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Title: Megafilament in air formed by self-guided terawatt long-wavelength infrared laser

Abstract

The diffraction-compensated propagation of high-power laser beams in air could open up new opportunities for atmospheric applications such as remote stand-off detection, long-range projection of high-energy laser pulses and free-space communications. Here, we experimentally demonstrate that a self-guided terawatt picosecond CO2 laser beam forms in air a single centimetre-scale-diameter megafilament that, in comparison with a short-wavelength laser filament, has four orders of magnitude larger cross-section and guides many joules of pulse energy over multiple Rayleigh distances at a clamped intensity of ~1012 W cm–2. We discover that this megafilament arises from the balance between self-focusing, diffraction and defocusing caused by free carriers generated via many-body Coulomb-induced ionization that effectively decrease the molecular polarizability during the long-wavelength laser pulse. Furthermore, modelling reveals that this guiding scheme may enable transport of high-power picosecond infrared pulses over many kilometres in the 8–14 μm atmospheric transmission window.

Authors:
ORCiD logo [1];  [1];  [2];  [2];  [3];  [3];  [3];  [4];  [3];  [1];  [1]
  1. Univ. of California, Los Angeles, CA (United States)
  2. Brookhaven National Lab. (BNL), Upton, NY (United States)
  3. Univ. of Arizona, Tucson, AZ (United States)
  4. Univ. of Arizona, Tucson, AZ (United States); Philipps-Univ., Marburg (Germany)
Publication Date:
Research Org.:
Brookhaven National Lab. (BNL), Upton, NY (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Nuclear Physics (NP)
OSTI Identifier:
1489355
Report Number(s):
BNL-210833-2018-JAAM
Journal ID: ISSN 1749-4885
Grant/Contract Number:  
SC0012704
Resource Type:
Accepted Manuscript
Journal Name:
Nature Photonics
Additional Journal Information:
Journal Volume: 13; Journal Issue: 1; Journal ID: ISSN 1749-4885
Publisher:
Nature Publishing Group
Country of Publication:
United States
Language:
English
Subject:
43 PARTICLE ACCELERATORS

Citation Formats

Tochitsky, Sergei, Welch, Eric, Polyanskiy, Mikhail, Pogorelsky, Igor, Panagiotopoulos, Paris, Kolesik, Miroslav, Wright, Ewan M., Koch, Stephan W., Moloney, Jerome V., Pigeon, Jeremy, and Joshi, Chan. Megafilament in air formed by self-guided terawatt long-wavelength infrared laser. United States: N. p., 2018. Web. doi:10.1038/s41566-018-0315-0.
Tochitsky, Sergei, Welch, Eric, Polyanskiy, Mikhail, Pogorelsky, Igor, Panagiotopoulos, Paris, Kolesik, Miroslav, Wright, Ewan M., Koch, Stephan W., Moloney, Jerome V., Pigeon, Jeremy, & Joshi, Chan. Megafilament in air formed by self-guided terawatt long-wavelength infrared laser. United States. https://doi.org/10.1038/s41566-018-0315-0
Tochitsky, Sergei, Welch, Eric, Polyanskiy, Mikhail, Pogorelsky, Igor, Panagiotopoulos, Paris, Kolesik, Miroslav, Wright, Ewan M., Koch, Stephan W., Moloney, Jerome V., Pigeon, Jeremy, and Joshi, Chan. Fri . "Megafilament in air formed by self-guided terawatt long-wavelength infrared laser". United States. https://doi.org/10.1038/s41566-018-0315-0. https://www.osti.gov/servlets/purl/1489355.
@article{osti_1489355,
title = {Megafilament in air formed by self-guided terawatt long-wavelength infrared laser},
author = {Tochitsky, Sergei and Welch, Eric and Polyanskiy, Mikhail and Pogorelsky, Igor and Panagiotopoulos, Paris and Kolesik, Miroslav and Wright, Ewan M. and Koch, Stephan W. and Moloney, Jerome V. and Pigeon, Jeremy and Joshi, Chan},
abstractNote = {The diffraction-compensated propagation of high-power laser beams in air could open up new opportunities for atmospheric applications such as remote stand-off detection, long-range projection of high-energy laser pulses and free-space communications. Here, we experimentally demonstrate that a self-guided terawatt picosecond CO2 laser beam forms in air a single centimetre-scale-diameter megafilament that, in comparison with a short-wavelength laser filament, has four orders of magnitude larger cross-section and guides many joules of pulse energy over multiple Rayleigh distances at a clamped intensity of ~1012 W cm–2. We discover that this megafilament arises from the balance between self-focusing, diffraction and defocusing caused by free carriers generated via many-body Coulomb-induced ionization that effectively decrease the molecular polarizability during the long-wavelength laser pulse. Furthermore, modelling reveals that this guiding scheme may enable transport of high-power picosecond infrared pulses over many kilometres in the 8–14 μm atmospheric transmission window.},
doi = {10.1038/s41566-018-0315-0},
journal = {Nature Photonics},
number = 1,
volume = 13,
place = {United States},
year = {2018},
month = {12}
}

