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Title: Low-lying states in Ra 219 and Rn 215 : Sampling microsecond α -decaying nuclei

Abstract

© 2018 American Physical Society. Short-lived α-decaying nuclei "northeast" of Pb208 in the chart of nuclides were studied using the reaction Ca48+Am243 with the decay station TASISpec at TASCA, GSI Darmstadt. Decay energies and times from pile-up events were extracted with a tailor-made pulse-shape analysis routine and specific α-decay chains were identified in a correlation analysis. Decay chains starting with the even-even Ra220 and its odd-A neighbors, Fr219, and Ra221,219, with a focus on the Ra219→Rn215 decay, were studied by means of α-γ spectroscopy. A revised α-decay scheme of Ra219 is proposed, including a new decay branch from a previously not considered isomeric state at 17 keV excitation energy. Conclusions on nuclear structure are drawn from the experimental data, aided by Geant4 simulations and a discussion on theoretical calculations.

Authors:
 [1];  [1];  [1];  [1];  [1];  [1];  [1];  [1];  [1];  [2];  [3];  [4];  [5];  [6];  [7];  [4];  [8];  [9];  [10];  [5] more »;  [10];  [11];  [12];  [13];  [5];  [13];  [5];  [5];  [7];  [5];  [5];  [5];  [14];  [8];  [15];  [12];  [16]; ORCiD logo [11];  [5];  [5];  [5];  [8];  [7];  [5];  [17];  [12];  [8];  [5] « less
  1. Lund Univ., Lund (Sweden)
  2. GSI Helmholtzzentrum für Schwerionenforschung GmbH, Darmstadt (Germany); GANIL, Caen (France)
  3. Helmholtz Inst. Mainz, Mainz (Germany)
  4. GSI Helmholtzzentrum für Schwerionenforschung GmbH, Darmstadt (Germany); Helmholtz Inst. Mainz, Mainz (Germany); Johannes Gutenberg-Univ. Mainz, Mainz (Germany)
  5. GSI Helmholtzzentrum für Schwerionenforschung GmbH, Darmstadt (Germany)
  6. Univ. of Liverpool, Liverpool (United Kingdom); Lund Univ., Lund (Sweden)
  7. Johannes Gutenberg-Univ. Mainz, Mainz (Germany)
  8. Helmholtz Inst. Mainz, Mainz (Germany); Johannes Gutenberg-Univ. Mainz, Mainz (Germany)
  9. Helmholtz Inst. Mainz, Mainz (Germany); Groningen, Groningen (Netherlands)
  10. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
  11. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
  12. Univ. of Liverpool, Liverpool (United Kingdom)
  13. GSI Helmholtzzentrum für Schwerionenforschung GmbH, Darmstadt (Germany); Helmholtz Inst. Mainz, Mainz (Germany)
  14. Univ. of Liverpool, Liverpool (United Kingdom); Helmholtz Inst. Mainz, Mainz (Germany)
  15. Univ. of Oslo, Oslo (Norway)
  16. GSI Helmholtzzentrum für Schwerionenforschung GmbH, Darmstadt (Germany); Johannes Gutenberg-Univ. Mainz, Mainz (Germany)
  17. Paul Scherrer Inst. and Univ. of Bern, Villigen (Switzerland)
Publication Date:
Research Org.:
Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States); Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Nuclear Physics (NP)
OSTI Identifier:
1571859
Alternate Identifier(s):
OSTI ID: 1477543; OSTI ID: 1650034
Grant/Contract Number:  
AC05-00OR22725; AC02-05CH11231
Resource Type:
Accepted Manuscript
Journal Name:
Physical Review C
Additional Journal Information:
Journal Volume: 98; Journal Issue: 4; Journal ID: ISSN 2469-9985
Publisher:
American Physical Society (APS)
Country of Publication:
United States
Language:
English
Subject:
73 NUCLEAR PHYSICS AND RADIATION PHYSICS

Citation Formats

Såmark-Roth, A., Sarmiento, L. G., Rudolph, D., Ljungberg, J., Carlsson, B. G., Fahlander, C., Forsberg, U., Golubev, P., Ragnarsson, I., Ackermann, D., Andersson, L. -L., Block, M., Brand, H., Cox, D. M., Di Nitto, A., Düllmann, Ch. E., Eberhardt, K., Even, J., Gates, J. M., Gerl, J., Gregorich, K. E., Gross, C. J., Herzberg, R. -D., Heßberger, F. P., Jäger, E., Khuyagbaatar, J., Kindler, B., Kojouharov, I., Kratz, J. V., Krier, J., Kurz, N., Lommel, B., Mistry, A., Mokry, C., Omtvedt, J. P., Papadakis, P., Runke, J., Rykaczewski, Krzysztof, Schädel, M., Schaffner, H., Schausten, B., Thörle-Pospiech, P., Trautmann, N., Torres, T., Türler, A., Ward, A., Wiehl, N., and Yakushev, A. Low-lying states in Ra219 and Rn215: Sampling microsecond α-decaying nuclei. United States: N. p., 2018. Web. doi:10.1103/PhysRevC.98.044307.
