Nanostructured Metal Hydrides for Hydrogen Storage

Schneemann, Andreas; White, James L.; Kang, ShinYoung; Jeong, Sohee; Wan, Liwen F.; Cho, Eun Seon; Heo, Tae Wook; Prendergast, David; Urban, Jeffrey J.; Wood, Brandon C.; Allendorf, Mark D.; Stavila, Vitalie

doi:10.1021/acs.chemrev.8b00313

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Title: Nanostructured Metal Hydrides for Hydrogen Storage

Journal Article · 01 October 2018 · Chemical Reviews

DOI: https://doi.org/10.1021/acs.chemrev.8b00313 · OSTI ID:1485458

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^[1]; Kang, ShinYoung ^[2]; Jeong, Sohee ^[3];

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^[4]; Heo, Tae Wook ^[2]; Prendergast, David ^[3];

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Sandia National Lab. (SNL-CA), Livermore, CA (United States)
Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Korea Advanced Institute of Science and Technology (KAIST), Daejeon (Republic of Korea)

Knowledge and foundational understanding of phenomena associated with the behavior of materials at the nanoscale is one of the key scientific challenges toward a sustainable energy future. Size reduction from bulk to the nanoscale leads to a variety of exciting and anomalous phenomena due to enhanced surface-to-volume ratio, reduced transport length, and tunable nanointerfaces. Nanostructured metal hydrides are an important class of materials with significant potential for energy storage applications. Hydrogen storage in nanoscale metal hydrides has been recognized as a potentially transformative technology, and the field is now growing steadily due to the ability to tune the material properties more independently and drastically compared to those of their bulk counterparts. The numerous advantages of nanostructured metal hydrides compared to bulk include improved reversibility, altered heats of hydrogen absorption/desorption, nanointerfacial reaction pathways with faster rates, and new surface states capable of activating chemical bonds. This review aims to summarize the progress to date in the area of nanostructured metal hydrides and intends to understand and explain the underpinnings of the innovative concepts and strategies developed over the past decade to tune the thermodynamics and kinetics of hydrogen storage reactions. Furthermore, these recent achievements have the potential to propel further the prospects of tuning the hydride properties at nanoscale, with several promising directions and strategies that could lead to the next generation of solid-state materials for hydrogen storage applications.

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Research Organization:: Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States); Sandia National Laboratories (SNL-CA), Livermore, CA (United States)

Sponsoring Organization:: USDOE; USDOE National Nuclear Security Administration (NNSA)

Grant/Contract Number:: AC04-94AL85000; AC52-07NA27344

OSTI ID:: 1485458

Report Number(s):: LLNL-JRNL--755043; SAND--2018-12080J; 668977

Journal Information:: Chemical Reviews, Journal Name: Chemical Reviews Journal Issue: 22 Vol. 118; ISSN 0009-2665

