Mn-induced Ferromagnetic Semiconducting Behavior with Linear Negative Magnetoresistance in Sr4(Ru1-xMnx)3O10 Single Crystals

Xing, Lingyi; Gui, Xin; Xie, Weiwei; Cao, Huibo; Yan, Jiaqiang; Sales, Brian C.; Jin, Rongying

doi:10.1038/s41598-018-31679-w

Title: Mn-induced Ferromagnetic Semiconducting Behavior with Linear Negative Magnetoresistance in Sr₄(Ru_1-xMn_x)₃O₁₀ Single Crystals

Abstract

Triple-layered Sr₄Ru₃O₁₀ is a unique ferromagnet with the central RuO₆ layer behaving differently from two outer layers both crystallographically and magnetically. Here, we report that the partial substitution of Ru by smaller Mn gives rise to modification in crystal structure, electronic and magnetic properties of Sr₄(Ru_1-xMn_x)₃O₁₀. Through the single crystal X-ray diffraction refinement, we find that (Ru/Mn)O₆ octahedral rotation is no longer detectable at x ≥ 0.23, leading to the tetragonal structure. The magnetization measurements indicate the ferromagnetic transition temperature T_C decreases from 105 K for x = 0 to 30 K for x = 0.41, with the reduced magnetic moment as well. Remarkably, Mn doping results in the change of magnetic anisotropy from the easy c axis in x = 0 to the easy ab plane seen in x = 0.34 and 0.41. Such change also removes the ab-plane metamagnetic transition observed in x = 0. Furthermore, the electrical resistivity increases with increasing x showing semiconducting behavior with Δ ~ 10 meV for x = 0.34 and 30 meV for x = 0.41. Under applied magnetic field, the magnetoresistance exhibits negative and linear field dependence in all current and field configurations. These results clearly indicate Sr₄(Ru_1-xMn_x)₃O₁₀ is a novelmore »« less

Authors:

Xing, Lingyi ^[1]; Gui, Xin ^[2]; Xie, Weiwei ^[2];

^[3];

^[4];

^[4]; Jin, Rongying ^[1]

Louisiana State Univ., Baton Rouge, LA (United States). Dept. of Physics and Astronomy
Louisiana State Univ., Baton Rouge, LA (United States). Dept. of Chemistry
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Neutron Scattering Division
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Materials Science & Technology Division

Publication Date:: 2018-09-05

Research Org.:: Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division; Board of Regents State of Louisiana Research Competitiveness Subprogram (RCS)

OSTI Identifier:: 1474446

Grant/Contract Number:: AC05-00OR22725; SC0016315; LEQSF(2017-20)-RD-A-08

Resource Type:: Accepted Manuscript

Journal Name:: Scientific Reports

Additional Journal Information:: Journal Volume: 8; Journal Issue: 1; Journal ID: ISSN 2045-2322

Publisher:: Nature Publishing Group

Country of Publication:: United States

Language:: English

Subject:: 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY

Citation Formats


                    Xing, Lingyi, Gui, Xin, Xie, Weiwei, Cao, Huibo, Yan, Jiaqiang, Sales, Brian C., and Jin, Rongying. Mn-induced Ferromagnetic Semiconducting Behavior with Linear Negative Magnetoresistance in Sr4(Ru1-xMnx)3O10 Single Crystals.  United States: N. p., 2018. 
Web.  doi:10.1038/s41598-018-31679-w.

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                    Xing, Lingyi, Gui, Xin, Xie, Weiwei, Cao, Huibo, Yan, Jiaqiang, Sales, Brian C., & Jin, Rongying. Mn-induced Ferromagnetic Semiconducting Behavior with Linear Negative Magnetoresistance in Sr4(Ru1-xMnx)3O10 Single Crystals.  United States.  https://doi.org/10.1038/s41598-018-31679-w

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                    Xing, Lingyi, Gui, Xin, Xie, Weiwei, Cao, Huibo, Yan, Jiaqiang, Sales, Brian C., and Jin, Rongying. Wed .  
"Mn-induced Ferromagnetic Semiconducting Behavior with Linear Negative Magnetoresistance in Sr4(Ru1-xMnx)3O10 Single Crystals".  United States.  https://doi.org/10.1038/s41598-018-31679-w.  https://www.osti.gov/servlets/purl/1474446.

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@article{osti_1474446,

  title        = {Mn-induced Ferromagnetic Semiconducting Behavior with Linear Negative Magnetoresistance in Sr4(Ru1-xMnx)3O10 Single Crystals},

  author       = {Xing, Lingyi and Gui, Xin and Xie, Weiwei and Cao, Huibo and Yan, Jiaqiang and Sales, Brian C. and Jin, Rongying},

  abstractNote = {Triple-layered Sr4Ru3O10 is a unique ferromagnet with the central RuO6 layer behaving differently from two outer layers both crystallographically and magnetically. Here, we report that the partial substitution of Ru by smaller Mn gives rise to modification in crystal structure, electronic and magnetic properties of Sr4(Ru1-xMnx)3O10. Through the single crystal X-ray diffraction refinement, we find that (Ru/Mn)O6 octahedral rotation is no longer detectable at x ≥ 0.23, leading to the tetragonal structure. The magnetization measurements indicate the ferromagnetic transition temperature TC decreases from 105 K for x = 0 to 30 K for x = 0.41, with the reduced magnetic moment as well. Remarkably, Mn doping results in the change of magnetic anisotropy from the easy c axis in x = 0 to the easy ab plane seen in x = 0.34 and 0.41. Such change also removes the ab-plane metamagnetic transition observed in x = 0. Furthermore, the electrical resistivity increases with increasing x showing semiconducting behavior with Δ ~ 10 meV for x = 0.34 and 30 meV for x = 0.41. Under applied magnetic field, the magnetoresistance exhibits negative and linear field dependence in all current and field configurations. These results clearly indicate Sr4(Ru1-xMnx)3O10 is a novel ferromagnetic semiconductor with exotic magnetotransport properties.},

  doi          = {10.1038/s41598-018-31679-w},

  journal      = {Scientific Reports},

  number       = 1,

  volume       = 8,

  place        = {United States},

  year         = {2018},

  month        = {9}

}

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Works referencing / citing this record:

