Flexible and stable high-energy lithium-sulfur full batteries with only 100% oversized lithium
Abstract
Lightweight and flexible energy storage devices are urgently needed to persistently power wearable devices, and lithium-sulfur batteries are promising technologies due to their low mass densities and high theoretical capacities. Here we report a flexible and high-energy lithium-sulfur full battery device with only 100% oversized lithium, enabled by rationally designed copper-coated and nickel-coated carbon fabrics as excellent hosts for lithium and sulfur, respectively. These metallic carbon fabrics endow mechanical flexibility, reduce local current density of the electrodes, and, more importantly, significantly stabilize the electrode materials to reach remarkable Coulombic efficiency of >99.89% for a lithium anode and >99.82% for a sulfur cathode over 400 half-cell charge-discharge cycles. Furthermore, the assembled lithium-sulfur full battery provides high areal capacity (3 mA h cm–2), high cell energy density (288 W h kg–1 and 360 W h L–1), excellent cycling stability (260 cycles), and remarkable bending stability at a small radius of curvature (<1 mm).
- Authors:
-
[3];
[1]
- The Hong Kong Polytechnic Univ., Hong Kong SAR (China)
- Stanford Univ., Stanford, CA (United States)
- Okinawa Institute of Science and Technology Graduate Univ., Okinawa (Japan)
- Stanford Univ., Stanford, CA (United States); SLAC National Accelerator Lab., Menlo Park, CA (United States)
- Publication Date:
- Research Org.:
- SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1490644
- Grant/Contract Number:
- AC02-76SF00515; N_PolyU528/16
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Communications
- Additional Journal Information:
- Journal Volume: 9; Journal Issue: 1; Journal ID: ISSN 2041-1723
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 25 ENERGY STORAGE
Citation Formats
Chang, Jian, Shang, Jian, Sun, Yongming, Ono, Luis K., Wang, Dongrui, Ma, Zhijun, Huang, Qiyao, Chen, Dongdong, Liu, Guoqiang, Cui, Yi, Qi, Yabing, and Zheng, Zijian. Flexible and stable high-energy lithium-sulfur full batteries with only 100% oversized lithium. United States: N. p., 2018.
Web. doi:10.1038/s41467-018-06879-7.
Chang, Jian, Shang, Jian, Sun, Yongming, Ono, Luis K., Wang, Dongrui, Ma, Zhijun, Huang, Qiyao, Chen, Dongdong, Liu, Guoqiang, Cui, Yi, Qi, Yabing, & Zheng, Zijian. Flexible and stable high-energy lithium-sulfur full batteries with only 100% oversized lithium. United States. https://doi.org/10.1038/s41467-018-06879-7
Chang, Jian, Shang, Jian, Sun, Yongming, Ono, Luis K., Wang, Dongrui, Ma, Zhijun, Huang, Qiyao, Chen, Dongdong, Liu, Guoqiang, Cui, Yi, Qi, Yabing, and Zheng, Zijian. Fri .
"Flexible and stable high-energy lithium-sulfur full batteries with only 100% oversized lithium". United States. https://doi.org/10.1038/s41467-018-06879-7. https://www.osti.gov/servlets/purl/1490644.
@article{osti_1490644,
title = {Flexible and stable high-energy lithium-sulfur full batteries with only 100% oversized lithium},
author = {Chang, Jian and Shang, Jian and Sun, Yongming and Ono, Luis K. and Wang, Dongrui and Ma, Zhijun and Huang, Qiyao and Chen, Dongdong and Liu, Guoqiang and Cui, Yi and Qi, Yabing and Zheng, Zijian},
abstractNote = {Lightweight and flexible energy storage devices are urgently needed to persistently power wearable devices, and lithium-sulfur batteries are promising technologies due to their low mass densities and high theoretical capacities. Here we report a flexible and high-energy lithium-sulfur full battery device with only 100% oversized lithium, enabled by rationally designed copper-coated and nickel-coated carbon fabrics as excellent hosts for lithium and sulfur, respectively. These metallic carbon fabrics endow mechanical flexibility, reduce local current density of the electrodes, and, more importantly, significantly stabilize the electrode materials to reach remarkable Coulombic efficiency of >99.89% for a lithium anode and >99.82% for a sulfur cathode over 400 half-cell charge-discharge cycles. Furthermore, the assembled lithium-sulfur full battery provides high areal capacity (3 mA h cm–2), high cell energy density (288 W h kg–1 and 360 W h L–1), excellent cycling stability (260 cycles), and remarkable bending stability at a small radius of curvature (<1 mm).},
doi = {10.1038/s41467-018-06879-7},
journal = {Nature Communications},
number = 1,
volume = 9,
place = {United States},
year = {Fri Oct 26 00:00:00 EDT 2018},
month = {Fri Oct 26 00:00:00 EDT 2018}
}
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Figures / Tables:
Fig. 1: Schematic of the fabrication process and design principle for the electrodes. a To simultaneously endow mechanical durability and cycling stability of Li-S batteries, chemically stable and highly conductive Cu or Ni thin layers are uniformly coated onto carbon fabrics (CuCF or NiCF) via a scalable polymer-assisted metal depositionmore »
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journal, January 2020
- Lu, Ruichao; Cheng, Meng; Mao, Lijuan
- EcoMat, Vol. 2, Issue 1
A review of rechargeable batteries for portable electronic devices
journal, March 2019
- Liang, Yeru; Zhao, Chen‐Zi; Yuan, Hong
- InfoMat, Vol. 1, Issue 1
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3D CNTs Networks Enable MnO 2 Cathodes with High Capacity and Superior Rate Capability for Flexible Rechargeable Zn–MnO 2 Batteries
journal, September 2019
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journal, July 2019
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- Nature Communications, Vol. 10, Issue 1
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Rational design of spontaneous reactions for protecting porous lithium electrodes in lithium–sulfur batteries
journal, July 2019
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- Nature Communications, Vol. 10, Issue 1
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