Såmark-Roth, A., Sarmiento, L. G., Rudolph, D., Ljungberg, J., Carlsson, B. G., Fahlander, C., Forsberg, U., Golubev, P., Ragnarsson, I., Ackermann, D., Andersson, L. -L., Block, M., Brand, H., Cox, D. M., Di Nitto, A., Düllmann, Ch. E., Eberhardt, K., Even, J., Gates, J. M., Gerl, J., Gregorich, K. E., Gross, C. J., Herzberg, R. -D., Heßberger, F. P., Jäger, E., Khuyagbaatar, J., Kindler, B., Kojouharov, I., Kratz, J. V., Krier, J., Kurz, N., Lommel, B., Mistry, A., Mokry, C., Omtvedt, J. P., Papadakis, P., Runke, J., Rykaczewski, Krzysztof, Schädel, M., Schaffner, H., Schausten, B., Thörle-Pospiech, P., Trautmann, N., Torres, T., Türler, A., Ward, A., Wiehl, N., & Yakushev, A. Low-lying states in Ra219 and Rn215: Sampling microsecond α-decaying nuclei. United States. https://doi.org/10.1103/PhysRevC.98.044307
Såmark-Roth, A., Sarmiento, L. G., Rudolph, D., Ljungberg, J., Carlsson, B. G., Fahlander, C., Forsberg, U., Golubev, P., Ragnarsson, I., Ackermann, D., Andersson, L. -L., Block, M., Brand, H., Cox, D. M., Di Nitto, A., Düllmann, Ch. E., Eberhardt, K., Even, J., Gates, J. M., Gerl, J., Gregorich, K. E., Gross, C. J., Herzberg, R. -D., Heßberger, F. P., Jäger, E., Khuyagbaatar, J., Kindler, B., Kojouharov, I., Kratz, J. V., Krier, J., Kurz, N., Lommel, B., Mistry, A., Mokry, C., Omtvedt, J. P., Papadakis, P., Runke, J., Rykaczewski, Krzysztof, Schädel, M., Schaffner, H., Schausten, B., Thörle-Pospiech, P., Trautmann, N., Torres, T., Türler, A., Ward, A., Wiehl, N., and Yakushev, A. Tue . "Low-lying states in Ra219 and Rn215: Sampling microsecond α-decaying nuclei". United States. https://doi.org/10.1103/PhysRevC.98.044307. https://www.osti.gov/servlets/purl/1571859.
@article{osti_1571859,
title = {Low-lying states in Ra219 and Rn215: Sampling microsecond α-decaying nuclei},
author = {Såmark-Roth, A. and Sarmiento, L. G. and Rudolph, D. and Ljungberg, J. and Carlsson, B. G. and Fahlander, C. and Forsberg, U. and Golubev, P. and Ragnarsson, I. and Ackermann, D. and Andersson, L. -L. and Block, M. and Brand, H. and Cox, D. M. and Di Nitto, A. and Düllmann, Ch. E. and Eberhardt, K. and Even, J. and Gates, J. M. and Gerl, J. and Gregorich, K. E. and Gross, C. J. and Herzberg, R. -D. and Heßberger, F. P. and Jäger, E. and Khuyagbaatar, J. and Kindler, B. and Kojouharov, I. and Kratz, J. V. and Krier, J. and Kurz, N. and Lommel, B. and Mistry, A. and Mokry, C. and Omtvedt, J. P. and Papadakis, P. and Runke, J. and Rykaczewski, Krzysztof and Schädel, M. and Schaffner, H. and Schausten, B. and Thörle-Pospiech, P. and Trautmann, N. and Torres, T. and Türler, A. and Ward, A. and Wiehl, N. and Yakushev, A.},
abstractNote = {© 2018 American Physical Society. Short-lived α-decaying nuclei "northeast" of Pb208 in the chart of nuclides were studied using the reaction Ca48+Am243 with the decay station TASISpec at TASCA, GSI Darmstadt. Decay energies and times from pile-up events were extracted with a tailor-made pulse-shape analysis routine and specific α-decay chains were identified in a correlation analysis. Decay chains starting with the even-even Ra220 and its odd-A neighbors, Fr219, and Ra221,219, with a focus on the Ra219→Rn215 decay, were studied by means of α-γ spectroscopy. A revised α-decay scheme of Ra219 is proposed, including a new decay branch from a previously not considered isomeric state at 17 keV excitation energy. Conclusions on nuclear structure are drawn from the experimental data, aided by Geant4 simulations and a discussion on theoretical calculations.},
doi = {10.1103/PhysRevC.98.044307},
journal = {Physical Review C},
number = 4,
volume = 98,
place = {United States},
year = {Tue Oct 09 00:00:00 EDT 2018},
month = {Tue Oct 09 00:00:00 EDT 2018}
}

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H.</span> </li> <li> Physics Letters B, Vol. 771</li> <li> <span class="text-muted related-url">DOI: <a href="https://doi.org/10.1016/j.physletb.2017.03.074" class="text-muted" target="_blank" rel="noopener noreferrer">10.1016/j.physletb.2017.03.074<span class="fa fa-external-link" aria-hidden="true"></span></a></span> </li> </ul> <hr/> </div> <div> <h2 class="title" style="margin-bottom:0;" data-apporder=""> <a href="https://doi.org/10.1016/0168-9002(94)91652-7" target="_blank" rel="noopener noreferrer" class="name">Digital techniques for real-time pulse shaping in radiation measurements<span class="fa fa-external-link" aria-hidden="true"></span></a> <small class="text-muted" style="text-transform:uppercase; font-size:0.75rem;"><br/> <span class="type">journal</span>, <span class="date" data-date="1994-12-01">December 1994</span></small> </h2> <ul class="small references-list" style="list-style-type:none; margin-top: 0.5em; padding-left: 0; line-height:1.8em;"> <li> <span style="color:#5C7B2D;"> Jordanov, Valentin T.; Knoll, Glenn F.; Huber, Alan C.