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Works referenced in this record:

The rotational and rotation-vibrational Raman spectra of 14N2, 14N15N and 15N2
journal, April 1974


Kilometer range filamentation
journal, January 2013

  • Durand, Magali; Houard, Aurélien; Prade, Bernard
  • Optics Express, Vol. 21, Issue 22
  • DOI: 10.1364/OE.21.026836

Laser-induced water condensation in air
journal, May 2010

  • Rohwetter, Philipp; Kasparian, Jérôme; Stelmaszczyk, Kamil
  • Nature Photonics, Vol. 4, Issue 7
  • DOI: 10.1038/nphoton.2010.115

Long-range self-channeling of infrared laser pulses in air: a new propagation regime without ionization
journal, August 2004


Fifteen terawatt picosecond CO_2 laser system
journal, January 2010

  • Haberberger, D.; Tochitsky, S.; Joshi, C.
  • Optics Express, Vol. 18, Issue 17
  • DOI: 10.1364/OE.18.017865

Mid-infrared laser filaments in the atmosphere
journal, February 2015

  • Mitrofanov, A. V.; Voronin, A. A.; Sidorov-Biryukov, D. A.
  • Scientific Reports, Vol. 5, Issue 1
  • DOI: 10.1038/srep08368

Nonlinear optical pulse propagation simulation: From Maxwell’s to unidirectional equations
journal, September 2004


Toward directed energy planetary defense
journal, February 2014


Femtosecond filamentation in transparent media
journal, March 2007


Microwave guiding in air by a cylindrical filament array waveguide
journal, March 2008

  • Châteauneuf, M.; Payeur, S.; Dubois, J.
  • Applied Physics Letters, Vol. 92, Issue 9
  • DOI: 10.1063/1.2889501

Research and Industry News
journal, January 2017

  • Daukantas, Patricia; Michaud, Sarah; Wills, Stewart
  • Optics and Photonics News, Vol. 28, Issue 12
  • DOI: 10.1364/OPN.28.12.000008

Measurements of the nonlinear refractive index of air, N_2, and O_2 at 10 μm using four-wave mixing
journal, January 2016

  • Pigeon, J. J.; Tochitsky, S. Ya.; Welch, E. C.
  • Optics Letters, Vol. 41, Issue 17
  • DOI: 10.1364/OL.41.003924

Simulations of 10  μm filaments in a realistically modeled atmosphere
journal, January 2016

  • Panagiotopoulos, Paris; Schuh, Kolja; Kolesik, Miroslav
  • Journal of the Optical Society of America B, Vol. 33, Issue 10
  • DOI: 10.1364/JOSAB.33.002154

Dynamics of CO 2 laser pulse filamentation in air influenced by spectrally selective molecular absorption
journal, January 2014

  • Geints, Yuri E.; Zemlyanov, Alexander A.
  • Applied Optics, Vol. 53, Issue 25
  • DOI: 10.1364/AO.53.005641

Picosecond pulse amplification in isotopic CO_2 active medium
journal, January 2011

  • Polyanskiy, Mikhail N.; Pogorelsky, Igor V.; Yakimenko, Vitaly
  • Optics Express, Vol. 19, Issue 8
  • DOI: 10.1364/OE.19.007717

Picosecond ionization dynamics in femtosecond filaments at high pressures
journal, January 2017


