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Title: Light propagation in a neutron detector based on 6Li glass scintillator particles in an organic matrix

Composite materials consisting of 6Li scintillator particles in an organic matrix can enable thermal neutron detectors with excellent rejection of gamma-ray backgrounds. The efficiency of transporting scintillation light through such a composite is critical to the detector performance. This optical raytracing study of a composite thermal neutron detector quantifies the various sources of scintillation light loss and identifies favorable photomultiplier tube (PMT) readout schemes. The composite material consisted of scintillator cubes within an organic matrix shaped as a right cylinder. The cylinder surface was surrounded by an optical reflector, and the light was detected by PMTs attached to the cylinder end faces. A reflector in direct contact with the composite caused 53% loss of scintillation light. This loss was reduced 8-fold by creating an air gap between the composite and the reflector to allow a fraction of the scintillation light to propagate by total internal reflection. Replacing a liquid mineral oil matrix with a solid acrylic matrix decreased the light transport efficiency by only ~10% for the benefit of creating an all-solid-state device. The light propagation loss was found to scale exponentially with the distance between the scintillation event and the PMT along the cylinder main axis. This enabled amore » PMT readout scheme that corrects for light propagation loss on an event-by-event basis and achieved a 4.0% energy resolution that approached Poisson-limited performance. These results demonstrate that composite materials can enable practical thermal neutron detectors for a wide range of nuclear non-proliferation and safeguard applications.« less
Authors:
ORCiD logo [1] ;  [1] ;  [1] ;  [1] ;  [1]
  1. Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Publication Date:
Report Number(s):
LA-UR-18-25954
Journal ID: ISSN 0021-8979
Grant/Contract Number:
AC52-06NA25396
Type:
Accepted Manuscript
Journal Name:
Journal of Applied Physics
Additional Journal Information:
Journal Volume: 124; Journal Issue: 12; Journal ID: ISSN 0021-8979
Publisher:
American Institute of Physics (AIP)
Research Org:
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Sponsoring Org:
USDOE National Nuclear Security Administration (NNSA), Office of Defense Nuclear Nonproliferation (NA-20)
Country of Publication:
United States
Language:
English
Subject:
46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND TECHNOLOGY; photocathodes; gamma rays; optical reflectors; photomultipliers; scintillators; neutron detectors; composite materials; luminescence; solid-state devices
OSTI Identifier:
1477701
Alternate Identifier(s):
OSTI ID: 1474776

Hehlen, Markus P., Wiggins, Brenden W., Favalli, Andrea, Iliev, Metodi, and Ianakiev, Kiril D.. Light propagation in a neutron detector based on 6Li glass scintillator particles in an organic matrix. United States: N. p., Web. doi:10.1063/1.5047433.
Hehlen, Markus P., Wiggins, Brenden W., Favalli, Andrea, Iliev, Metodi, & Ianakiev, Kiril D.. Light propagation in a neutron detector based on 6Li glass scintillator particles in an organic matrix. United States. doi:10.1063/1.5047433.
Hehlen, Markus P., Wiggins, Brenden W., Favalli, Andrea, Iliev, Metodi, and Ianakiev, Kiril D.. 2018. "Light propagation in a neutron detector based on 6Li glass scintillator particles in an organic matrix". United States. doi:10.1063/1.5047433. https://www.osti.gov/servlets/purl/1477701.
@article{osti_1477701,
title = {Light propagation in a neutron detector based on 6Li glass scintillator particles in an organic matrix},
author = {Hehlen, Markus P. and Wiggins, Brenden W. and Favalli, Andrea and Iliev, Metodi and Ianakiev, Kiril D.},
abstractNote = {Composite materials consisting of 6Li scintillator particles in an organic matrix can enable thermal neutron detectors with excellent rejection of gamma-ray backgrounds. The efficiency of transporting scintillation light through such a composite is critical to the detector performance. This optical raytracing study of a composite thermal neutron detector quantifies the various sources of scintillation light loss and identifies favorable photomultiplier tube (PMT) readout schemes. The composite material consisted of scintillator cubes within an organic matrix shaped as a right cylinder. The cylinder surface was surrounded by an optical reflector, and the light was detected by PMTs attached to the cylinder end faces. A reflector in direct contact with the composite caused 53% loss of scintillation light. This loss was reduced 8-fold by creating an air gap between the composite and the reflector to allow a fraction of the scintillation light to propagate by total internal reflection. Replacing a liquid mineral oil matrix with a solid acrylic matrix decreased the light transport efficiency by only ~10% for the benefit of creating an all-solid-state device. The light propagation loss was found to scale exponentially with the distance between the scintillation event and the PMT along the cylinder main axis. This enabled a PMT readout scheme that corrects for light propagation loss on an event-by-event basis and achieved a 4.0% energy resolution that approached Poisson-limited performance. These results demonstrate that composite materials can enable practical thermal neutron detectors for a wide range of nuclear non-proliferation and safeguard applications.},
doi = {10.1063/1.5047433},
journal = {Journal of Applied Physics},
number = 12,
volume = 124,
place = {United States},
year = {2018},
month = {9}
}

Works referenced in this record:

Securing special nuclear material: Recent advances in neutron detection and their role in nonproliferation
journal, December 2010
  • Runkle, R. C.; Bernstein, A.; Vanier, P. E.
  • Journal of Applied Physics, Vol. 108, Issue 11, Article No. 111101
  • DOI: 10.1063/1.3503495

Lithium glass scintillator neutron detector as an improved alternative to the standard 3 he proportional counter
conference, October 2010