Multidimensional Coherent Spectroscopy of Semiconductors

Smallwood, Christopher L.; Cundiff, Steven T.

doi:10.1002/lpor.201800171

Title: Multidimensional Coherent Spectroscopy of Semiconductors

Journal Article · 07 November 2018 · Laser & Photonics Reviews

DOI: https://doi.org/10.1002/lpor.201800171 · OSTI ID:1481430

Smallwood, Christopher L. ^[1];

^[1]

Department of Physics University of Michigan Ann Arbor MI 48109 USA

Abstract Optical multidimensional coherent spectroscopy (MDCS) is a nonlinear spectroscopy technique where a material is excited by a series of laser pulses to produce a spectrum as a function of multiple frequencies. The technique's ability to elucidate excited‐state structure and interactions has made MDCS a valuable tool in the study of excitons in semiconductors. This review introduces the method and describes progress it has fostered establishing a better understanding of dephasing rates, coherent coupling mechanisms, and many‐body interactions pertaining to optically generated electronic excitations in a variety of semiconductor material systems. Emphasis is placed on nanostructured gallium arsenide quantum wells and quantum dots, on quantum dots in other III–V and II–VI semiconductors, and on atomically thin transition metal dichalcogenides. Recent technical advances and potential future directions in the field are also discussed.

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Sponsoring Organization:: USDOE

Grant/Contract Number:: NONE; SC0015782

OSTI ID:: 1481430

Journal Information:: Laser & Photonics Reviews, Journal Name: Laser & Photonics Reviews Journal Issue: 12 Vol. 12; ISSN 1863-8880

