Phase separation at the dimer-superconductor transition in Ir1-xRhxTe2

Yu, Runze; Bozin, Emil S.; Banerjee, S.; Lei, H.; Abeykoon, M.; Petrovic, C.; Guguchia, Z.

doi:10.1103/PhysRevB.98.134506

Title: Phase separation at the dimer-superconductor transition in Ir_1-xRh_xTe₂

Journal Article · 15 October 2018 · Physical Review B

DOI: https://doi.org/10.1103/PhysRevB.98.134506 · OSTI ID:1477484

Yu, Runze ^[1];

^[2]; Banerjee, S. ^[3]; Lei, H. ^[4]; Abeykoon, M. ^[2]; Petrovic, C. ^[2]; Guguchia, Z. ^[5]

Brookhaven National Lab. (BNL), Upton, NY (United States); Chinese Academy of Science, Beijing (People's Republic of China)
Brookhaven National Lab. (BNL), Upton, NY (United States)
Columbia Univ., New York, NY (United States)
Brookhaven National Lab. (BNL), Upton, NY (United States); Renmin Univ., Beijing (People's Republic of China)
Brookhaven National Lab. (BNL), Upton, NY (United States); Columbia Univ., New York, NY (United States)

The detailed evolution of the local atomic structure across the (x, T) phase diagram of transition metal dichalcogenide superconductor Ir_1–xRh_xTe₂ (0≤x≤0.3, 10 K≤T≤300 K) is obtained from high quality x-ray diffraction data using the atomic pair distribution function (PDF) method. Observed hysteretic thermal structural phase transition from trigonal (P3¯m1) to triclinic (P1¯) dimer phase for low Rh content emphasizes intimate connection between the lattice and electronic properties. For superconducting samples away from the dimer/superconductor phase boundary structural transition is absent and the local structure remains trigonal down to 10 K. In the narrow range of compositions close to the boundary PDF analysis reveals structural phase separation, suggestive of weak first order character of the Rh-doping induced dimer-superconductor quantum phase transition. Samples from this narrow range show weak anomalies in electronic transport and magnetization, hallmarks of the dimer phase, as well as superconductivity albeit with incomplete diamagnetic screening. Furthermore, results suggest that the dimer and superconducting orders exist in the mutually exclusive spatial regions

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Research Organization:: Brookhaven National Laboratory (BNL), Upton, NY (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

Grant/Contract Number:: SC0012704

OSTI ID:: 1477484

Report Number(s):: BNL--209163-2018-JAAM

Journal Information:: Physical Review B, Journal Name: Physical Review B Journal Issue: 13 Vol. 98; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Title: Phase separation at the dimer-superconductor transition in Ir_1-xRh_xTe₂