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Title: Scanning electron microscopy examination of a Fast Flux Test Facility irradiated U-10Zr fuel cross section clad with HT-9

Abstract

Observations from a scanning electron microscopy examination of irradiated U-10Zr fuel are presented. The sample studied had a local burnup of 5.7 atom percent and a local inner cladding temperature of 615°C. This examination by electron microscopy has concentrated on producing data relevant to facilitating a better understanding of Zr redistribution in irradiated U-10Zr fuel and on a better understanding of the complex microstructure present in fuel cladding chemical interaction (FCCI) layers. The presented zirconium redistribution data supplements the existing literature by providing a data set at these particular local conditions. In addition to FCCI layers that are readily visible in optical microscopy, this examination has revealed lanthanide degradation of the cladding by what appears to be a grain boundary facilitated pathway. Precipitates of fission produced Pd-lanthanide compounds were observed in the fuel. Furthermore, precipitated regions with elevated Mo and elevated W content were also observed in the HT-9 cladding of this sample.

Authors:
ORCiD logo [1]; ORCiD logo [1]; ORCiD logo [1]; ORCiD logo [1]; ORCiD logo [1]
  1. Idaho National Lab. (INL), Idaho Falls, ID (United States)
Publication Date:
Research Org.:
Idaho National Lab. (INL), Idaho Falls, ID (United States)
Sponsoring Org.:
USDOE Office of Nuclear Energy (NE), Fuel Cycle Technologies (NE-5); USDOE Office of Nuclear Energy (NE)
OSTI Identifier:
1481288
Alternate Identifier(s):
OSTI ID: 1495575
Report Number(s):
INL/JOU-17-42679-Rev000
Journal ID: ISSN 0022-3115
Grant/Contract Number:  
AC07-05ID14517
Resource Type:
Accepted Manuscript
Journal Name:
Journal of Nuclear Materials
Additional Journal Information:
Journal Volume: 494; Journal Issue: C; Journal ID: ISSN 0022-3115
Publisher:
Elsevier
Country of Publication:
United States
Language:
English
Subject:
11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS; Scanning Electron Microscopy; Irradiated U-10Zr; Fast Flux Test Facility Irradiated; Fuel Cladding Chemical Interaction; Zr redistribution; HT-9

Citation Formats

Harp, Jason M., Porter, Douglas L., Miller, Brandon D., Trowbridge, Tammy L., and Carmack, William J. Scanning electron microscopy examination of a Fast Flux Test Facility irradiated U-10Zr fuel cross section clad with HT-9. United States: N. p., 2017. Web. doi:10.1016/j.jnucmat.2017.07.040.
Harp, Jason M., Porter, Douglas L., Miller, Brandon D., Trowbridge, Tammy L., & Carmack, William J. Scanning electron microscopy examination of a Fast Flux Test Facility irradiated U-10Zr fuel cross section clad with HT-9. United States. https://doi.org/10.1016/j.jnucmat.2017.07.040
Harp, Jason M., Porter, Douglas L., Miller, Brandon D., Trowbridge, Tammy L., and Carmack, William J. Sat . "Scanning electron microscopy examination of a Fast Flux Test Facility irradiated U-10Zr fuel cross section clad with HT-9". United States. https://doi.org/10.1016/j.jnucmat.2017.07.040. https://www.osti.gov/servlets/purl/1481288.
@article{osti_1481288,
title = {Scanning electron microscopy examination of a Fast Flux Test Facility irradiated U-10Zr fuel cross section clad with HT-9},
author = {Harp, Jason M. and Porter, Douglas L. and Miller, Brandon D. and Trowbridge, Tammy L. and Carmack, William J.},
abstractNote = {Observations from a scanning electron microscopy examination of irradiated U-10Zr fuel are presented. The sample studied had a local burnup of 5.7 atom percent and a local inner cladding temperature of 615°C. This examination by electron microscopy has concentrated on producing data relevant to facilitating a better understanding of Zr redistribution in irradiated U-10Zr fuel and on a better understanding of the complex microstructure present in fuel cladding chemical interaction (FCCI) layers. The presented zirconium redistribution data supplements the existing literature by providing a data set at these particular local conditions. In addition to FCCI layers that are readily visible in optical microscopy, this examination has revealed lanthanide degradation of the cladding by what appears to be a grain boundary facilitated pathway. Precipitates of fission produced Pd-lanthanide compounds were observed in the fuel. Furthermore, precipitated regions with elevated Mo and elevated W content were also observed in the HT-9 cladding of this sample.},
doi = {10.1016/j.jnucmat.2017.07.040},
journal = {Journal of Nuclear Materials},
number = C,
volume = 494,
place = {United States},
year = {Sat Jul 22 00:00:00 EDT 2017},
month = {Sat Jul 22 00:00:00 EDT 2017}
}

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