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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The effects of ball milling and nanometric nickel additive on the hydrogen desorption from lithium borohydride and manganese chloride (3LiBH4+MnCl2) mixture Varin, R. A.; Zbroniec, L. International Journal of Hydrogen Energy, Vol. 35, Issue 8 https://doi.org/10.1016/j.ijhydene.2010.01.137	journal	April 2010
Raman spectroscopic observation of dehydrogenation in ball-milled LiNH2–LiBH4–MgH2 nanoparticles Hattrick-Simpers, Jason R.; Maslar, James E.; Niemann, Michael U. International Journal of Hydrogen Energy, Vol. 35, Issue 12 https://doi.org/10.1016/j.ijhydene.2010.02.101	journal	June 2010
Hydrogen storage properties of spark generated palladium nanoparticles Vons, V. A.; Leegwater, H.; Legerstee, W. J. International Journal of Hydrogen Energy, Vol. 35, Issue 11 https://doi.org/10.1016/j.ijhydene.2010.02.118	journal	June 2010
Hydrogen desorption from LiBH4 destabilized by chlorides of transition metal Fe, Co, and Ni Zhang, Bang Jie; Liu, Bin Hong International Journal of Hydrogen Energy, Vol. 35, Issue 14 https://doi.org/10.1016/j.ijhydene.2010.04.165	journal	July 2010
Reversibility aspect of lithium borohydrides Au, Ming; Walters, R. Tom International Journal of Hydrogen Energy, Vol. 35, Issue 19 https://doi.org/10.1016/j.ijhydene.2010.07.130	journal	October 2010
The processing of Mg–Ti for hydrogen storage; mechanical milling and plasma synthesis Çakmak, G.; Károly, Z.; Mohai, I. International Journal of Hydrogen Energy, Vol. 35, Issue 19 https://doi.org/10.1016/j.ijhydene.2010.08.013	journal	October 2010
The influence of Cu substitution on the hydrogen sorption properties of magnesium rich Mg-Ni films Tan, X.; Danaie, M.; Kalisvaart, W. P. International Journal of Hydrogen Energy, Vol. 36, Issue 3 https://doi.org/10.1016/j.ijhydene.2010.11.058	journal	February 2011
Synthesis and hydrogen storage properties of ultrafine Mg–Zn particles Liu, Tong; Zhang, Tongwen; Zhang, Xuanzhou International Journal of Hydrogen Energy, Vol. 36, Issue 5 https://doi.org/10.1016/j.ijhydene.2010.12.049	journal	March 2011
Synthesis of magnesium nanoparticles with superior hydrogen storage properties by acetylene plasma metal reaction Zhang, Xuanzhou; Yang, Rong; Yang, Junzhi International Journal of Hydrogen Energy, Vol. 36, Issue 8 https://doi.org/10.1016/j.ijhydene.2010.12.052	journal	April 2011
Hydrogen absorption and optical properties of Pd/Mg thin films prepared by DC magnetron sputtering Gautam, Yogendra K.; Chawla, Amit K.; Khan, Saif A. International Journal of Hydrogen Energy, Vol. 37, Issue 4 https://doi.org/10.1016/j.ijhydene.2011.04.041	journal	February 2012
Thermodynamics, kinetics and microstructural evolution during hydrogenation of iron-doped magnesium thin films Tan, Zhuopeng; Chiu, Chun; Heilweil, Edwin J. International Journal of Hydrogen Energy, Vol. 36, Issue 16 https://doi.org/10.1016/j.ijhydene.2011.04.196	journal	August 2011
First principle study of hydrogen diffusion in equilibrium rutile, rutile with deformation twins and fluorite polymorph of Mg hydride Tao, S. X.; Kalisvaart, W. P.; Danaie, M. International Journal of Hydrogen Energy, Vol. 36, Issue 18 https://doi.org/10.1016/j.ijhydene.2011.06.075	journal	September 2011
Nanoconfined mixed Li and Mg borohydrides as materials for solid state hydrogen storage Capurso, Giovanni; Agresti, Filippo; Crociani, Laura International Journal of Hydrogen Energy, Vol. 37, Issue 14 https://doi.org/10.1016/j.ijhydene.2012.04.111	journal	July 2012
Hydrogen storage properties of nano-structured 0.65MgH2/0.35ScH2 Luo, Xuanli; Grant, David M.; Walker, Gavin S. International Journal of Hydrogen Energy, Vol. 38, Issue 1 https://doi.org/10.1016/j.ijhydene.2012.10.025	journal	January 2013
