Colloidal Binary Supracrystals with Tunable Structural Lattices

Wang, Peng-peng; Qiao, Qiao; Zhu, Yimei; Ouyang, Min

doi:10.1021/jacs.8b05643

Title: Colloidal Binary Supracrystals with Tunable Structural Lattices

Journal Article · 09 July 2018 · Journal of the American Chemical Society

DOI: https://doi.org/10.1021/jacs.8b05643 · OSTI ID:1476758

Wang, Peng-peng ^[1];

^[2]; Zhu, Yimei ^[3];

^[1]

Univ. of Maryland, College Park, MD (United States)
Brookhaven National Lab. (BNL), Upton, NY (United States); Temple Univ., Philadelphia, PA (United States)
Brookhaven National Lab. (BNL), Upton, NY (United States)

Here, colloidal binary supracrystals (SCs) possessing tunable and ordered assembly of two different types of functional nanoparticles (NPs) represent a unique class of artificial materials for both fundamental study and technological applications, but related study has been limited due to substantial challenges in materials growth. Here we report the controlled growth of colloidal binary SCs consisting of Au and Fe₃O₄ NPs via an oil-in-water emulsion process. The size, stoichiometry, and lattice structure of the SCs can be broadly tuned by the growth parameters. Furthermore, our growth method is general and applicable to other NP building blocks to achieve various functional binary SCs. These as-grown free-standing binary SCs should therefore enable new test beds for exploring different nanoscale interactions ranging from the formation and stability of nanoscale binary phase to the emerging magneto-plasmonic coupling physics.

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Research Organization:: Energy Frontier Research Centers (EFRC) (United States). Center for Complex Materials from First Principles (CCM); Brookhaven National Laboratory (BNL), Upton, NY (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

Grant/Contract Number:: SC0012704

OSTI ID:: 1476758

Report Number(s):: BNL--209145-2018-JAAM

Journal Information:: Journal of the American Chemical Society, Journal Name: Journal of the American Chemical Society Journal Issue: 29 Vol. 140; ISSN 0002-7863

Publisher:: American Chemical Society (ACS)Copyright Statement

Country of Publication:: United States

Language:: English

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From Atoms to Lives: The Evolution of Nanoparticle Assemblies Xue, Zhenjie; Yan, Cong; Wang, Tie Advanced Functional Materials, Vol. 29, Issue 12 https://doi.org/10.1002/adfm.201807658	journal	January 2019
Local Acoustic Fields Powered Assembly of Microparticles and Applications Shen, Hui; Zhao, Kangdong; Wang, Zhiwen Micromachines, Vol. 10, Issue 12 https://doi.org/10.3390/mi10120882	journal	December 2019
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Recent Advances in Multicomponent Particle Assembly Guo, Dan; Song, Yanlin Chemistry - A European Journal, Vol. 24, Issue 61 https://doi.org/10.1002/chem.201800264	journal	August 2018
Assembly by solvent evaporation: equilibrium structures and relaxation times Waltmannn, Tommy; Travesset, Alex Nanoscale, Vol. 11, Issue 40 https://doi.org/10.1039/c9nr05908c	journal	January 2019
Supramolecular Modification of ABC Triblock Terpolymers in Confinement Assembly Quintieri, Giada; Saccone, Marco; Spengler, Matthias Nanomaterials, Vol. 8, Issue 12 https://doi.org/10.3390/nano8121029	journal	December 2018

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