Dimensional crossover in the quasi-one-dimensional superconductor Tl2Mo6Se6

Mitra, S.; Petrović, A. P.; Salloum, D.; Gougeon, P.; Potel, M.; Zhu, Jian -Xin; Panagopoulos, C.; Chia, Elbert E. M.

doi:10.1103/PhysRevB.98.054507

Title: Dimensional crossover in the quasi-one-dimensional superconductor ${Tl}_{2} {Mo}_{6} {Se}_{6}$

Journal Article · 14 August 2018 · Physical Review B

DOI: https://doi.org/10.1103/PhysRevB.98.054507 · OSTI ID:1477720

Mitra, S. ^[1]; Petrović, A. P. ^[1]; Salloum, D. ^[2]; Gougeon, P. ^[3]; Potel, M. ^[3];

^[4]; Panagopoulos, C. ^[1]; Chia, Elbert E. M. ^[1]

Nanyang Technological Univ. (Singapore)
Univ. de Rennes, Rennes Cedex (France); Lebanese Univ., Kobbeh-Tripoli (Lebanon)
Univ. de Rennes, Rennes Cedex (France)
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)

Here, we present magnetic penetration depth and electrical transport data in single crystals of quasi-one-dimensional (q1D) Tl₂Mo₆Se₆, which reveal a 1D→3D superconducting dimensional crossover. The c-axis penetration depth shows the onset of superconducting fluctuations below T^ons_1D = 6.7 K, whereas signatures of superconductivity in the ab-plane penetration depth (a uniquely sensitive probe of the transverse phase stiffness) only emerge below T^ons_3D = 4.9 K. An anomalously low superfluid density persists down to ~3 K before rising steeply, in agreement with a theoretical model for crossovers in q1D superconductors. Our data analysis suggests that a sequence of pairing and phase fluctuation regimes controls the unusually broad superconducting transition. In particular, the electrical resistivity below T^ons_3D is quantitatively consistent with the establishment of phase coherence through gradual binding of Josephson vortex strings to form 3D loops. This dimensional crossover within the superconducting state occurs despite the relatively large transverse hopping predicted from the band structure. Furthermore, our results have important consequences for the low-temperature normal state in Tl₂Mo₆Se₆ and similar q1D metals, which may retain one-dimensional behavior to lower temperatures than expected from theory.

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Research Organization:: Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC52-06NA25396; E3B7

OSTI ID:: 1477720

Alternate ID(s):: OSTI ID: 1464580

Report Number(s):: LA-UR-17-28618; PRBMDO

Journal Information:: Physical Review B, Vol. 98, Issue 5; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 8 works

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Title: Dimensional crossover in the quasi-one-dimensional superconductor ${Tl}_{2} {Mo}_{6} {Se}_{6}$