Hydrogen storage in hybrid nanostructured carbon/palladium materials: Influence of particle size and surface chemistry Dibandjo, Philippe; Zlotea, Claudia; Gadiou, Roger International Journal of Hydrogen Energy, Vol. 38, Issue 2 https://doi.org/10.1016/j.ijhydene.2012.10.050	journal	January 2013
Improved hydrogen cycling kinetics of nano-structured magnesium/transition metal multilayer thin films Fry, Christopher M. P.; Grant, David M.; Walker, Gavin S. International Journal of Hydrogen Energy, Vol. 38, Issue 2 https://doi.org/10.1016/j.ijhydene.2012.10.089	journal	January 2013
Improved reversible hydrogen storage of LiAlH4 by nano-sized TiH2 Liu, Shu-Sheng; Li, Zhi-Bao; Jiao, Cheng-Li International Journal of Hydrogen Energy, Vol. 38, Issue 6 https://doi.org/10.1016/j.ijhydene.2012.11.042	journal	February 2013
Studies on de/rehydrogenation characteristics of nanocrystalline MgH2 co-catalyzed with Ti, Fe and Ni Shahi, Rohit R.; Tiwari, Anand P.; Shaz, M. A. International Journal of Hydrogen Energy, Vol. 38, Issue 6 https://doi.org/10.1016/j.ijhydene.2012.11.073	journal	February 2013
Nanoconfined 2LiBH4–MgH2–TiCl3 in carbon aerogel scaffold for reversible hydrogen storage Gosalawit-Utke, Rapee; Milanese, Chiara; Javadian, Payam International Journal of Hydrogen Energy, Vol. 38, Issue 8 https://doi.org/10.1016/j.ijhydene.2012.12.123	journal	March 2013
Strain effect on structural and dehydrogenation properties of MgH2 hydride from first-principles calculations Zhang, J.; Zhou, Y. C.; Ma, Z. S. International Journal of Hydrogen Energy, Vol. 38, Issue 9 https://doi.org/10.1016/j.ijhydene.2013.01.089	journal	March 2013
Phase field modeling of hydrogen transport and reaction in metal hydrides Voskuilen, Tyler G.; Pourpoint, Timothée L. International Journal of Hydrogen Energy, Vol. 38, Issue 18 https://doi.org/10.1016/j.ijhydene.2013.04.049	journal	June 2013
Hydrogen storage properties of Mg–TM–La (TM = Ti, Fe, Ni) ternary composite powders prepared through arc plasma method Zou, Jianxin; Guo, Hao; Zeng, Xiaoqin International Journal of Hydrogen Energy, Vol. 38, Issue 21 https://doi.org/10.1016/j.ijhydene.2013.05.007	journal	July 2013
Hydrogen storage properties of Mg–Ni nanoparticles Callini, E.; Pasquini, L.; Jensen, T. R. International Journal of Hydrogen Energy, Vol. 38, Issue 27 https://doi.org/10.1016/j.ijhydene.2013.05.139	journal	September 2013
X-ray photoelectron spectroscopy investigation of magnetron sputtered Mg–Ti–H thin films Jensen, I. J. T.; Thøgersen, A.; Løvvik, O. M. International Journal of Hydrogen Energy, Vol. 38, Issue 25 https://doi.org/10.1016/j.ijhydene.2013.05.142	journal	August 2013
Catalysis and evolution on cycling of nano-structured magnesium multilayer thin films Fry, Christopher M. P.; Grant, David M.; Walker, Gavin S. International Journal of Hydrogen Energy, Vol. 39, Issue 2 https://doi.org/10.1016/j.ijhydene.2013.10.136	journal	January 2014
Hydride destabilization in core–shell nanoparticles Pasquini, L.; Sacchi, M.; Brighi, M. International Journal of Hydrogen Energy, Vol. 39, Issue 5 https://doi.org/10.1016/j.ijhydene.2013.11.085	journal	February 2014
The effects of the nanometric interstitial compounds TiC, ZrC and TiN on the mechanical and thermal dehydrogenation and rehydrogenation of the nanocomposite lithium alanate (LiAlH4) hydride Varin, R. A.; Parviz, R. International Journal of Hydrogen Energy, Vol. 39, Issue 6 https://doi.org/10.1016/j.ijhydene.2013.11.118	journal	February 2014
Size and stress dependent hydrogen desorption in metastable Mg hydride films Ham, B.; Junkaew, A.; Arróyave, R. International Journal of Hydrogen Energy, Vol. 39, Issue 6 https://doi.org/10.1016/j.ijhydene.2013.12.017	journal	February 2014
