Multi-principal element transition metal dichalcogenides via reactive fusion of 3D-heterostructures

Hlova, Ihor Z.; Dolotko, Oleksandr; Boote, Brett W.; Pathak, Arjun K.; Smith, Emily A.; Pecharsky, Vitalij K.; Balema, Viktor P.

doi:10.1039/C8CC06766J

Title: Multi-principal element transition metal dichalcogenides via reactive fusion of 3D-heterostructures

Journal Article · 24 September 2018 · ChemComm

DOI: https://doi.org/10.1039/C8CC06766J · OSTI ID:1477202

Hlova, Ihor Z. ^[1]; Dolotko, Oleksandr ^[1]; Boote, Brett W. ^[1];

^[1];

^[1]

Ames Lab. and Iowa State Univ., Ames, IA (United States)

Transition metal dichalcogenides combining multiple principal elements in their structures are synthesized via mechanochemical exfoliation and spontaneous reassembly of binary precursors into 3D-heterostructures that are converted into single-phase layered materials by high-temperature reactive fusion. As a result, physical and chemical events enabling these transformations are summarized in the form of a conceivable reaction mechanism.

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Research Organization:: Ames Laboratory (AMES), Ames, IA (United States)

Sponsoring Organization:: USDOE

Grant/Contract Number:: AC02-07CH11358; Laboratory Directed Research and Development (LDRD) program

OSTI ID:: 1477202

Alternate ID(s):: OSTI ID: 1475079

Report Number(s):: IS-J-9760

Journal Information:: ChemComm, Vol. 54, Issue 89; ISSN 1359-7345

Publisher:: Royal Society of ChemistryCopyright Statement

Country of Publication:: United States

Language:: English

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