</span> </li> <li> Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 353, Issue 1-3</li> <li> <span class="text-muted related-url">DOI: <a href="https://doi.org/10.1016/0168-9002(94)91652-7" class="text-muted" target="_blank" rel="noopener noreferrer">10.1016/0168-9002(94)91652-7<span class="fa fa-external-link" aria-hidden="true"></span></a></span> </li> </ul> <hr/> </div> <div> <h2 class="title" style="margin-bottom:0;" data-apporder=""> <a href="https://doi.org/10.1103/PhysRevC.96.014324" target="_blank" rel="noopener noreferrer" class="name"><math> <mi>α</mi> </math> -decay chain of the short-lived isotope <math> <mmultiscripts> <mi mathvariant="bold">Pa</mi> <mprescripts/> <none/> <mn>220</mn> </mmultiscripts> </math> established using a digital pulse processing technique<span class="fa fa-external-link" aria-hidden="true"></span></a> <small class="text-muted" style="text-transform:uppercase; font-size:0.75rem;"><br/> <span class="type">journal</span>, <span class="date" data-date="2017-07-01">July 2017</span></small> </h2> <ul class="small references-list" style="list-style-type:none; margin-top: 0.5em; padding-left: 0; line-height:1.8em;"> <li> <span style="color:#5C7B2D;"> Huang, T. H.; Zhang, W. Q.; Sun, M. D.</span> </li> <li> Physical Review C, Vol. 96, Issue 1</li> <li> <span class="text-muted related-url">DOI: <a href="https://doi.org/10.1103/PhysRevC.96.014324" class="text-muted" target="_blank" rel="noopener noreferrer">10.1103/PhysRevC.96.014324<span class="fa fa-external-link" aria-hidden="true"></span></a></span> </li> </ul> <hr/> </div> <div> <h2 class="title" style="margin-bottom:0;" data-apporder=""> <a href="https://doi.org/10.1103/PhysRevC.74.044310" target="_blank" rel="noopener noreferrer" class="name">Many-particles–plus–rotor description of magnetic bands at high spin<span class="fa fa-external-link" aria-hidden="true"></span></a> <small class="text-muted" style="text-transform:uppercase; font-size:0.75rem;"><br/> <span class="type">journal</span>, <span class="date" data-date="2006-10-01">October 2006</span></small> </h2> <ul class="small references-list" style="list-style-type:none; margin-top: 0.5em; padding-left: 0; line-height:1.8em;"> <li> <span style="color:#5C7B2D;"> Carlsson, B. G.; Ragnarsson, I.</span> </li> <li> Physical Review C, Vol. 74, Issue 4</li> <li> <span class="text-muted related-url">DOI: <a href="https://doi.org/10.1103/PhysRevC.74.044310" class="text-muted" target="_blank" rel="noopener noreferrer">10.1103/PhysRevC.74.044310<span class="fa fa-external-link" aria-hidden="true"></span></a></span> </li> </ul> <hr/> </div> <div> <h2 class="title" style="margin-bottom:0;" data-apporder=""> <a href="https://doi.org/10.1103/PhysRevC.37.2744" target="_blank" rel="noopener noreferrer" class="name">Reflection-asymmetric rotor model of odd <em>A∼</em> 219 <em>–</em> 229 nuclei<span class="fa fa-external-link" aria-hidden="true"></span></a> <small class="text-muted" style="text-transform:uppercase; font-size:0.75rem;"><br/> <span class="type">journal</span>, <span class="date" data-date="1988-06-01">June 1988</span></small> </h2> <ul class="small references-list" style="list-style-type:none; margin-top: 0.5em; padding-left: 0; line-height:1.8em;"> <li> <span style="color:#5C7B2D;"> Leander, G. A.; Chen, Y. S.</span> </li> <li> Physical Review C, Vol. 37, Issue 6</li> <li> <span class="text-muted related-url">DOI: <a href="https://doi.org/10.1103/PhysRevC.37.2744" class="text-muted" target="_blank" rel="noopener noreferrer">10.1103/PhysRevC.37.2744<span class="fa fa-external-link" aria-hidden="true"></span></a></span> </li> </ul> <hr/> </div> <div> <h2 class="title" style="margin-bottom:0;" data-apporder=""> <a href="https://doi.org/10.1103/PhysRev.182.1329" target="_blank" rel="noopener noreferrer" class="name">Alpha Decay of <math display="inline"> <mrow> <mmultiscripts> <mrow> <mi mathvariant="normal">U</mi> </mrow> <mprescripts/> <mrow/> <mrow> <mn>227</mn> </mrow> <mrow/> <mrow/> </mmultiscripts> </mrow> </math><span class="fa fa-external-link" aria-hidden="true"></span></a> <small class="text-muted" style="text-transform:uppercase; font-size:0.75rem;"><br/> <span class="type">journal</span>, <span class="date" data-date="1969-06-01">June 1969</span></small> </h2> <ul class="small references-list" style="list-style-type:none; margin-top: 0.5em; padding-left: 0; line-height:1.8em;"> <li> <span style="color:#5C7B2D;"> Hahn, R. L.; Roche, M. F.; Toth, K. S.</span> </li> <li> Physical Review, Vol. 182, Issue 4</li> <li> <span class="text-muted related-url">DOI: <a href="https://doi.org/10.1103/PhysRev.182.1329" class="text-muted" target="_blank" rel="noopener noreferrer">10.1103/PhysRev.182.1329<span class="fa fa-external-link" aria-hidden="true"></span></a></span> </li> </ul> <hr/> </div> <div> <h2 class="title" style="margin-bottom:0;" data-apporder=""> <a href="https://doi.org/10.1016/S0168-9002(03)01368-8" target="_blank" rel="noopener noreferrer" class="name">Geant4—a simulation toolkit<span class="fa fa-external-link" aria-hidden="true"></span></a> <small class="text-muted" style="text-transform:uppercase; font-size:0.75rem;"><br/> <span class="type">journal</span>, <span class="date" data-date="2003-07-01">July 2003</span></small> </h2> <ul class="small references-list" style="list-style-type:none; margin-top: 0.5em; padding-left: 0; line-height:1.8em;"> <li> <span style="color:#5C7B2D;"> Agostinelli, S.; Allison, J.; Amako, K.