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This content will become publicly available on November 27, 2019

Title: Freestanding 1T MoS 2 /graphene heterostructures as a highly efficient electrocatalyst for lithium polysulfides in Li–S batteries

A novel approach to effectively suppress the “polysulfide shuttle” in Li–S batteries is presented by designing a freestanding, three-dimensional graphene/1T MoS 2 (3DG/TM) heterostructure with highly efficient electrocatalysis properties for lithium polysulfides (LiPSs).
Authors:
 [1] ;  [2] ;  [2] ; ORCiD logo [2] ; ORCiD logo [3] ; ORCiD logo [4]
  1. Materials Science and Engineering Program & Texas Materials Institute, The University of Texas at Austin, Austin, USA, State Key Laboratory of Electronic Thin Films and Integrated Devices
  2. McKetta Department of Chemical Engineering, The University of Texas at Austin, Austin, USA
  3. State Key Laboratory of Electronic Thin Films and Integrated Devices, University of Electronic Science and Technology of China, Chengdu 610054, P. R. China
  4. Materials Science and Engineering Program & Texas Materials Institute, The University of Texas at Austin, Austin, USA
Publication Date:
Grant/Contract Number:
SC0005397
Type:
Publisher's Accepted Manuscript
Journal Name:
Energy & Environmental Science
Additional Journal Information:
Journal Name: Energy & Environmental Science Journal Volume: 12 Journal Issue: 1; Journal ID: ISSN 1754-5692
Publisher:
Royal Society of Chemistry (RSC)
Sponsoring Org:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
Country of Publication:
United Kingdom
Language:
English
OSTI Identifier:
1485180

He, Jiarui, Hartmann, Gregory, Lee, Myungsuk, Hwang, Gyeong S., Chen, Yuanfu, and Manthiram, Arumugam. Freestanding 1T MoS 2 /graphene heterostructures as a highly efficient electrocatalyst for lithium polysulfides in Li–S batteries. United Kingdom: N. p., Web. doi:10.1039/C8EE03252A.
He, Jiarui, Hartmann, Gregory, Lee, Myungsuk, Hwang, Gyeong S., Chen, Yuanfu, & Manthiram, Arumugam. Freestanding 1T MoS 2 /graphene heterostructures as a highly efficient electrocatalyst for lithium polysulfides in Li–S batteries. United Kingdom. doi:10.1039/C8EE03252A.
He, Jiarui, Hartmann, Gregory, Lee, Myungsuk, Hwang, Gyeong S., Chen, Yuanfu, and Manthiram, Arumugam. 2019. "Freestanding 1T MoS 2 /graphene heterostructures as a highly efficient electrocatalyst for lithium polysulfides in Li–S batteries". United Kingdom. doi:10.1039/C8EE03252A.
@article{osti_1485180,
title = {Freestanding 1T MoS 2 /graphene heterostructures as a highly efficient electrocatalyst for lithium polysulfides in Li–S batteries},
author = {He, Jiarui and Hartmann, Gregory and Lee, Myungsuk and Hwang, Gyeong S. and Chen, Yuanfu and Manthiram, Arumugam},
abstractNote = {A novel approach to effectively suppress the “polysulfide shuttle” in Li–S batteries is presented by designing a freestanding, three-dimensional graphene/1T MoS 2 (3DG/TM) heterostructure with highly efficient electrocatalysis properties for lithium polysulfides (LiPSs).},
doi = {10.1039/C8EE03252A},
journal = {Energy & Environmental Science},
number = 1,
volume = 12,
place = {United Kingdom},
year = {2019},
month = {1}
}

Works referenced in this record:

MoS2 Nanoparticles Grown on Graphene An Advanced Catalyst for the Hydrogen Evolution Reaction
journal, May 2011
  • Li, Yanguang; Wang, Hailiang; Xie, Liming
  • Journal of the American Chemical Society, Vol. 133, Issue 19, p. 7296-7299
  • DOI: 10.1021/ja201269b