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Title: Mn-induced Ferromagnetic Semiconducting Behavior with Linear Negative Magnetoresistance in Sr4(Ru1-xMnx)3O10 Single Crystals

Abstract

Citation Formats

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Neutron Powder Diffraction Study of the Crystal Structures of Sr2RuO4 and Sr2IrO4 at Room Temperature and at 10 K journal, October 1994

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Electronic structure of SrRu 1 − x Mn x O 3 studied by photoemission and x-ray absorption spectroscopy journal, June 2010

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Linear negative magnetoresistance in two-dimensional Lorentz gases journal, March 2018

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Title: Mn-induced Ferromagnetic Semiconducting Behavior with Linear Negative Magnetoresistance in Sr₄(Ru_1-xMn_x)₃O₁₀ Single Crystals

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Anomalous Low-Field Classical Magnetoresistance in Two Dimensions
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The Change of Electrical Conductivity in Strong Magnetic Fields. Part I. Experimental Results
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Negative linear classical magnetoresistance in a corrugated two-dimensional electron gas
journal, December 2004

Magnetic phase diagram of ${Ca}_{2 - x} {Sr}_{x} {RuO}_{4}$ governed by structural distortions
journal, June 2001

In-depth study of the $H - T$ phase diagram of ${Sr}_{4} {Ru}_{3} O_{10}$ by magnetization experiments
journal, May 2018

Ferromagnetism in ${Sr}_{4} {Ru}_{3} O_{10} :$ Relationship to other layered metallic oxides
journal, September 1997

Ground state in ${Sr}_{3} {Ru}_{2} O_{7} :$ Fermi liquid close to a ferromagnetic instability
journal, September 2000

Positive and negative linear magnetoresistance of graphite
journal, January 2004

Classical magnetotransport of inhomogeneous conductors
journal, September 2005

Neutron Diffraction Study of the Structural Distortions in Sr3Ru2O7
journal, November 2000

Structure, Raman scattering, and transport properties of boron-doped graphite
journal, May 2001

Missing magnetism in Sr4Ru3O10: Indication for Antisymmetric Exchange Interaction
journal, June 2017

Quantum linear magnetoresistance; solution of an old mystery
journal, August 2003

Ferromagnetism Stabilized by Lattice Distortion at the Surface of the p-Wave Superconductor Sr2RuO4
journal, August 2000

Superconductivity in a layered perovskite without copper
journal, December 1994

Negative magnetoresistance in carbons and diffuse scattering at crystallite boundaries
journal, October 1968

Dependence of magnetoresistivity on charge-carrier density in metallic ferromagnets and doped magnetic semiconductors
journal, October 1998

Nature of the apical and planar oxygen bonds in the Sr $_{n + 1}$ Ru $_{n}$ O $_{3 n + 1}$ family ( $n = 1, 2, 3$ )
journal, November 2013

Electronic structure and magnetism of ${Sr}_{3} {Ru}_{2} O_{7}$
journal, March 2001

Anisotropy of magnetoresistivities in ${Sr}_{4} {Ru}_{3} O_{10}$ : Evidence for an orbital-selective metamagnetic transition
journal, May 2010

Anomalous negative magnetoresistance caused by non-Markovian effects
journal, November 2003

Metamagnetism and Critical Fluctuations in High Quality Single Crystals of the Bilayer Ruthenate ${Sr}_{3} {Ru}_{2} O_{7}$
journal, March 2001

Neutron Powder Diffraction Study of the Crystal Structures of Sr2RuO4 and Sr2IrO4 at Room Temperature and at 10 K
journal, October 1994

Competition Between Antiferromagnetism and Ferromagnetism in Sr2RuO4 Probed by Mn and Co Doping
journal, October 2013

Electronic structure of ${SrRu}_{1 - x} {Mn}_{x} O_{3}$ studied by photoemission and x-ray absorption spectroscopy
journal, June 2010

Non-saturating magnetoresistance in heavily disordered semiconductors
journal, November 2003

Quantum linear magnetoresistance
journal, March 2000

Magnetic Interactions in Ternary Ruthenium Oxides
journal, September 1966

Linear negative magnetoresistance in two-dimensional Lorentz gases
journal, March 2018

Electronic structure trends in the Sr $_{n + 1}$ Ru $_{n}$ O $_{3 n + 1}$ family ( $n = 1, 2, 3$ )
journal, April 2011

Phase diagram of the electronic states of trilayered ruthenate ${Sr}_{4} {Ru}_{3} O_{10}$
journal, March 2007

Magnetic Field-Tuned Quantum Criticality in the Metallic Ruthenate Sr3Ru2O7
journal, October 2001

Double metamagnetic transition in ${Sr}_{4} {Ru}_{3} O_{10}$
journal, November 2014

Impurity-induced transition to a Mott insulator in ${Sr}_{3} {Ru}_{2} O_{7}$
journal, September 2005

Itinerant ferromagnetism to insulating antiferromagnetism: A magnetic and transport study of single crystal ${SrRu}_{1 - x} {Mn}_{x} O_{3} (0 ⩽ x < 0.60)$
journal, January 2005

Negative Magnetoresistance in the Anderson Localized States
journal, January 1979

Interface-induced magnetic polar metal phase in complex oxides
journal, November 2019