</span> </li> <li> Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 506, Issue 3</li> <li> <span class="text-muted related-url">DOI: <a href="https://doi.org/10.1016/S0168-9002(03)01368-8" class="text-muted" target="_blank" rel="noopener noreferrer">10.1016/S0168-9002(03)01368-8<span class="fa fa-external-link" aria-hidden="true"></span></a></span> </li> </ul> <hr/> </div> <div> <h2 class="title" style="margin-bottom:0;" data-apporder=""> <a href="https://doi.org/10.1103/PhysRevLett.97.082501" target="_blank" rel="noopener noreferrer" class="name">Discovery of <math display="inline"> <mmultiscripts> <mi>Xe</mi> <mprescripts/> <none/> <mn>109</mn> </mmultiscripts> </math> and <math display="inline"> <mmultiscripts> <mi>Te</mi> <mprescripts/> <none/> <mn>105</mn> </mmultiscripts> </math> : Superallowed <math display="inline"> <mi>α</mi> </math> Decay near Doubly Magic <math display="inline"> <mmultiscripts> <mi>Sn</mi> <mprescripts/> <none/> <mn>100</mn> </mmultiscripts> </math><span class="fa fa-external-link" aria-hidden="true"></span></a> <small class="text-muted" style="text-transform:uppercase; font-size:0.75rem;"><br/> <span class="type">journal</span>, <span class="date" data-date="2006-08-01">August 2006</span></small> </h2> <ul class="small references-list" style="list-style-type:none; margin-top: 0.5em; padding-left: 0; line-height:1.8em;"> <li> <span style="color:#5C7B2D;"> Liddick, S. N.; Grzywacz, R.; Mazzocchi, C.</span> </li> <li> Physical Review Letters, Vol. 97, Issue 8</li> <li> <span class="text-muted related-url">DOI: <a href="https://doi.org/10.1103/PhysRevLett.97.082501" class="text-muted" target="_blank" rel="noopener noreferrer">10.1103/PhysRevLett.97.082501<span class="fa fa-external-link" aria-hidden="true"></span></a></span> </li> </ul> <hr/> </div> <div> <h2 class="title" style="margin-bottom:0;" data-apporder=""> <a href="https://doi.org/10.1016/j.nima.2011.11.074" target="_blank" rel="noopener noreferrer" class="name">A Geant4 simulation package for the TASISpec experimental detector setup<span class="fa fa-external-link" aria-hidden="true"></span></a> <small class="text-muted" style="text-transform:uppercase; font-size:0.75rem;"><br/> <span class="type">journal</span>, <span class="date" data-date="2012-03-01">March 2012</span></small> </h2> <ul class="small references-list" style="list-style-type:none; margin-top: 0.5em; padding-left: 0; line-height:1.8em;"> <li> <span style="color:#5C7B2D;"> Sarmiento, L. G.; Andersson, L. -L.; Rudolph, D.</span> </li> <li> Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 667</li> <li> <span class="text-muted related-url">DOI: <a href="https://doi.org/10.1016/j.nima.2011.11.074" class="text-muted" target="_blank" rel="noopener noreferrer">10.1016/j.nima.2011.11.074<span class="fa fa-external-link" aria-hidden="true"></span></a></span> </li> </ul> <hr/> </div> <div> <h2 class="title" style="margin-bottom:0;" data-apporder=""> <a href="https://doi.org/10.1103/RevModPhys.68.349" target="_blank" rel="noopener noreferrer" class="name">Intrinsic reflection asymmetry in atomic nuclei<span class="fa fa-external-link" aria-hidden="true"></span></a> <small class="text-muted" style="text-transform:uppercase; font-size:0.75rem;"><br/> <span class="type">journal</span>, <span class="date" data-date="1996-04-01">April 1996</span></small> </h2> <ul class="small references-list" style="list-style-type:none; margin-top: 0.5em; padding-left: 0; line-height:1.8em;"> <li> <span style="color:#5C7B2D;"> Butler, P. A.; Nazarewicz, W.</span> </li> <li> Reviews of Modern Physics, Vol. 68, Issue 2</li> <li> <span class="text-muted related-url">DOI: <a href="https://doi.org/10.1103/RevModPhys.68.349" class="text-muted" target="_blank" rel="noopener noreferrer">10.1103/RevModPhys.68.349<span class="fa fa-external-link" aria-hidden="true"></span></a></span> </li> </ul> <hr/> </div> </div> <div class="pagination-container small"> <a class="pure-button prev page" href="#" rel="prev"><span class="sr-only">Previous Page</span><span class="fa fa-angle-left"></span></a> <ul class="pagination d-inline-block" style="padding-left:.2em;"></ul> <a class="pure-button next page" href="#" rel="next"><span class="sr-only">Next Page</span><span class="fa fa-angle-right"></span></a> </div> </div> </div> <div class="col-sm-3 order-sm-3"> <ul class="nav nav-stacked"> <li class="active"><a href="" class="reference-type-filter tab-nav" data-tab="biblio-references" data-filter="type" data-pattern="*"><span class="fa fa-angle-right"></span> All References</a></li> <li class="small" style="margin-left:.75em; text-transform:capitalize;"><a href="" class="reference-type-filter