Publisher:: Wiley Blackwell (John Wiley & Sons)Copyright Statement

Country of Publication:: Germany

Language:: English

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Coherent Control and Polarization Readout of Individual Excitonic States Patton, B.; Woggon, U.; Langbein, W. Physical Review Letters, Vol. 95, Issue 26 https://doi.org/10.1103/PhysRevLett.95.266401	journal	December 2005
Many-Body Interactions in Semiconductors Probed by Optical Two-Dimensional Fourier Transform Spectroscopy Li, Xiaoqin; Zhang, Tianhao; Borca, Camelia N. Physical Review Letters, Vol. 96, Issue 5 https://doi.org/10.1103/PhysRevLett.96.057406	journal	February 2006
Femtosecond Phase-Coherent Two-Dimensional Spectroscopy Tian, Peifang; Keusters, Dorine; Suzaki, Yoshifumi Science, Vol. 300, Issue 5625, p. 1553-1555 https://doi.org/10.1126/science.1083433	journal	June 2003
Ultrafast Dynamics of Solute-Solvent Complexation Observed at Thermal Equilibrium in Real Time Zheng, J. Science, Vol. 309, Issue 5739 https://doi.org/10.1126/science.1116213	journal	August 2005
Bose-Einstein Condensation of Microcavity Polaritons in a Trap Balili, R.; Hartwell, V.; Snoke, D. Science, Vol. 316, Issue 5827 https://doi.org/10.1126/science.1140990	journal	May 2007
Two-Quantum 2D FT Electronic Spectroscopy of Biexcitons in GaAs Quantum Wells Stone, K. W.; Gundogdu, K.; Turner, D. B. Science, Vol. 324, Issue 5931 https://doi.org/10.1126/science.1170274	journal	May 2009
Coherent Two-Dimensional Nanoscopy Aeschlimann, M.; Brixner, T.; Fischer, A. Science, Vol. 333, Issue 6050 https://doi.org/10.1126/science.1209206	journal	August 2011
Frequency combs enable rapid and high-resolution multidimensional coherent spectroscopy Lomsadze, Bachana; Cundiff, Steven T. Science, Vol. 357, Issue 6358 https://doi.org/10.1126/science.aao1090	journal	September 2017
Optical Rabi Oscillations in a Quantum Dot Ensemble Kujiraoka, Mamiko; Ishi-Hayase, Junko; Akahane, Kouichi Applied Physics Express, Vol. 3, Issue 9 https://doi.org/10.1143/APEX.3.092801	journal	August 2010
Spatial Optical Parametric Coupling of Picosecond Light Pulses and Transverse Relaxation Effect in Resonant Media Yajima, Tatsuo; Taira, Yoichi Journal of the Physical Society of Japan, Vol. 47, Issue 5 https://doi.org/10.1143/JPSJ.47.1620	journal	November 1979
Experimental Implementations of Two-Dimensional Fourier Transform Electronic Spectroscopy Fuller, Franklin D.; Ogilvie, Jennifer P. Annual Review of Physical Chemistry, Vol. 66, Issue 1 https://doi.org/10.1146/annurev-physchem-040513-103623	journal	April 2015
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Spectral signatures of χ^(5) processes in four-wave mixing of homogeneously broadened excitons Langbein, W.; Meier, T.; Koch, S. W. Journal of the Optical Society of America B, Vol. 18, Issue 9 https://doi.org/10.1364/JOSAB.18.001318	journal	January 2001
Nonperturbative transient four-wave-mixing line shapes due to excitation-induced shift and excitation-induced dephasing Shacklette, J. M.; Cundiff, S. T. Journal of the Optical Society of America B, Vol. 20, Issue 4 https://doi.org/10.1364/JOSAB.20.000764	journal	January 2003
Quantifying spectral diffusion by the direct measurement of the correlation function for excitons in semiconductor quantum wells Singh, Rohan; Moody, Galan; Siemens, Mark E. Journal of the Optical Society of America B, Vol. 33, Issue 7 https://doi.org/10.1364/JOSAB.33.00C137	journal	January 2016
Analytical solutions to the finite-pulse Bloch model for multidimensional coherent spectroscopy Smallwood, Christopher L.; Autry, Travis M.; Cundiff, Steven T. Journal of the Optical Society of America B, Vol. 34, Issue 2 https://doi.org/10.1364/JOSAB.34.000419	journal	January 2017
Coherent spectroscopy of semiconductors Cundiff, Steven T. Optics Express, Vol. 16, Issue 7 https://doi.org/10.1364/OE.16.004639	journal	January 2008
Two-Dimensional Ultrafast Fourier Transform Spectroscopy in the Deep Ultraviolet Tseng, Chien-hung; Matsika, Spiridoula; Weinacht, Thomas C. Optics Express, Vol. 17, Issue 21 https://doi.org/10.1364/OE.17.018788	journal	January 2009
Resonance lineshapes in two-dimensional Fourier transform spectroscopy Siemens, Mark E.; Moody, Galan; Li, Hebin Optics Express, Vol. 18, Issue 17 https://doi.org/10.1364/OE.18.017699	journal	January 2010
Multidimensional coherent photocurrent spectroscopy of a semiconductor nanostructure Nardin, Gaël; Autry, Travis M.; Silverman, Kevin L. Optics Express, Vol. 21, Issue 23 https://doi.org/10.1364/OE.21.028617	journal	January 2013
Heterodyne spectral interferometry for multidimensional nonlinear spectroscopy of individual quantum systems Langbein, Wolfgang; Patton, Brian Optics Letters, Vol. 31, Issue 8 https://doi.org/10.1364/OL.31.001151	journal	January 2006
Coherent two-dimensional ultraviolet spectroscopy in fully noncollinear geometry Selig, Ulrike; Schleussner, Carl-Friedrich; Foerster, Michael Optics Letters, Vol. 35, Issue 24 https://doi.org/10.1364/OL.35.004178	journal	January 2010
Analytical calculation of two-dimensional spectra Bell, Joshua D.; Conrad, Rebecca; Siemens, Mark E. Optics Letters, Vol. 40, Issue 7 https://doi.org/10.1364/OL.40.001157	journal	January 2015
Frequency comb-based four-wave-mixing spectroscopy Lomsadze, Bachana; Cundiff, Steven T. Optics Letters, Vol. 42, Issue 12 https://doi.org/10.1364/OL.42.002346	journal	January 2017
Optical two-dimensional Fourier transform spectroscopy with active interferometric stabilization Zhang, Tianhao; Borca, Camelia N.; Li, Xiaoqin Optics Express, Vol. 13, Issue 19 https://doi.org/10.1364/OPEX.13.007432	journal	January 2005
Dynamics of excitons in individual InAs quantum dots revealed in four-wave mixing spectroscopy Mermillod, Q.; Wigger, D.; Delmonte, V. Optica, Vol. 3, Issue 4 https://doi.org/10.1364/OPTICA.3.000377	journal	January 2016
Dual-comb spectroscopy Coddington, Ian; Newbury, Nathan; Swann, William Optica, Vol. 3, Issue 4 https://doi.org/10.1364/OPTICA.3.000414	journal	January 2016

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