Solitary Oxygen Dopant Emission from Carbon Nanotubes Modified by Dielectric Metasurfaces
Abstract
All-dielectric metasurfaces made from arrays of high index nanoresonators supporting strong magnetic dipole modes have emerged as a low-loss alternative to plasmonic metasurfaces. Here we use oxygen-doped single-walled carbon nanotubes (SWCNTs) as quantum emitters and couple them to silicon metasurfaces to study effects of the magnetic dipole modes of the constituent nanoresonators on the photoluminescence (PL) of individual SWCNTs. We find that when in resonance, the magnetic mode of the silicon nanoresonators can lead to a moderate average PL enhancement of 0.8–4.0 of the SWCNTs, accompanied by an average increase in the radiative decay rate by a factor of 1.5–3.0. More interestingly, single dopant polarization experiments show an anomalous photoluminescence polarization rotation by coupling individual SWCNTs to silicon nanoresonators. Numerical simulations indicate that this is caused by modification of near-field polarization distribution at certain areas in the proximity of the silicon nanoresonators at the excitation wavelength, thus presenting an approach to control emission polarization. In conclusion, these findings indicate silicon nanoresonators as potential building blocks of quantum photonic circuits capable of manipulating PL intensity and polarization of single photon sources.
- Authors:
-
[1];
[2];
[2];
[2];
- Sandia National Lab. (SNL-NM), Albuquerque, NM (United States). Center for Integrated Nanotechnologies
- Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
- Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
- Publication Date:
- Research Org.:
- Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE National Nuclear Security Administration (NNSA)
- OSTI Identifier:
- 1481990
- Report Number(s):
- LA-UR-18-21087
Journal ID: ISSN 1936-0851
- Grant/Contract Number:
- AC52-06NA25396; NA0003525
- Resource Type:
- Accepted Manuscript
- Journal Name:
- ACS Nano
- Additional Journal Information:
- Journal Volume: 11; Journal Issue: 6; Journal ID: ISSN 1936-0851
- Publisher:
- American Chemical Society (ACS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 77 NANOSCIENCE AND NANOTECHNOLOGY; 36 MATERIALS SCIENCE; Material Science; all-dielectric metasurfaces; magnetic resonance; oxygen-doped single-walled carbon nanotubes; photoluminescence; polarization
Citation Formats
Ma, Xuedan, James, Anthony R., Hartmann, Nicolai F., Baldwin, Jon Kevin Scott, Dominguez, Jason, Sinclair, Michael B., Luk, Ting S., Wolf, Omri, Liu, Sheng, Doorn, Stephen K., Htoon, Han, and Brener, Igal. Solitary Oxygen Dopant Emission from Carbon Nanotubes Modified by Dielectric Metasurfaces. United States: N. p., 2017.
Web. doi:10.1021/acsnano.7b02951.
Ma, Xuedan, James, Anthony R., Hartmann, Nicolai F., Baldwin, Jon Kevin Scott, Dominguez, Jason, Sinclair, Michael B., Luk, Ting S., Wolf, Omri, Liu, Sheng, Doorn, Stephen K., Htoon, Han, & Brener, Igal. Solitary Oxygen Dopant Emission from Carbon Nanotubes Modified by Dielectric Metasurfaces. United States. https://doi.org/10.1021/acsnano.7b02951
Ma, Xuedan, James, Anthony R., Hartmann, Nicolai F., Baldwin, Jon Kevin Scott, Dominguez, Jason, Sinclair, Michael B., Luk, Ting S., Wolf, Omri, Liu, Sheng, Doorn, Stephen K., Htoon, Han, and Brener, Igal. Thu .
"Solitary Oxygen Dopant Emission from Carbon Nanotubes Modified by Dielectric Metasurfaces". United States. https://doi.org/10.1021/acsnano.7b02951. https://www.osti.gov/servlets/purl/1481990.
@article{osti_1481990,
title = {Solitary Oxygen Dopant Emission from Carbon Nanotubes Modified by Dielectric Metasurfaces},
author = {Ma, Xuedan and James, Anthony R. and Hartmann, Nicolai F. and Baldwin, Jon Kevin Scott and Dominguez, Jason and Sinclair, Michael B. and Luk, Ting S. and Wolf, Omri and Liu, Sheng and Doorn, Stephen K. and Htoon, Han and Brener, Igal},
abstractNote = {All-dielectric metasurfaces made from arrays of high index nanoresonators supporting strong magnetic dipole modes have emerged as a low-loss alternative to plasmonic metasurfaces. Here we use oxygen-doped single-walled carbon nanotubes (SWCNTs) as quantum emitters and couple them to silicon metasurfaces to study effects of the magnetic dipole modes of the constituent nanoresonators on the photoluminescence (PL) of individual SWCNTs. We find that when in resonance, the magnetic mode of the silicon nanoresonators can lead to a moderate average PL enhancement of 0.8–4.0 of the SWCNTs, accompanied by an average increase in the radiative decay rate by a factor of 1.5–3.0. More interestingly, single dopant polarization experiments show an anomalous photoluminescence polarization rotation by coupling individual SWCNTs to silicon nanoresonators. Numerical simulations indicate that this is caused by modification of near-field polarization distribution at certain areas in the proximity of the silicon nanoresonators at the excitation wavelength, thus presenting an approach to control emission polarization. In conclusion, these findings indicate silicon nanoresonators as potential building blocks of quantum photonic circuits capable of manipulating PL intensity and polarization of single photon sources.},
doi = {10.1021/acsnano.7b02951},
journal = {ACS Nano},
number = 6,
volume = 11,
place = {United States},
year = {Thu May 18 00:00:00 EDT 2017},
month = {Thu May 18 00:00:00 EDT 2017}
}
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