tab-nav" data-tab="biblio-references" data-filter="type" data-pattern="journal"><span class="fa fa-angle-right"></span> journal<small class="text-muted"> (49)</small></a></li> </ul> <div style="margin-top:2em;"> <form class="pure-form small text-muted reference-search"> <label for="reference-search-text" class="sr-only">Search</label> <input class="search form-control pure-input-1" id="reference-search-text" placeholder="Search" style="margin-bottom:10px;" /> <fieldset aria-label="Sort By"> <legend class="legend-filters sr-only">Sort by:</legend> <div style="margin-left:1em; font-weight:normal; line-height: 1.6em;"><input type="radio" class="sort" name="references-sort" data-sort="name" style="position:relative;top:2px;" id="reference-search-sort-name"><label for="reference-search-sort-name" style="margin-left: .3em;">Sort by title</label></div> <div style="margin-left:1em; font-weight:normal; line-height: 1.6em;"><input type="radio" class="sort" name="references-sort" data-sort="date" data-order="desc" style="position:relative;top:2px;" id="reference-search-sort-date"><label for="reference-search-sort-date" style="margin-left: .3em;">Sort by date</label></div> </fieldset> <div class="text-left" style="margin-left:1em;"> <a href="" class="filter-clear clearfix" title="Clear filter / sort" style="font-weight:normal; float:none;">[ × clear filter / sort ]</a> </div> <input type="submit" id="sort_submit_references" name="submit" aria-label="submit" style="display: none;"/> </form> </div> </div> </div> </section> <section id="biblio-related" class="tab-content tab-content-sec " data-tab="biblio"> <div class="row"> <div class="col-sm-9 order-sm-9"> <section id="biblio-similar" class="tab-content tab-content-sec active" data-tab="related"> <div class="padding"> <p class="lead text-muted" style="font-size: 18px; margin-top:0px;">Similar Records in DOE PAGES and OSTI.GOV collections:</p> <aside> <ul class="item-list" itemscope itemtype="http://schema.org/ItemList" style="padding-left:0; list-style-type: none;"> <li> <div class="article item document" itemprop="itemListElement" itemscope itemtype="http://schema.org/WebPage"><meta itemprop="position" content="1" /><div class="item-info"> <h2 class="title" itemprop="name headline"><a href="/pages/biblio/1923574-spectroscopy-along-flerovium-decay-chains-iii-details-experiment-analysis-cn-spontaneous-fission-branches" itemprop="url">Spectroscopy along flerovium decay chains. III. Details on experiment, analysis, <math> <mmultiscripts> <mi>Cn</mi> <mprescripts/> <none/> <mn>282</mn> </mmultiscripts> </math> , and spontaneous fission branches</a></h2> <div class="metadata"> <small class="text-muted" style="text-transform:uppercase;display:block;line-height:2.5em;">Journal Article</small><span class="authors"> <span class="author">Såmark-Roth, A.</span> ; <span class="author">Cox, D. M.</span> ; <span class="author">Rudolph, D.</span> ; <span class="author">...</span> <span class="text-muted pubdata"> - Physical Review C</span> </span> </div> <div class="abstract">Flerovium isotopes (element Z = 114) were produced in the fusion-evaporation reactions <sup>48</sup>Ca + <sup>242,244</sup>Pu and studied with an upgraded TASISpec decay station placed in the focal plane of the gas-filled separator TASCA at the GSI Helmholtzzentrum für Schwerionenforschung in Darmstadt, Germany. Twenty-nine flerovium decay chains were identified by means of correlated implantation, α decay, and spontaneous fission events. Data analysis aspects and statistical assessments, primarily based on measured rates of various events, which laid the foundation for the comprehensive spectroscopic information on the flerovium decay chains, are presented in detail. Various decay scenarios of an excited state observed in<a href='#' onclick='$(this).hide().next().show().next().show();return false;' style='margin-left:10px;'>more »</a><span style='display:none;'> <sup>282</sup>Cn are examined in depth with the help of Geant4 simulations and assessed by predictions of beyond mean-field calculations including triaxial shape degrees of freedom. Previous, revised, and newly derived fission probabilities of even-even superheavy nuclei are compared with various theoretical predictions.</span><a href='#' onclick='$(this).hide().prev().hide().prev().show();return false;' style='margin-left:10px;display:none;'>« less</a></div><div class="metadata-links small clearfix text-muted" style="margin-top:15px;"> <div class="pure-menu pure-menu-horizontal pull-right" style="width:unset;"> <ul class="pure-menu-list"> <li class="pure-menu-item"><span class="item-info-ftlink"><a class="misc doi-link " href="https://doi.org/10.1103/PhysRevC.107.024301" target="_blank" rel="noopener" title="Link to document DOI" data-ostiid="1923574" data-product-type="Journal Article" data-product-subtype="PA" >https://doi.org/10.1103/PhysRevC.107.024301</a></span></li> </ul> </div> </div> </div> <div class="clearfix"></div> </div> </li> <li> <div class="article item