Formation kinetics and microstructure of Mg–Ti hydrides made by reactive ball milling Biasetti, A.; Meyer, M.; Zélis, L. Mendoza International Journal of Hydrogen Energy, Vol. 39, Issue 16 https://doi.org/10.1016/j.ijhydene.2013.12.034	journal	May 2014
Destabilization of LiBH4 by nanoconfinement in PMMA–co–BM polymer matrix for reversible hydrogen storage Gosalawit-Utke, Rapee; Meethom, Sukanya; Pistidda, Claudio International Journal of Hydrogen Energy, Vol. 39, Issue 10 https://doi.org/10.1016/j.ijhydene.2014.01.078	journal	March 2014
Nanoconfinement degradation in NaAlH4/CMK-1 Chumphongphan, Somwan; Filsø, Uffe; Paskevicius, Mark International Journal of Hydrogen Energy, Vol. 39, Issue 21 https://doi.org/10.1016/j.ijhydene.2014.05.087	journal	July 2014
Improvement of thermal stability and reduction of LiBH 4 /polymer host interaction of nanoconfined LiBH 4 for reversible hydrogen storage Plerdsranoy, Praphatsorn; Wiset, Nuntida; Milanese, Chiara International Journal of Hydrogen Energy, Vol. 40, Issue 1 https://doi.org/10.1016/j.ijhydene.2014.10.090	journal	January 2015
Controlled mechanochemical synthesis and hydrogen desorption mechanisms of nanostructured Mg2CoH5 Zepon, G.; Leiva, D. R.; Kaufman, M. J. International Journal of Hydrogen Energy, Vol. 40, Issue 3 https://doi.org/10.1016/j.ijhydene.2014.11.085	journal	January 2015
Preparation and hydrogen sorption properties of a Ni decorated Mg based Mg@Ni nano-composite Zou, Jianxin; Long, Sheng; Chen, Xi International Journal of Hydrogen Energy, Vol. 40, Issue 4 https://doi.org/10.1016/j.ijhydene.2014.11.113	journal	January 2015
Mechanical behavior of highly reactive nanostructured MgH 2 Nachev, S.; de Rango, P.; Skryabina, N. International Journal of Hydrogen Energy, Vol. 40, Issue 47 https://doi.org/10.1016/j.ijhydene.2015.05.022	journal	December 2015
Catalytic and inhibitive effects of Pd and Pt decorated MWCNTs on the dehydrogenation behavior of LiAlH4 Tan, Chia-Yen; Tsai, Wen-Ta International Journal of Hydrogen Energy, Vol. 40, Issue 32 https://doi.org/10.1016/j.ijhydene.2015.06.106	journal	August 2015
Hydrogen storage properties of in-situ stabilised magnesium nanoparticles generated by electroless reduction with alkali metals Liu, Wei; Aguey-Zinsou, Kondo-Francois International Journal of Hydrogen Energy, Vol. 40, Issue 47 https://doi.org/10.1016/j.ijhydene.2015.07.020	journal	December 2015
Synthesis of destabilized nanostructured lithium hydride via hydrogenation of lithium electrochemically inserted into graphite Huang, Liwu; Bonnet, Jean-Pierre; Zlotea, Claudia International Journal of Hydrogen Energy, Vol. 40, Issue 40 https://doi.org/10.1016/j.ijhydene.2015.07.130	journal	October 2015
Ni coated LiH nanoparticles for reversible hydrogen storage Wang, Lei; Quadir, M. Z.; Aguey-Zinsou, Kondo-Francois International Journal of Hydrogen Energy, Vol. 41, Issue 15 https://doi.org/10.1016/j.ijhydene.2016.01.173	journal	April 2016
Interface and strain effects on the H-sorption thermodynamics of size-selected Mg nanodots Molinari, Alan; D'Amico, Federico; Calizzi, Marco International Journal of Hydrogen Energy, Vol. 41, Issue 23 https://doi.org/10.1016/j.ijhydene.2016.02.003	journal	June 2016
Recent progress in magnesium borohydride Mg(BH4)2: Fundamentals and applications for energy storage Zavorotynska, Olena; El-Kharbachi, Abdelouahab; Deledda, Stefano International Journal of Hydrogen Energy, Vol. 41, Issue 32 https://doi.org/10.1016/j.ijhydene.2016.02.015	journal	August 2016
Synthesis of highly dispersed nanosized LaNi5 on carbon: Revisiting particle size effects on hydrogen storage properties Liu, Wei; Aguey-Zinsou, Kondo-Francois International Journal of Hydrogen Energy, Vol. 41, Issue 32 https://doi.org/10.1016/j.ijhydene.2016.02.024	journal	August 2016
