body states Mootz, M.; Kira, M.; Koch, S. W. New Journal of Physics, Vol. 15, Issue 9 https://doi.org/10.1088/1367-2630/15/9/093040	journal	September 2013
Terahertz-light quantum tuning of a metastable emergent phase hidden by superconductivity Yang, X.; Vaswani, C.; Sundahl, C. Nature Materials, Vol. 17, Issue 7 https://doi.org/10.1038/s41563-018-0096-3	journal	June 2018
FeAs-Based Superconductivity: A Case Study of the Effects of Transition Metal Doping on BaFe ₂ As ₂ Canfield, Paul C.; Bud'ko, Sergey L. Annual Review of Condensed Matter Physics, Vol. 1, Issue 1 https://doi.org/10.1146/annurev-conmatphys-070909-104041	journal	August 2010
Theory of the Anomalous Skin Effect in Normal and Superconducting Metals Mattis, D. C.; Bardeen, J. Physical Review, Vol. 111, Issue 2 https://doi.org/10.1103/PhysRev.111.412	journal	July 1958
Femtosecond switching of magnetism via strongly correlated spin–charge quantum excitations Li, Tianqi; Patz, Aaron; Mouchliadis, Leonidas Nature, Vol. 496, Issue 7443 https://doi.org/10.1038/nature11934	journal	April 2013
Ultrafast optical spectroscopy of strongly correlated materials and high-temperature superconductors: a non-equilibrium approach Giannetti, Claudio; Capone, Massimo; Fausti, Daniele Advances in Physics, Vol. 65, Issue 2 https://doi.org/10.1080/00018732.2016.1194044	journal	March 2016
Dynamics of exciton formation for near band-gap excitations Siantidis, K.; Axt, V. M.; Kuhn, T. Physical Review B, Vol. 65, Issue 3 https://doi.org/10.1103/PhysRevB.65.035303	journal	December 2001
FeAs-based superconductivity: a case study of the effects of transition metal doping on BaFe2As2 Canfield, Paul C.; Bud'ko, Sergey L. arXiv https://doi.org/10.48550/arxiv.1002.0858	text	January 2010
Coherent dynamics and pump-probe spectra of BCS superconductors Papenkort, T.; Axt, V. M.; Kuhn, T. Physical Review B, Vol. 76, Issue 22 https://doi.org/10.1103/PhysRevB.76.224522	journal	December 2007
Competing order and nature of the pairing state in the iron pnictides Fernandes, Rafael M.; Schmalian, Jörg Physical Review B, Vol. 82, Issue 1 https://doi.org/10.1103/PhysRevB.82.014521	journal	July 2010
Quantum mechanical kinetic equations Wyld, H. W.; Fried, Burton D. Annals of Physics, Vol. 23, Issue 3 https://doi.org/10.1016/0003-4916(63)90260-4	journal	September 1963
Ultrafast Terahertz Probes of Interacting Dark Excitons in Chirality-Specific Semiconducting Single-Walled Carbon Nanotubes Luo, Liang; Chatzakis, Ioannis; Patz, Aaron Physical Review Letters, Vol. 114, Issue 10 https://doi.org/10.1103/PhysRevLett.114.107402	journal	March 2015
Ultrafast observation of critical nematic fluctuations and giant magnetoelastic coupling in iron pnictides Patz, Aaron; Li, Tianqi; Ran, Sheng arXiv https://doi.org/10.48550/arxiv.1402.4890	text	January 2014
Broadband terahertz generation from metamaterials Luo, Liang; Chatzakis, Ioannis; Wang, Jigang Nature Communications, Vol. 5, Article No. 3055 https://doi.org/10.1038/ncomms4055	journal	January 2014
Competing order and nature of the pairing state in the iron pnictides Fernandes, Rafael M.; Schmalian, Jörg arXiv https://doi.org/10.48550/arxiv.1005.2437	text	January 2010
Non-thermal separation of electronic and structural orders in a persisting charge density wave Porer, M.; Leierseder, U.; Ménard, J. -M. Nature Materials, Vol. 13, Issue 9 https://doi.org/10.1038/nmat4042	journal	July 2014

Cited By (6)

Terahertz-light quantum tuning of a metastable emergent phase hidden by superconductivity Yang, X.; Vaswani, C.; Sundahl, C. Nature Materials, Vol. 17, Issue 7 https://doi.org/10.1038/s41563-018-0096-3	journal	June 2018
Light control of surface–bulk coupling by terahertz vibrational coherence in a topological insulator Yang, Xu; Luo, Liang; Vaswani, Chirag npj Quantum Materials, Vol. 5, Issue 1 https://doi.org/10.1038/s41535-020-0215-7	journal	February 2020
Ultrafast manipulation of topologically enhanced surface transport driven by mid-infrared and terahertz pulses in Bi2Se3 Luo, L.; Yang, X.; Liu, X. Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-08559-6	journal	February 2019
Accelerating terahertz all-optical modulation by hot carriers effects of silver nanorods in PVA film Yu, Jian-Ping; Chen, Sai; Fan, Fei AIP Advances, Vol. 9, Issue 7 https://doi.org/10.1063/1.5098386	journal	July 2019
Lightwave-driven gapless superconductivity and forbidden quantum beats by terahertz symmetry breaking Yang, X.; Vaswani, C.; Sundahl, C. Nature Photonics, Vol. 13, Issue 10 https://doi.org/10.1038/s41566-019-0470-y	journal	July 2019
Higgs Oscillations in time-resolved Optical Conductivity Kumar, A.; Kemper, A. F. arXiv https://doi.org/10.48550/arxiv.1902.09549	text	January 2019

Similar Records

Femtosecond x-ray scattering study of ultrafast photoinduced structural dynamics in solvated

[Co (terpy)_{2}]^{2 +}

Journal Article · 2016 · Physical Review Letters · OSTI ID:1335954

Biasin, Elisa; van Driel, Tim Brandt; Kjær, Kasper S.; +30 more

Unconventional Charge Density Wave Order in the Pnictide Superconductor

Ba ({Ni}_{1 - x} {Co}_{x})_{2} {As}_{2}

Journal Article · 2019 · Physical Review Letters · OSTI ID:1526465

Lee, Sangjun; de la Peña, Gilberto; Sun, Stella X. -L.; +10 more

Structural and Magnetic Phase Transitions near Optimal Superconductivity in

{{BaFe}_{2} ({As}_{1 - x} P_{x})}_{2}

Journal Article · 2015 · Physical Review Letters · OSTI ID:1391767

Hu, Ding; Lu, Xingye; Zhang, Wenliang; +17 more

Related Subjects

75 CONDENSED MATTER PHYSICS
SUPERCONDUCTIVITY AND SUPERFLUIDITY

Title: Nonequilibrium Pair Breaking in Ba ( Fe 1 - x Co x ) 2 As 2 Superconductors: Evidence for Formation of a Photoinduced Excitonic State

Citation Formats

References (42)

Cited By (6)

Similar Records

Related Subjects

Title: Nonequilibrium Pair Breaking in $Ba ({Fe}_{1 - x} {Co}_{x})_{2} {As}_{2}$ Superconductors: Evidence for Formation of a Photoinduced Excitonic State