document" itemprop="itemListElement" itemscope itemtype="http://schema.org/WebPage"><meta itemprop="position" content="2" /><div class="item-info"> <h2 class="title" itemprop="name headline"><a href="/pages/biblio/1761549-spectroscopy-along-flerovium-decay-chains-discovery-ds-excited-state-cn" itemprop="url">Spectroscopy along Flerovium Decay Chains: Discovery of <math> <mrow> <mmultiscripts> <mrow> <mi>Ds</mi> </mrow> <mprescripts/> <none/> <mrow> <mn>280</mn> </mrow> </mmultiscripts> </mrow> </math> and an Excited State in <math> <mrow> <mmultiscripts> <mrow> <mi>Cn</mi> </mrow> <mprescripts/> <none/> <mrow> <mn>282</mn> </mrow> </mmultiscripts> </mrow> </math></a></h2> <div class="metadata"> <small class="text-muted" style="text-transform:uppercase;display:block;line-height:2.5em;">Journal Article</small><span class="authors"> <span class="author">Såmark-Roth, A.</span> ; <span class="author">Cox, D. M.</span> ; <span class="author">Rudolph, D.</span> ; <span class="author">...</span> <span class="text-muted pubdata"> - Physical Review Letters</span> </span> </div> <div class="abstract">A nuclear spectroscopy experiment was conducted to study α-decay chains stemming from isotopes of flerovium (element Z=114). An upgraded TASISpec decay station was placed behind the gas-filled separator TASCA at the GSI Helmholtzzentrum für Schwerionenforschung in Darmstadt, Germany. The fusion-evaporation reactions <sup>48</sup>Ca + <sup>242</sup>Pu and <sup>48</sup>Ca + <sup>244</sup>Pu provided a total of 32 flerovium-candidate decay chains, of which two and eleven were firmly assigned to <sup>286</sup>Fl and <sup>288</sup>Fl, respectively. A prompt coincidence between a 9.60(1)-MeV α particle event and a 0.36(1)-MeV conversion electron marked the first observation of an excited state in an even-even isotope of the heaviest man-made elements,<a href='#' onclick='$(this).hide().next().show().next().show();return false;' style='margin-left:10px;'>more »</a><span style='display:none;'> namely <sup>282</sup>Cn. Spectroscopy of <sup>288</sup>Fl decay chains fixed Q<sub>α</sub> = 10.06(1) MeV. In one case, a Q<sub>α</sub> = 9.46(1)-MeV decay from <sup>284</sup>Cn into <sup>280</sup>Ds was observed, with <sup>280</sup>Ds fissioning after only 518 μs. The impact of these findings, aggregated with existing data on decay chains of <sup>286,288</sup>Fl, on the size of an anticipated shell gap at proton number Z = 114 is discussed in light of predictions from two beyond-mean-field calculations, which take into account triaxial deformation.</span><a href='#' onclick='$(this).hide().prev().hide().prev().show();return false;' style='margin-left:10px;display:none;'>« less</a></div><div class="metadata-links small clearfix text-muted" style="margin-top:15px;"> <div class="pure-menu pure-menu-horizontal pull-right" style="width:unset;"> <ul class="pure-menu-list"> <li class="pure-menu-item"><span class="item-info-ftlink"><a class="misc doi-link " href="https://doi.org/10.1103/PhysRevLett.126.032503" target="_blank" rel="noopener" title="Link to document DOI" data-ostiid="1761549" data-product-type="Journal Article" data-product-subtype="PA" >https://doi.org/10.1103/PhysRevLett.126.032503</a></span></li> </ul> </div> </div> </div> <div class="clearfix"></div> </div> </li> <li> <div class="article item document" itemprop="itemListElement" itemscope itemtype="http://schema.org/WebPage"><meta itemprop="position" content="5" /><div class="item-info"> <h2 class="title" itemprop="name headline"><a href="/pages/biblio/1430686-decay-high-isomers-ds270-hs266-superfluid-tunneling-model" itemprop="url"><math> <mi>α</mi> </math> decay of high- <i>K</i> isomers in <math> <mmultiscripts> <mi>Ds</mi><mprescripts/><none/> <mn>270</mn> </mmultiscripts> </math> and <math> <mmultiscripts> <mi>Hs</mi><mprescripts/><none/> <mn>266</mn> </mmultiscripts> </math> in a superfluid tunneling model</a></h2> <div class="metadata"> <small class="text-muted" style="text-transform:uppercase;display:block;line-height:2.5em;">Journal Article</small><span class="authors"> <span class="author">Clark, R. M.</span> ; <span class="author">Rudolph, D.</span> <span class="text-muted pubdata"> - Physical Review C</span> </span> </div> <div class="abstract">Here, we use the superfluid tunneling model (STM) to calculate the half-lives of ground-state α decays of even-even superheavy nuclei (SHN) with Z ≥ 100 . The experimental data are reproduced to accuracies comparable to other contemporary models of α decay of SHN. We apply the STM to the case of the α decaying high-K isomers identified in the decay chains of <sup>270</sup>Ds . By accounting for the α -decay Q values, Q<sub>α</sub>, the angular momentum difference between initial and final states, L, and a reduction in the pairing gap, Δ, we are able to reproduce the observed α decay<a href='#' onclick='$(this).hide().next().show().next().show();return false;' style='margin-left:10px;'>more »</a><span style='display:none;'> of the isomers, including the unusual competition between L ≈ 10 and L ≈ 0 α branches seen for the K isomer in <sup>270</sup>Ds ( Z = 110 ).