Enhanced quantum efficiency of photoelectron emission, through surface textured metal electrodes
Abstract
Here, it is predicted that the quantum efficiency (QE) of photoelectron emission from metals may be enhanced, possibly by an order of magnitude, through optimized surface texture. Through extensive computational simulations, it is shown that the absorption enhancement in select surface groove geometries may be a dominant contributor to enhanced QE and corresponds to localized Fabry–Perot resonances. Finally, the inadequacy of extant analytical models in predicting the QE increase, and suggestions for further improvement, are discussed.
- Authors:
-
- Univ. of California, San Diego, CA (United States). Program in Materials Science. Dept. of Mechanical Engineering
- Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
- Publication Date:
- Research Org.:
- Los Alamos National Laboratory (LANL), Los Alamos, NM (United States); Univ. of California, San Diego, CA (United States)
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1477689
- Alternate Identifier(s):
- OSTI ID: 1421139
- Report Number(s):
- LA-UR-17-28079
Journal ID: ISSN 0734-2101
- Grant/Contract Number:
- AC52-06NA25396
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Journal of Vacuum Science and Technology A
- Additional Journal Information:
- Journal Volume: 34; Journal Issue: 2; Journal ID: ISSN 0734-2101
- Publisher:
- American Vacuum Society
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 42 ENGINEERING
Citation Formats
Alexander, Anna, Moody, Nathan A., and Bandaru, Prabhakar R. Enhanced quantum efficiency of photoelectron emission, through surface textured metal electrodes. United States: N. p., 2015.
Web. doi:10.1116/1.4936082.
Alexander, Anna, Moody, Nathan A., & Bandaru, Prabhakar R. Enhanced quantum efficiency of photoelectron emission, through surface textured metal electrodes. United States. https://doi.org/10.1116/1.4936082
Alexander, Anna, Moody, Nathan A., and Bandaru, Prabhakar R. Mon .
"Enhanced quantum efficiency of photoelectron emission, through surface textured metal electrodes". United States. https://doi.org/10.1116/1.4936082. https://www.osti.gov/servlets/purl/1477689.
@article{osti_1477689,
title = {Enhanced quantum efficiency of photoelectron emission, through surface textured metal electrodes},
author = {Alexander, Anna and Moody, Nathan A. and Bandaru, Prabhakar R.},
abstractNote = {Here, it is predicted that the quantum efficiency (QE) of photoelectron emission from metals may be enhanced, possibly by an order of magnitude, through optimized surface texture. Through extensive computational simulations, it is shown that the absorption enhancement in select surface groove geometries may be a dominant contributor to enhanced QE and corresponds to localized Fabry–Perot resonances. Finally, the inadequacy of extant analytical models in predicting the QE increase, and suggestions for further improvement, are discussed.},
doi = {10.1116/1.4936082},
journal = {Journal of Vacuum Science and Technology A},
number = 2,
volume = 34,
place = {United States},
year = {Mon Nov 23 00:00:00 EST 2015},
month = {Mon Nov 23 00:00:00 EST 2015}
}
Free Publicly Available Full Text
Publisher's Version of Record
Other availability
Cited by: 6 works
Citation information provided by
Web of Science
Web of Science
Save to My Library
You must Sign In or Create an Account in order to save documents to your library.
Works referenced in this record:
Exact eigenfunctions for square-wave gratings: Application to diffraction and surface-plasmon calculations
journal, September 1982
- Sheng, Ping; Stepleman, R. S.; Sanda, P. N.
- Physical Review B, Vol. 26, Issue 6
Why Metallic Surfaces with Grooves a Few Nanometers Deep and Wide May Strongly Absorb Visible Light
journal, February 2008
- Le Perchec, J.; Quémerais, P.; Barbara, A.
- Physical Review Letters, Vol. 100, Issue 6
Cathode R&D for future light sources
journal, October 2010
- Dowell, D. H.; Bazarov, I.; Dunham, B.
- Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 622, Issue 3
In situ cleaning of metal cathodes using a hydrogen ion beam
journal, June 2006
- Dowell, D. H.; King, F. K.; Kirby, R. E.
- Physical Review Special Topics - Accelerators and Beams, Vol. 9, Issue 6
Photoemission Studies of Copper and Silver: Theory
journal, November 1964
- Berglund, C. N.; Spicer, W. E.
- Physical Review, Vol. 136, Issue 4A
Quantum efficiency and thermal emittance of metal photocathodes
journal, July 2009
- Dowell, David H.; Schmerge, John F.
- Physical Review Special Topics - Accelerators and Beams, Vol. 12, Issue 7
Electron dynamics of aluminum investigated by means of time-resolved photoemission
conference, April 1998
- Bauer, M.; Pawlik, S.; Aeschlimann, Martin
- SPIE Proceedings
Range of Excited Electrons in Metals
journal, May 1962
- Quinn, John J.
- Physical Review, Vol. 126, Issue 4
Theory of the Energy Distribution of Photoelectrons
journal, May 1933
- DuBridge, Lee A.
- Physical Review, Vol. 43, Issue 9
Generalized electron emission model for field, thermal, and photoemission
journal, November 2002
- Jensen, Kevin L.; O’Shea, Patrick G.; Feldman, Donald W.
- Applied Physics Letters, Vol. 81, Issue 20
Works referencing / citing this record:
Quantum Efficiency Enhancement of Bialkali Photocathodes by an Atomically Thin Layer on Substrates
journal, October 2019
- Yamaguchi, Hisato; Liu, Fangze; DeFazio, Jeffrey
- physica status solidi (a), Vol. 216, Issue 23
Quantum Efficiency Enhancement of Bialkali Photocathodes by an Atomically Thin Layer on Substrates
journal, October 2019
- Yamaguchi, Hisato; Liu, Fangze; DeFazio, Jeffrey
- physica status solidi (a), Vol. 216, Issue 23
Time-resolved XUV ARPES with tunable 24–33 eV laser pulses at 30 meV resolution
journal, August 2019
- Sie, Edbert J.; Rohwer, Timm; Lee, Changmin
- Nature Communications, Vol. 10, Issue 1
Time-resolved XUV ARPES with tunable 24–33 eV laser pulses at 30 meV resolution
journal, August 2019
- Sie, Edbert J.; Rohwer, Timm; Lee, Changmin
- Nature Communications, Vol. 10, Issue 1