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Title: Dynamics in hard condensed matter probed by X-ray photon correlation spectroscopy: Present and beyond

Abstract

Insight into the spatial ordering and dynamics of structural heterogeneity in materials is at the heart of understanding their structure and function. X-ray photon correlation spectroscopy (XPCS) measures the dynamic structure factor providing S(Q,t) information on the spontaneous low-energy dynamics intrinsic to many materials. Combined with in situ and in operando capabilities, XPCS provides unique insight into a variety of scientific areas, including phase separation in binary alloys, aging in metallic glasses, surface dynamics during growth, domain wall dynamics in ferroic complex oxides and charge and spin density wave motion in quantum materials. In conclusion, this review summarizes some recent XPCS work in these areas and discusses scientific opportunities that will be made possible with the many-fold increase in coherent flux provided by the world-wide construction and commissioning of X-ray sources based on multi-bend achromat (MBA) storage ring (SR) lattices and high repetition rate free electron lasers (FELs).

Authors:
ORCiD logo [1];  [2];  [2]
  1. (张庆腾), Qingteng [Argonne National Lab. (ANL), Lemont, IL (United States)
  2. Argonne National Lab. (ANL), Lemont, IL (United States)
Publication Date:
Research Org.:
Argonne National Lab. (ANL), Argonne, IL (United States)
Sponsoring Org.:
USDOE Office of Science (SC)
OSTI Identifier:
1481770
Grant/Contract Number:  
AC02-06CH11357
Resource Type:
Accepted Manuscript
Journal Name:
Current Opinion in Solid State and Materials Science
Additional Journal Information:
Journal Volume: 22; Journal Issue: 5; Journal ID: ISSN 1359-0286
Publisher:
Elsevier
Country of Publication:
United States
Language:
English
Subject:
74 ATOMIC AND MOLECULAR PHYSICS; Atomic dynamics; Quantum fluctuations; Solid state materials; X-ray photon correlation spectroscopy

Citation Formats

Zhang, Dufresne, Eric M., and Sandy, Alec R. Dynamics in hard condensed matter probed by X-ray photon correlation spectroscopy: Present and beyond. United States: N. p., 2018. Web. doi:10.1016/j.cossms.2018.06.002.
Zhang, Dufresne, Eric M., & Sandy, Alec R. Dynamics in hard condensed matter probed by X-ray photon correlation spectroscopy: Present and beyond. United States. https://doi.org/10.1016/j.cossms.2018.06.002
Zhang, Dufresne, Eric M., and Sandy, Alec R. Wed . "Dynamics in hard condensed matter probed by X-ray photon correlation spectroscopy: Present and beyond". United States. https://doi.org/10.1016/j.cossms.2018.06.002. https://www.osti.gov/servlets/purl/1481770.
@article{osti_1481770,
title = {Dynamics in hard condensed matter probed by X-ray photon correlation spectroscopy: Present and beyond},
author = {Zhang and Dufresne, Eric M. and Sandy, Alec R.},
abstractNote = {Insight into the spatial ordering and dynamics of structural heterogeneity in materials is at the heart of understanding their structure and function. X-ray photon correlation spectroscopy (XPCS) measures the dynamic structure factor providing S(Q,t) information on the spontaneous low-energy dynamics intrinsic to many materials. Combined with in situ and in operando capabilities, XPCS provides unique insight into a variety of scientific areas, including phase separation in binary alloys, aging in metallic glasses, surface dynamics during growth, domain wall dynamics in ferroic complex oxides and charge and spin density wave motion in quantum materials. In conclusion, this review summarizes some recent XPCS work in these areas and discusses scientific opportunities that will be made possible with the many-fold increase in coherent flux provided by the world-wide construction and commissioning of X-ray sources based on multi-bend achromat (MBA) storage ring (SR) lattices and high repetition rate free electron lasers (FELs).},
doi = {10.1016/j.cossms.2018.06.002},
journal = {Current Opinion in Solid State and Materials Science},
number = 5,
volume = 22,
place = {United States},
year = {Wed Aug 01 00:00:00 EDT 2018},
month = {Wed Aug 01 00:00:00 EDT 2018}
}

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