</span><a href='#' onclick='$(this).hide().prev().hide().prev().show();return false;' style='margin-left:10px;display:none;'>« less</a></div><div class="metadata-links small clearfix text-muted" style="margin-top:15px;"> <span class="fa fa-book text-muted" aria-hidden="true"></span> Cited by 12<div class="pure-menu pure-menu-horizontal pull-right" style="width:unset;"> <ul class="pure-menu-list"> <li class="pure-menu-item"><span class="item-info-ftlink"><a class="misc doi-link " href="https://doi.org/10.1103/PhysRevC.97.024333" target="_blank" rel="noopener" title="Link to document DOI" data-ostiid="1430686" data-product-type="Journal Article" data-product-subtype="AM" >https://doi.org/10.1103/PhysRevC.97.024333</a></span></li> <li class="pure-menu-item"><span class="item-info-ftlink"><a class="misc fulltext-link " href="/pages/servlets/purl/1430686" title="Link to document media" target="_blank" rel="noopener" data-ostiid="1430686" data-product-type="Journal Article" data-product-subtype="AM" >Full Text Available</a></span></li> </ul> </div> </div> </div> <div class="clearfix"></div> </div> </li> <li> <div class="article item document" itemprop="itemListElement" itemscope itemtype="http://schema.org/WebPage"><meta itemprop="position" content="8" /><div class="item-info"> <h2 class="title" itemprop="name headline"><a href="/pages/biblio/1332816-recoil-fission-recoil-fission-events-observed-reaction" itemprop="url">Recoil-α-fission and recoil-α–α-fission events observed in the reaction <sup>48</sup>Ca + <sup>243</sup>Am</a></h2> <div class="metadata"> <small class="text-muted" style="text-transform:uppercase;display:block;line-height:2.5em;">Journal Article</small><span class="authors"> <span class="author">Forsberg, Ulrika</span> ; <span class="author">Rudolph, D.</span> ; <span class="author">Andersson, L. -L.</span> ; <span class="author">...</span> <span class="text-muted pubdata"> - Nuclear Physics. A</span> </span> </div> <div class="abstract">Products of the fusion-evaporation reaction 48Ca + 243Am were studied with the TASISpec set-up at the gas-filled separator TASCA at the GSI Helmholtzzentrum für Schwerionenforschung, Darmstadt, Germany. Amongst the detected thirty correlated α-decay chains associated with the production of element , two recoil-α-fission and five recoil--fission events were observed. The latter five chains are similar to four such events reported from experiments performed at the Dubna gas-filled separator, and three such events reported from an experiment at the Berkeley gas-filled separator. The four chains observed at the Dubna gas-filled separator were assigned to start from the 2n-evaporation channel 289 115<a href='#' onclick='$(this).hide().next().show().next().show();return false;' style='margin-left:10px;'>more »</a><span style='display:none;'> due to the fact that these recoil--fission events were observed only at low excitation energies. Contrary to this interpretation, we suggest that some of these recoil--fission decay chains, as well as some of the recoil--fission and recoil-α-fission decay chains reported from Berkeley and in this article, start from the 3n-evaporation channel 288 115.</span><a href='#' onclick='$(this).hide().prev().hide().prev().show();return false;' style='margin-left:10px;display:none;'>« less</a></div><div class="metadata-links small clearfix text-muted" style="margin-top:15px;"> <span class="fa fa-book text-muted" aria-hidden="true"></span> Cited by 44<div class="pure-menu pure-menu-horizontal pull-right" style="width:unset;"> <ul class="pure-menu-list"> <li class="pure-menu-item"><span class="item-info-ftlink"><a class="misc doi-link " href="https://doi.org/10.1016/j.nuclphysa.2016.04.025" target="_blank" rel="noopener" title="Link to document DOI" data-ostiid="1332816" data-product-type="Journal Article" data-product-subtype="AM" >https://doi.org/10.1016/j.nuclphysa.2016.04.025</a></span></li> <li class="pure-menu-item"><span class="item-info-ftlink"><a class="misc fulltext-link " href="/pages/servlets/purl/1332816" title="Link to document media" target="_blank" rel="noopener" data-ostiid="1332816" data-product-type="Journal Article" data-product-subtype="AM" >Full Text Available</a></span></li> </ul> </div> </div> </div> <div class="clearfix"></div> </div> </li> <li> <div class="article item document" itemprop="itemListElement" itemscope itemtype="http://schema.org/WebPage"><meta itemprop="position" content="9" /><div class="item-info"> <h2 class="title" itemprop="name headline"><a href="/pages/biblio/1763497-search-decay-te104-novel-recoil-decay-scintillation-detector" itemprop="url">Search for <math> <mi>α</mi> </math> decay of <math> <mmultiscripts> <mi>Te</mi> <mprescripts></mprescripts> <mn>104</mn> </mmultiscripts> </math> with a novel recoil-decay scintillation detector</a></h2> <div class="metadata"> <small class="text-muted" style="text-transform:uppercase;display:block;line-height:2.5em;">Journal Article</small><span class="authors"> <span class="author">Xiao, Y.