Kinetics studies of the reversible partial decomposition reaction in Mg(BH4)2 Zavorotynska, Olena; Deledda, Stefano; Hauback, Bjørn C. International Journal of Hydrogen Energy, Vol. 41, Issue 23 https://doi.org/10.1016/j.ijhydene.2016.02.153	journal	June 2016
Nanostructured materials for solid-state hydrogen storage: A review of the achievement of COST Action MP1103 Callini, Elsa; Aguey-Zinsou, Kondo-Francois; Ahuja, Rajeev International Journal of Hydrogen Energy, Vol. 41, Issue 32 https://doi.org/10.1016/j.ijhydene.2016.04.025	journal	August 2016
A review on the current progress of metal hydrides material for solid-state hydrogen storage applications Rusman, N. A. A.; Dahari, M. International Journal of Hydrogen Energy, Vol. 41, Issue 28 https://doi.org/10.1016/j.ijhydene.2016.05.244	journal	July 2016
A review on kinetic models and corresponding analysis methods for hydrogen storage materials Pang, Yuepeng; Li, Qian International Journal of Hydrogen Energy, Vol. 41, Issue 40 https://doi.org/10.1016/j.ijhydene.2016.08.018	journal	October 2016
Compaction of LiBH4-LiAlH4 nanoconfined in activated carbon nanofibers: Dehydrogenation kinetics, reversibility, and mechanical stability during cycling Plerdsranoy, Praphatsorn; Javadian, Payam; Jensen, Nicholai Daugaard International Journal of Hydrogen Energy, Vol. 42, Issue 2 https://doi.org/10.1016/j.ijhydene.2016.09.056	journal	January 2017
Low-temperature hydrogen desorption from Mg(BH4)2 catalysed by ultrafine Ni nanoparticles in a mesoporous carbon matrix Wahab, Mohammad A.; Young, David J.; Karim, Azharul International Journal of Hydrogen Energy, Vol. 41, Issue 45 https://doi.org/10.1016/j.ijhydene.2016.09.098	journal	December 2016
Metal hydride based thermal energy storage system requirements for high performance concentrating solar power plants Corgnale, Claudio; Hardy, Bruce; Motyka, Theodore International Journal of Hydrogen Energy, Vol. 41, Issue 44 https://doi.org/10.1016/j.ijhydene.2016.09.108	journal	November 2016
Carbon supported lithium hydride nanoparticles: Impact of preparation conditions on particle size and hydrogen sorption Bramwell, Peter L.; Ngene, Peter; de Jongh, Petra E. International Journal of Hydrogen Energy, Vol. 42, Issue 8 https://doi.org/10.1016/j.ijhydene.2016.10.062	journal	February 2017
Synthesis and hydrogen storage properties of core–shell structured binary Mg@Ti and ternary Mg@Ti@Ni composites Lu, Chong; Zou, Jianxin; Shi, Xiaoying International Journal of Hydrogen Energy, Vol. 42, Issue 4 https://doi.org/10.1016/j.ijhydene.2016.10.088	journal	January 2017
Enhanced reversibility of the electrochemical Li conversion reaction with MgH 2 –TiH 2 nanocomposites Berti, Nicola; Cuevas, Fermín; Zhang, Junxian International Journal of Hydrogen Energy, Vol. 42, Issue 35 https://doi.org/10.1016/j.ijhydene.2017.03.048	journal	August 2017
Nanoconfined lithium aluminium hydride (LiAlH4) and hydrogen reversibility Wang, Lei; Rawal, Aditya; Quadir, Md Zakaria International Journal of Hydrogen Energy, Vol. 42, Issue 20 https://doi.org/10.1016/j.ijhydene.2017.04.104	journal	May 2017
First principle study of strain effect on structural and dehydrogenation properties of complex hydride LiBH4 Benzidi, H.; Lakhal, M.; Benyoussef, A. International Journal of Hydrogen Energy, Vol. 42, Issue 30 https://doi.org/10.1016/j.ijhydene.2017.06.068	journal	July 2017
Carbon scaffold modified by metal (Ni) or non-metal (N) to enhance hydrogen storage of MgH2 through nanoconfinement Jia, Yi; Yao, Xiangdong International Journal of Hydrogen Energy, Vol. 42, Issue 36 https://doi.org/10.1016/j.ijhydene.2017.07.106	journal	September 2017
