Multi-principal element transition metal dichalcogenides via reactive fusion of 3D-heterostructures
Abstract
Transition metal dichalcogenides combining multiple principal elements in their structures are synthesized via mechanochemical exfoliation and spontaneous reassembly of binary precursors into 3D-heterostructures that are converted into single-phase layered materials by high-temperature reactive fusion. As a result, physical and chemical events enabling these transformations are summarized in the form of a conceivable reaction mechanism.
- Authors:
-
- Ames Lab. and Iowa State Univ., Ames, IA (United States)
- Publication Date:
- Research Org.:
- Ames Lab., Ames, IA (United States)
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1477202
- Alternate Identifier(s):
- OSTI ID: 1475079
- Report Number(s):
- IS-J-9760
Journal ID: ISSN 1359-7345
- Grant/Contract Number:
- AC02-07CH11358; Laboratory Directed Research and Development (LDRD) program
- Resource Type:
- Accepted Manuscript
- Journal Name:
- ChemComm
- Additional Journal Information:
- Journal Volume: 54; Journal Issue: 89; Journal ID: ISSN 1359-7345
- Publisher:
- Royal Society of Chemistry
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE
Citation Formats
Hlova, Ihor Z., Dolotko, Oleksandr, Boote, Brett W., Pathak, Arjun K., Smith, Emily A., Pecharsky, Vitalij K., and Balema, Viktor P.. Multi-principal element transition metal dichalcogenides via reactive fusion of 3D-heterostructures. United States: N. p., 2018.
Web. doi:10.1039/C8CC06766J.
Hlova, Ihor Z., Dolotko, Oleksandr, Boote, Brett W., Pathak, Arjun K., Smith, Emily A., Pecharsky, Vitalij K., & Balema, Viktor P.. Multi-principal element transition metal dichalcogenides via reactive fusion of 3D-heterostructures. United States. https://doi.org/10.1039/C8CC06766J
Hlova, Ihor Z., Dolotko, Oleksandr, Boote, Brett W., Pathak, Arjun K., Smith, Emily A., Pecharsky, Vitalij K., and Balema, Viktor P.. Mon .
"Multi-principal element transition metal dichalcogenides via reactive fusion of 3D-heterostructures". United States. https://doi.org/10.1039/C8CC06766J. https://www.osti.gov/servlets/purl/1477202.
@article{osti_1477202,
title = {Multi-principal element transition metal dichalcogenides via reactive fusion of 3D-heterostructures},
author = {Hlova, Ihor Z. and Dolotko, Oleksandr and Boote, Brett W. and Pathak, Arjun K. and Smith, Emily A. and Pecharsky, Vitalij K. and Balema, Viktor P.},
abstractNote = {Transition metal dichalcogenides combining multiple principal elements in their structures are synthesized via mechanochemical exfoliation and spontaneous reassembly of binary precursors into 3D-heterostructures that are converted into single-phase layered materials by high-temperature reactive fusion. As a result, physical and chemical events enabling these transformations are summarized in the form of a conceivable reaction mechanism.},
doi = {10.1039/C8CC06766J},
journal = {ChemComm},
number = 89,
volume = 54,
place = {United States},
year = {2018},
month = {9}
}
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Cited by: 7 works
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