Efficient shortening of self-chirped picosecond pulses in a high-power CO_2 amplifier
journal, January 2001

  • Tochitsky, S. Ya.; Filip, C.; Narang, R.
  • Optics Letters, Vol. 26, Issue 11
  • DOI: 10.1364/OL.26.000813

Long-distance remote laser-induced breakdown spectroscopy using filamentation in air
journal, November 2004

  • Stelmaszczyk, Kamil; Rohwetter, Philipp; Méjean, Guillaume
  • Applied Physics Letters, Vol. 85, Issue 18
  • DOI: 10.1063/1.1812843

Filamentation of mid-IR pulses in ambient air in the vicinity of molecular resonances
journal, January 2018

  • Shumakova, V.; Ališauskas, S.; Malevich, P.
  • Optics Letters, Vol. 43, Issue 9
  • DOI: 10.1364/OL.43.002185

Wavelength-dependent spectral extinction of atmospheric aerosols
journal, January 1984


Nonlinear refractive index of optical crystals
journal, February 1989


Self-Channeling of High-Power Long-Wave Infrared Pulses in Atomic Gases
journal, February 2017


Free-space nitrogen gas laser driven by a femtosecond filament
journal, September 2012

  • Kartashov, Daniil; Ališauskas, Skirmantas; Andriukaitis, Giedrius
  • Physical Review A, Vol. 86, Issue 3
  • DOI: 10.1103/PhysRevA.86.033831

Nonequilibrium evolution of strong-field anisotropic ionized electrons towards a delayed plasma-state
journal, January 2012

  • Pasenow, B.; Moloney, J. V.; Koch, S. W.
  • Optics Express, Vol. 20, Issue 3
  • DOI: 10.1364/OE.20.002310

The HITRAN2012 molecular spectroscopic database
journal, November 2013

  • Rothman, L. S.; Gordon, I. E.; Babikov, Y.
  • Journal of Quantitative Spectroscopy and Radiative Transfer, Vol. 130, p. 4-50
  • DOI: 10.1016/j.jqsrt.2013.07.002

Practitioner’s guide to laser pulse propagation models and simulation: Numerical implementation and practical usage of modern pulse propagation models
journal, November 2011

  • Couairon, A.; Brambilla, E.; Corti, T.
  • The European Physical Journal Special Topics, Vol. 199, Issue 1
  • DOI: 10.1140/epjst/e2011-01503-3

Femtosecond ultraviolet laser pulse induced lightning discharges in gases
journal, March 1995

  • Xin Miao Zhao, ; Diels, J. -C.
  • IEEE Journal of Quantum Electronics, Vol. 31, Issue 3
  • DOI: 10.1109/3.364418

Single and multiple filamentation of multi-terawatt CO_2-laser pulses in air: numerical simulations
journal, January 2014

  • Geints, Y. E.; Zemlyanov, A. A.
  • Journal of the Optical Society of America B, Vol. 31, Issue 4
  • DOI: 10.1364/JOSAB.31.000788

Chirped-pulse amplification in a CO_2 laser
journal, January 2015

  • Polyanskiy, Mikhail N.; Babzien, Marcus; Pogorelsky, Igor V.
  • Optica, Vol. 2, Issue 8
  • DOI: 10.1364/OPTICA.2.000675

Self-channeling of high-peak-power femtosecond laser pulses in air
journal, January 1995


Influence of many-body interactions during the ionization of gases by short intense optical pulses
journal, March 2014


Superfilamentation in Air
journal, June 2014


Experimental study of the third-order nonlinearity of atomic and molecular gases using 10-μm laser pulses
journal, April 2018


Laser-induced water condensation in air
conference, May 2011

  • Kasparian, Jerome; Rohwetter, Philipp; Stelmaszczyk, Kamil
  • 12th European Quantum Electronics Conference CLEO EUROPE/EQEC, 2011 Conference on Lasers and Electro-Optics Europe and 12th European Quantum Electronics Conference (CLEO EUROPE/EQEC)
  • DOI: 10.1109/cleoe.2011.5943024

Research and Industry News
journal, January 2018

  • Daukantas, Patricia; Michaud, Sarah; Wills, Stewart
  • Optics and Photonics News, Vol. 29, Issue 3
  • DOI: 10.1364/opn.29.3.000008