Formation of aluminium hydride (AlH3) via the decomposition of organoaluminium and hydrogen storage properties Wang, Lei; Rawal, Aditya; Quadir, Md Zakaria International Journal of Hydrogen Energy, Vol. 43, Issue 34 https://doi.org/10.1016/j.ijhydene.2017.12.052	journal	August 2018
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Characterisation of Mg–x wt.% FeTi (x = 5–30) and Mg–40 wt.% FeTiMn hydrogen absorbing materials prepared by mechanical alloying Vijay, R.; Sundaresan, R.; Maiya, M. P. Journal of Alloys and Compounds, Vol. 384, Issue 1-2 https://doi.org/10.1016/j.jallcom.2004.04.115	journal	December 2004
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Mechanochemical synthesis of nanostructured chemical hydrides in hydrogen alloying mills Wronski, Z.; Varin, R. A.; Chiu, C. Journal of Alloys and Compounds, Vol. 434-435 https://doi.org/10.1016/j.jallcom.2006.08.301	journal	May 2007
SEM and TEM characterization of magnesium hydride catalyzed with Ni nano-particle or Nb2O5 Hanada, Nobuko; Hirotoshi, Enoki; Ichikawa, Takayuki Journal of Alloys and Compounds, Vol. 450, Issue 1-2 https://doi.org/10.1016/j.jallcom.2006.10.128	journal	February 2008
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Novel Sieverts’ type volumetric measurements of hydrogen storage properties for very small sample quantities Lee, Yong-Won; Clemens, Bruce M.; Gross, Karl J. Journal of Alloys and Compounds, Vol. 452, Issue 2 https://doi.org/10.1016/j.jallcom.2006.11.014	journal	March 2008
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A quantum chemical study on magnesium(Mg)/magnesium–hydrogen(Mg–H) nanowires Peng, Bo; Li, Lanlan; Ji, Weiqiang Journal of Alloys and Compounds, Vol. 484, Issue 1-2 https://doi.org/10.1016/j.jallcom.2009.04.087	journal	September 2009
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Enhanced hydrogen storage properties of magnesium by the synergic catalytic effect of TiH1.971 and TiH1.5 nanoparticles at room temperature Liu, Tong; Chen, Chunguang; Wang, Fan Journal of Power Sources, Vol. 267 https://doi.org/10.1016/j.jpowsour.2014.05.066	journal	December 2014
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Hydrogen storage properties of magnesium ultrafine particles prepared by hydrogen plasma-metal reaction Shao, Huaiyu; Wang, Yuntao; Xu, Hairuo Materials Science and Engineering: B, Vol. 110, Issue 2 https://doi.org/10.1016/j.mseb.2004.03.013	journal	July 2004
The development of mixture, alloy, and core-shell nanocatalysts with nanomaterial supports for energy conversion in low-temperature fuel cells Long, Nguyen Viet; Yang, Yong; Minh Thi, Cao Nano Energy, Vol. 2, Issue 5 https://doi.org/10.1016/j.nanoen.2013.06.001	journal	September 2013
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Recent developments in the fabrication, characterization and implementation of MgH ₂ -based solid-hydrogen materials in the Kuwait Institute for Scientific Research El-Eskandarany, Mohamed Sherif RSC Advances, Vol. 9, Issue 18 https://doi.org/10.1039/c9ra00287a	journal	January 2019
Environmentally friendly nanocrystalline magnesium hydride decorated with metallic glassy-zirconium palladium nanopowders for fuel cell applications El-Eskandarany, M. Sherif; Banyan, Mohammad; Al-Ajmi, Fahad RSC Advances, Vol. 9, Issue 48 https://doi.org/10.1039/c9ra05121j	journal	January 2019
Molecular modelling and machine learning for high-throughput screening of metal-organic frameworks for hydrogen storage Bobbitt, N. Scott; Snurr, Randall Q. Molecular Simulation, Vol. 45, Issue 14-15 https://doi.org/10.1080/08927022.2019.1597271	journal	April 2019
Investigations of Physical Properties of XTiH3 and Implications for Solid State Hydrogen Storage Al, Selgin Zeitschrift für Naturforschung A, Vol. 74, Issue 11 https://doi.org/10.1515/zna-2019-0184	journal	November 2019

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