Chemical complexity induced local structural distortion in NiCoFeMnCr high-entropy alloy

Zhang, Fuxiang; Tong, Yang; Jin, Ke; Bei, Hongbin; Weber, William J.; Huq, Ashfia; Lanzirotti, Antonio; Newville, Matt; Pagan, Darren C.; Ko, J. Y. P.; Zhang, Yanwen

doi:10.1080/21663831.2018.1478332

Title: Chemical complexity induced local structural distortion in NiCoFeMnCr high-entropy alloy

Abstract

In order to study chemical complexity-induced lattice distortion in high-entropy alloys, the static Debye–Waller (D-W) factor of NiCoFeMnCr solid solution alloy is measured with low temperature neutron diffraction, ambient X-ray diffraction, and total scattering methods. Here, the static atomic displacement parameter of the multi-element component alloy at 0 K is 0.035–0.041 Å, which is obvious larger than that of element Ni (~0 Å). The atomic pair distance between individual atoms in the alloy investigated with extended X-ray absorption fine structure (EXAFS) measurements indicates that Mn has a slightly larger bond distance (~0.4%) with neighbor atoms than that of others.

Authors:

^[1];

^[1]; Jin, Ke ^[1];

^[1];

^[2]; Huq, Ashfia ^[3]; Lanzirotti, Antonio ^[4]; Newville, Matt ^[4]; Pagan, Darren C. ^[5]; Ko, J. Y. P. ^[5];

^[1]

Division of Materials Science and Technology, Oak Ridge National Laboratory, Oak Ridge, TN, USA
Division of Materials Science and Technology, Oak Ridge National Laboratory, Oak Ridge, TN, USA, Department of Materials Science and Engineering, The University of Tennessee, Knoxville, TN, USA
Spallation Neutron Source, Oak Ridge National Laboratory, Oak Ridge, TN, USA
University of Chicago, Center for Advanced Radiation Sources, Chicago, IL, USA
Cornell High Energy Synchrotron Source, Cornell University, Ithaca, NY, USA

Publication Date:: Sat Jun 16 00:00:00 EDT 2018

Research Org.:: Energy Frontier Research Centers (EFRC) (United States). Energy Dissipation to Defect Evolution (EDDE); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI Identifier:: 1483331

Alternate Identifier(s):: OSTI ID: 1456802

Grant/Contract Number:: AC02-06CH11357; AC05-00OR22725

Resource Type:: Published Article

Journal Name:: Materials Research Letters

Additional Journal Information:: Journal Name: Materials Research Letters Journal Volume: 6 Journal Issue: 8; Journal ID: ISSN 2166-3831

Publisher:: Informa UK Limited

Country of Publication:: United Kingdom

Language:: English

Subject:: 36 MATERIALS SCIENCE; solid solution alloys; neutron diffraction; EXAFS; local structure

Citation Formats


                    Zhang, Fuxiang, Tong, Yang, Jin, Ke, Bei, Hongbin, Weber, William J., Huq, Ashfia, Lanzirotti, Antonio, Newville, Matt, Pagan, Darren C., Ko, J. Y. P., and Zhang, Yanwen. Chemical complexity induced local structural distortion in NiCoFeMnCr high-entropy alloy.  United Kingdom: N. p., 2018. 
Web.  doi:10.1080/21663831.2018.1478332.

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                    Zhang, Fuxiang, Tong, Yang, Jin, Ke, Bei, Hongbin, Weber, William J., Huq, Ashfia, Lanzirotti, Antonio, Newville, Matt, Pagan, Darren C., Ko, J. Y. P., & Zhang, Yanwen. Chemical complexity induced local structural distortion in NiCoFeMnCr high-entropy alloy.  United Kingdom.  https://doi.org/10.1080/21663831.2018.1478332

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                    Zhang, Fuxiang, Tong, Yang, Jin, Ke, Bei, Hongbin, Weber, William J., Huq, Ashfia, Lanzirotti, Antonio, Newville, Matt, Pagan, Darren C., Ko, J. Y. P., and Zhang, Yanwen. Sat .  
"Chemical complexity induced local structural distortion in NiCoFeMnCr high-entropy alloy".  United Kingdom.  https://doi.org/10.1080/21663831.2018.1478332.

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@article{osti_1483331,

  title        = {Chemical complexity induced local structural distortion in NiCoFeMnCr high-entropy alloy},

  author       = {Zhang, Fuxiang and Tong, Yang and Jin, Ke and Bei, Hongbin and Weber, William J. and Huq, Ashfia and Lanzirotti, Antonio and Newville, Matt and Pagan, Darren C. and Ko, J. Y. P. and Zhang, Yanwen},

  abstractNote = {In order to study chemical complexity-induced lattice distortion in high-entropy alloys, the static Debye–Waller (D-W) factor of NiCoFeMnCr solid solution alloy is measured with low temperature neutron diffraction, ambient X-ray diffraction, and total scattering methods. Here, the static atomic displacement parameter of the multi-element component alloy at 0 K is 0.035–0.041 Å, which is obvious larger than that of element Ni (~0 Å). The atomic pair distance between individual atoms in the alloy investigated with extended X-ray absorption fine structure (EXAFS) measurements indicates that Mn has a slightly larger bond distance (~0.4%) with neighbor atoms than that of others.},

  doi          = {10.1080/21663831.2018.1478332},

  journal      = {Materials Research Letters},

  number       = 8,

  volume       = 6,

  place        = {United Kingdom},

  year         = {Sat Jun 16 00:00:00 EDT 2018},

  month        = {Sat Jun 16 00:00:00 EDT 2018}

}

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Works referencing / citing this record:

Critical Review of Chemical Complexity Effect on Local Structure of Multi-principal-Element Alloys
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Title: Chemical complexity induced local structural distortion in NiCoFeMnCr high-entropy alloy

Abstract

Citation Formats

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