</span> ; <span class="author">Go, S.</span> ; <span class="author">Grzywacz, Robert Kazimierz</span> ; <span class="author">...</span> <span class="text-muted pubdata"> - Physical Review C</span> </span> </div> <div class="abstract">A se<a href='#' onclick='$(this).hide().next().show().next().show();return false;' style='margin-left:10px;'>more »</a><span style='display:none;'> arch for superallowed <math> <mi>α</mi> </math> decay of <math> <mrow> <mi>N</mi> <mo>=</mo> <mi>Z</mi> </mrow> </math> nuclei <math> <mmultiscripts> <mi>Te</mi> <mprescripts></mprescripts> <mn>104</mn> </mmultiscripts> </math> and <math> <mmultiscripts> <mi>Xe</mi> <mprescripts></mprescripts> <mn>108</mn> </mmultiscripts> </math> was carried out using a novel recoil-decay scintillator detector at the tandem accelerator facility at the Japan Atomic Energy Agency (JAEA). In this study, inorganic crystal scintillation material YAP:Ce (yttrium aluminum perovskite) coupled to a position-sensitive photomultiplier tube (PSPMT) was implemented for the first time in a radioactive decay experiment. Residues from the fusion-evaporation reaction <math> <mrow> <mmultiscripts> <mi>Ni</mi> <mprescripts></mprescripts> <mn>58</mn> </mmultiscripts> <mo>+</mo> <mmultiscripts> <mi>Fe</mi> <mprescripts></mprescripts> <mn>54</mn> </mmultiscripts> <mspace></mspace> <mo>→</mo> <mspace></mspace> <mmultiscripts> <mi>Xe</mi> <mo>*</mo> <mprescripts></mprescripts> <mn>112</mn> </mmultiscripts> </mrow> </math> were separated by the JAEA Recoil Mass Separator (RMS) and implanted into the YAP:Ce crystal. <math> <mi>α</mi> </math> decays of neutron-deficient tellurium isotopes were identified and proton emission of <math> <mmultiscripts> <mi mathvariant="normal">I</mi> <mprescripts></mprescripts> <mn>109</mn> </mmultiscripts> </math> was observed. The <math> <mi>α</mi> </math>-decay chain <math> <mrow> <mmultiscripts> <mi>Xe</mi> <mprescripts></mprescripts> <mn>109</mn> </mmultiscripts> <mspace></mspace> <mo>→</mo> <mspace></mspace> <mmultiscripts> <mi>Te</mi> <mprescripts></mprescripts> <mn>105</mn> </mmultiscripts> <mspace></mspace> <mo>→</mo> <mspace></mspace> <mmultiscripts> <mi>Sn</mi> <mprescripts></mprescripts> <mn>101</mn> </mmultiscripts> </mrow> </math> was recorded with a time interval of 960 ns between two <math> <mi>α</mi> </math> pulses. Position localization in the crystal for decays and ions in the energy range from hundreds of keV to 60 MeV was achieved with an accuracy of 0.67 mm, proving that this detector is capable of making temporal and spatial correlations for fast decay events. No conclusive evidence was found for the decay chain <math> <mrow> <mmultiscripts> <mi>Xe</mi> <mprescripts></mprescripts> <mn>108</mn> </mmultiscripts> <mspace></mspace> <mo>→</mo> <mspace></mspace> <mmultiscripts> <mi>Te</mi> <mprescripts></mprescripts> <mn>104</mn> </mmultiscripts> <mspace></mspace> <mo>→</mo> <mspace></mspace> <mmultiscripts> <mi>Sn</mi> <mprescripts></mprescripts> <mn>100</mn> </mmultiscripts> </mrow> </math> within 3 days of experiment. However, two events were observed with properties consistent with the reported observation at the Fragment Mass Analyzer (FMA), but with a separation between signals of less than 4 ns. The cross section limit of 130 pb was obtained for production of two events of <math> <mmultiscripts> <mi>Xe</mi> <mprescripts></mprescripts> <mn>108</mn> </mmultiscripts> </math>, about an order of magnitude below the expectation based on earlier cross section measurements and the HIVAP fusion-evaporation code.</span><a href='#' onclick='$(this).hide().prev().hide().prev().show();return false;' style='margin-left:10px;display:none;'>« less</a></div><div class="metadata-links small clearfix text-muted" style="margin-top:15px;"> <div class="pure-menu pure-menu-horizontal pull-right" style="width:unset;"> <ul class="pure-menu-list"> <li class="pure-menu-item"><span class="item-info-ftlink"><a class="misc doi-link " href="https://doi.org/10.1103/physrevc.100.034315" target="_blank" rel="noopener" title="Link to document DOI" data-ostiid="1763497" data-product-type="Journal Article" data-product-subtype="AM" >https://doi.org/10.1103/physrevc.100.034315</a></span></li> <li class="pure-menu-item"><span class="item-info-ftlink"><a class="misc fulltext-link " href="/pages/servlets/purl/1763497" title="Link to document media" target="_blank" rel="noopener" data-ostiid="1763497" data-product-type="Journal Article" data-product-subtype="AM" >Full Text Available</a></span></li> </ul> </div> </div> </div> <div class="clearfix"></div> </div> </li> </ul> </aside> </div> </section> </div> <div class="col-sm-3 order-sm-3"> <ul class="nav nav-stacked"> <li class="active"><a class="tab-nav disabled" data-tab="related" style="color: #636c72 !important; 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