Correlated Materials Characterization via Multimodal Chemical and Functional Imaging

Belianinov, Alex; Ievlev, Anton V.; Lorenz, Matthias; Borodinov, Nikolay; Doughty, Benjamin; Kalinin, Sergei V.; Fernández, Facundo M.; Ovchinnikova, Olga S.

doi:10.1021/acsnano.8b07292

Title: Correlated Materials Characterization via Multimodal Chemical and Functional Imaging

Journal Article · 12 November 2018 · ACS Nano

DOI: https://doi.org/10.1021/acsnano.8b07292 · OSTI ID:1489099

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Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Georgia Inst. of Technology and Petit Institute for Biochemistry and Bioscience, Atlanta, GA (United States)

Multimodal chemical imaging simultaneously offers high-resolution chemical and physical information with nanoscale and, in select cases, atomic resolution. By coupling modalities that collect physical and chemical information, we can address scientific problems in biological systems, battery and fuel cell research, catalysis, pharmaceuticals, photovoltaics, medicine, and many others. The combined systems enable the local correlation of material properties with chemical makeup, making fundamental questions of how chemistry and structure drive functionality approachable. In this Review, we present recent progress and offer a perspective for chemical imaging used to characterize a variety of samples by a number of platforms. Specifically, we present cases of infrared and Raman spectroscopies combined with scanning probe microscopy; optical microscopy and mass spectrometry; nonlinear optical microscopy; and, finally, ion, electron, and probe microscopies with mass spectrometry. As a result, we also discuss the challenges associated with the use of data originated by the combinatorial hardware, analysis, and machine learning as well as processing tools necessary for the interpretation of multidimensional data acquired from multimodal studies.

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Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1489099

Journal Information:: ACS Nano, Journal Name: ACS Nano Journal Issue: 12 Vol. 12; ISSN 1936-0851

Publisher:: American Chemical Society (ACS)Copyright Statement

Country of Publication:: United States

Language:: English

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