Ultrafast manipulation of mirror domain walls in a charge density wave

Zong, Alfred; Shen, Xiaozhe; Kogar, Anshul; Ye, Linda; Marks, Carolyn; Chowdhury, Debanjan; Rohwer, Timm; Freelon, Byron; Weathersby, Stephen; Li, Renkai; Yang, Jie; Checkelsky, Joseph; Wang, Xijie; Gedik, Nuh

doi:10.1126/sciadv.aau5501

Title: Ultrafast manipulation of mirror domain walls in a charge density wave

Journal Article · 19 October 2018 · Science Advances

DOI: https://doi.org/10.1126/sciadv.aau5501 · OSTI ID:1490444

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^[2];

^[1];

^[1]; Marks, Carolyn ^[3];

^[1]; Rohwer, Timm ^[1]; Freelon, Byron ^[1]; Weathersby, Stephen ^[2];

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^[2]; Checkelsky, Joseph ^[1]; Wang, Xijie ^[2];

^[1]

Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States). Dept. of Physics
SLAC National Accelerator Lab., Menlo Park, CA (United States)
Harvard Univ., Cambridge, MA (United States). Center for Nanoscale Systems

Domain walls (DWs) are singularities in an ordered medium that often host exotic phenomena such as charge ordering, insulator-metal transition, or superconductivity. The ability to locally write and erase DWs is highly desirable, as it allows one to design material functionality by patterning DWs in specific configurations. We demonstrate such capability at room temperature in a charge density wave (CDW), a macroscopic condensate of electrons and phonons, in ultrathin 1T-TaS₂. A single femtosecond light pulse is shown to locally inject or remove mirror DWs in the CDW condensate, with probabilities tunable by pulse energy and temperature. Using time-resolved electron diffraction, we are able to simultaneously track anti-synchronized CDW amplitude oscillations from both the lattice and the condensate, where photoinjected DWs lead to a red-shifted frequency. Our demonstration of reversible DW manipulation may pave new ways for engineering correlated material systems with light.

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Research Organization:: Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States); SLAC National Accelerator Lab., Menlo Park, CA (United States)

Sponsoring Organization:: Gordon and Betty Moore Foundation (United States); National Science Foundation (NSF) (United States); USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

Grant/Contract Number:: AC02-05CH11231; AC02-76SF00515

OSTI ID:: 1490444

Journal Information:: Science Advances, Journal Name: Science Advances Journal Issue: 10 Vol. 4; ISSN 2375-2548

Publisher:: AAASCopyright Statement

Country of Publication:: United States

Language:: English

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