Research and Industry News
journal, January 2019

  • Daukantas, Patricia; Michaud, Sarah; Wills, Stewart
  • Optics and Photonics News, Vol. 30, Issue 7
  • DOI: 10.1364/opn.30.7.000008

Research and Industry News
journal, January 2016

  • Daukantas, Patricia; Michaud, Sarah; Wills, Stewart
  • Optics and Photonics News, Vol. 27, Issue 7
  • DOI: 10.1364/opn.27.7.000010

Research and Industry News
journal, January 2017

  • Daukantas, Patricia; Michaud, Sarah; Wills, Stewart
  • Optics and Photonics News, Vol. 28, Issue 3
  • DOI: 10.1364/opn.28.3.000008

Research and Industry News
journal, January 2016

  • Daukantas, Patricia; Michaud, Sarah; Wills, Stewart
  • Optics and Photonics News, Vol. 27, Issue 5
  • DOI: 10.1364/opn.27.5.000008

Mid-infrared laser filaments in the atmosphere
preprint, January 2014


Works referencing / citing this record:

Filamentation in Atmospheric Air with Tunable 1100–2400 nm Near-Infrared Femtosecond Laser Source
journal, August 2019

  • O’Connor, Sean P.; Marble, Christopher B.; Nodurft, Dawson T.
  • Scientific Reports, Vol. 9, Issue 1
  • DOI: 10.1038/s41598-019-48542-1

Single-Shot Multi-Stage Damage and Ablation of Silicon by Femtosecond Mid-infrared Laser Pulses
journal, December 2019


Memory effects in the long-wave infrared avalanche ionization of gases: a review of recent progress
journal, May 2019

  • Wright, E. M.; Koch, S. W.; Kolesik, M.
  • Reports on Progress in Physics, Vol. 82, Issue 6
  • DOI: 10.1088/1361-6633/ab1a07

Nonlinear transparency window for ultraintense femtosecond laser pulses in the atmosphere
journal, August 2019


Control of the filament dynamics of 10  µm pulses via designer pulse trains
journal, January 2019

  • Panagiotopoulos, Paris; Kolesik, Miroslav; Koch, Stephan W.
  • Journal of the Optical Society of America B, Vol. 36, Issue 10
  • DOI: 10.1364/josab.36.000g33

Filamentation of long-wave infrared pulses in the atmosphere [Invited]
journal, January 2019

  • Tochitsky, Sergei; Welch, Eric; Panagiotopoulos, Paris
  • Journal of the Optical Society of America B, Vol. 36, Issue 10
  • DOI: 10.1364/josab.36.000g40

Nonlinear rovibrational response in the propagation of long-wavelength infrared pulses and pulse trains
journal, January 2019

  • Rosenow, Phil; Panagiotopoulos, Paris; Kolesik, Miroslav
  • Journal of the Optical Society of America B, Vol. 36, Issue 12
  • DOI: 10.1364/josab.36.003457

Engineering equations for the filamentation collapse distance in lossy, turbulent, nonlinear media
journal, January 2019

  • Stotts, Larry B.; Peñano, Joseph R.; Tellez, Jason A.
  • Optics Express, Vol. 27, Issue 18
  • DOI: 10.1364/oe.27.025126

Molecular quantum wakes for clearing fog
journal, January 2020

  • Schroeder, Malte C.; Larkin, Ilia; Produit, Thomas
  • Optics Express, Vol. 28, Issue 8
  • DOI: 10.1364/oe.389393

Plasma-free water droplet shattering by long-wave infrared ultrashort pulses for efficient fog clearing
journal, January 2020


Molecular Quantum Wakes for Clearing Fog
conference, January 2020

  • Schroeder, Malte C.; Larkin, Ilia; Produit, Thomas
  • The 22nd International Conference on Ultrafast Phenomena 2020
  • DOI: 10.1364/up.2020.tu3a.8

Memory effects in the long-wave infrared avalanche ionization of gases: A review of recent progress
text, January 2018


Table-top high-energy 7 um OPCPA and 260 mJ Ho:YLF pump laser
text, January 2019